Journal Description
Atmosphere
Atmosphere
is an international, peer-reviewed, open access journal of scientific studies related to the atmosphere published monthly online by MDPI. The Italian Aerosol Society (IAS) and Working Group of Air Quality in European Citizen Science Association (ECSA) are affiliated with Atmosphere and their members receive a discount on the article processing charges.
- Open Access— free for readers, with article processing charges (APC) paid by authors or their institutions.
- High Visibility: indexed within Scopus, SCIE (Web of Science), Ei Compendex, GEOBASE, GeoRef, Inspec, CAPlus / SciFinder, Astrophysics Data System, and other databases.
- Journal Rank: CiteScore - Q2 (Environmental Science (miscellaneous))
- Rapid Publication: manuscripts are peer-reviewed and a first decision is provided to authors approximately 17.7 days after submission; acceptance to publication is undertaken in 2.8 days (median values for papers published in this journal in the second half of 2023).
- Recognition of Reviewers: reviewers who provide timely, thorough peer-review reports receive vouchers entitling them to a discount on the APC of their next publication in any MDPI journal, in appreciation of the work done.
- Testimonials: See what our editors and authors say about the Atmosphere.
- Companion journal: Meteorology.
Impact Factor:
2.9 (2022);
5-Year Impact Factor:
3.0 (2022)
Latest Articles
Modeling Yield of Irrigated and Rainfed Bean in Central and Southern Sinaloa State, Mexico, Based on Essential Climate Variables
Atmosphere 2024, 15(5), 573; https://doi.org/10.3390/atmos15050573 - 07 May 2024
Abstract
The goal was to model irrigated (IBY) and rainfed (RBY) bean yields in central (Culiacán) and southern (Rosario) Sinaloa state as a function of the essential climate variables soil moisture, temperature, reference evapotranspiration, and precipitation. For Sinaloa, for the period 1982–2013 (October–March), the
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The goal was to model irrigated (IBY) and rainfed (RBY) bean yields in central (Culiacán) and southern (Rosario) Sinaloa state as a function of the essential climate variables soil moisture, temperature, reference evapotranspiration, and precipitation. For Sinaloa, for the period 1982–2013 (October–March), the following were calculated: (a) temperatures, (b) average degree days for the bean, (c) cumulative reference evapotranspiration, and (d) cumulative effective precipitation. For essential climate variables, (e) daily soil moisture obtained from the European Space Agency and (f) IBY and RBY from the Agrifood and Fisheries Information Service were used. Multiple linear regressions were significant for predicting IBY–RBY (dependent variables) as a function of essential climate variables (independent variables). The four models obtained were significantly predictive: IBY–Culiacán (Pearson correlation (PC) = 0.590 > Pearson critical correlation (CPC) = |0.349|), RBY–Culiacán (PC = 0.734 > CPC = |0.349|), IBY–Rosario (PC = 0.621 > CPC = |0.355|), and RBY–Rosario (PC = 0.532 > CPC = |0.349|). Due to the lack of irrigation depth data, many studies only focus on modeling RBY; this study is the first in Sinaloa to predict IBY and RBY based on essential climate variables, contributing to the production of sustainable food.
Full article
(This article belongs to the Section Climatology)
Open AccessReview
Review on Sampling Methods and Health Impacts of Fine (PM2.5, ≤2.5 µm) and Ultrafine (UFP, PM0.1, ≤0.1 µm) Particles
by
Balendra V. S. Chauhan, Karina Corada, Connor Young, Kirsty L. Smallbone and Kevin P. Wyche
Atmosphere 2024, 15(5), 572; https://doi.org/10.3390/atmos15050572 - 07 May 2024
Abstract
Airborne particulate matter (PM) is of great concern in the modern-day atmosphere owing to its association with a variety of health impacts, such as respiratory and cardiovascular diseases. Of the various size fractions of PM, it is the finer fractions that are most
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Airborne particulate matter (PM) is of great concern in the modern-day atmosphere owing to its association with a variety of health impacts, such as respiratory and cardiovascular diseases. Of the various size fractions of PM, it is the finer fractions that are most harmful to health, in particular ultrafine particles (PM0.1; UFPs), with an aerodynamic diameter ≤ 100 nm. The smaller size fractions, of ≤2.5 µm (PM2.5; fine particles) and ≤0.1 µm (PM0.1; ultrafine particles), have been shown to have numerous linkages to negative health effects; however, their collection/sampling remains challenging. This review paper employed a comprehensive literature review methodology; 200 studies were evaluated based on the rigor of their methodologies, including the validity of experimental designs, data collection methods, and statistical analyses. Studies with robust methodologies were prioritised for inclusion. This review paper critically assesses the health risks associated with fine and ultrafine particles, highlighting vehicular emissions as the most significant source of particulate-related health effects. While coal combustion, diesel exhaust, household wood combustors’ emissions, and Earth’s crust dust also pose health risks, evidence suggests that exposure to particulates from vehicular emissions has the greatest impact on human health due to their widespread distribution and contribution to air pollution-related diseases. This article comprehensively examines current sampling technologies, specifically focusing on the collection and sampling of ultrafine particles (UFP) from ambient air to facilitate toxicological and physiochemical characterisation efforts. This article discusses diverse approaches to collect fine and ultrafine particulates, along with experimental endeavours to assess ultrafine particle concentrations across various microenvironments. Following meticulous evaluation of sampling techniques, high-volume air samplers such as the Chem Vol Model 2400 High Volume Cascade Impactor and low-volume samplers like the Personal Cascade Impactor Sampler (PCIS) emerge as effective methods. These techniques offer advantages in particle size fractionation, collection efficiency, and adaptability to different sampling environments, positioning them as valuable tools for precise characterisation of particulate matter in air quality research and environmental monitoring.
Full article
(This article belongs to the Section Air Quality and Human Health)
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Open AccessArticle
Sand Supply Affects Wind Erosion Efficiency and Sand Transport on Sand-Cemented Body Mulch Bed
by
Jie Zhou, Haifeng Wang and Beibei Han
Atmosphere 2024, 15(5), 571; https://doi.org/10.3390/atmos15050571 - 07 May 2024
Abstract
Sand-cemented bodies (SCBs) are naturally distributed in some interdune corridors in the central Taklimakan Desert, northwest China. In this study, field-collected SCB particles were used as the experimental material, and wind tunnel experiments were conducted with different sand supplies, wind velocities, and SCB
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Sand-cemented bodies (SCBs) are naturally distributed in some interdune corridors in the central Taklimakan Desert, northwest China. In this study, field-collected SCB particles were used as the experimental material, and wind tunnel experiments were conducted with different sand supplies, wind velocities, and SCB coverages to evaluate SCB wind erosion efficiency and vertical mass flux. The results showed that wind erosion efficiency decreased as SCB coverage increased. When the SCB coverage was above 40%, sand deposition processes occurred only under saturated sand flow, while sand transport remained unaffected by increases in SCB coverage under unsaturated sand flow. Under saturated flow, the highest concentrations of transported sand were found at 0–6 cm above the surface, and the main sand bed process was deposition. The sand bed process changed from aeolian erosion to deposition with increasing SCB coverage and tended to remain stable until the SCB coverage exceeded 40%. By contrast, under unsaturated sand flow, the sand bed process was primarily aeolian erosion, and the highest concentrations of transported sand were found at 0–4 cm above the surface. At high SCB coverage levels (more than 40%), a general balance between aeolian erosion and deposition processes was reached. In summary, increasing SCB coverage had a significant impact on surface wind erosion processes. Thus, SCBs can be used as a novel sand retention material.
Full article
(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)
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Open AccessArticle
Resolving the Loss of Intermediate-Size Speech Aerosols in Funnel-Guided Particle Counting Measurements
by
Tayeb Kakeshpour and Adriaan Bax
Atmosphere 2024, 15(5), 570; https://doi.org/10.3390/atmos15050570 - 07 May 2024
Abstract
Modeling of airborne virus transmission and protection against it requires knowledge of the amount of biofluid emitted into the atmosphere and its viral load. Whereas viral concentrations in biofluids are readily measured by quantitative PCR, the total volume of fluids aerosolized during speaking,
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Modeling of airborne virus transmission and protection against it requires knowledge of the amount of biofluid emitted into the atmosphere and its viral load. Whereas viral concentrations in biofluids are readily measured by quantitative PCR, the total volume of fluids aerosolized during speaking, as measured by different researchers using various technologies, differs by several orders of magnitude. We compared collection methods in which the aerosols first enter into a low-humidity chamber either by direct injection or via commonly used funnel and tubing arrangements, followed by standard optical particle sizer measurement. This “collect first, measure later” approach sacrifices the recording of the temporal correlation between aerosol generation and sound types such as plosives and vowels. However, the direct-injection mode prevents inertia deposition associated with the funnel arrangements and reveals far more intermediate-size (5–20 μm in diameter) particles that can dominate the total mass of ejected respiratory aerosol. The larger aerosol mass observed with our method partially reconciles the large discrepancy between the SARS-CoV-2 infectious dose estimated from superspreader event analyses and that from human challenge data. Our results also impact measures to combat airborne virus transmission because they indicate that aerosols that settle faster than good room ventilation rates can dominate this process.
Full article
(This article belongs to the Special Issue Atmospheric Bioaerosols: Detection, Characterization and Modelling)
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Open AccessArticle
A Short-Term Forecasting Method for High-Frequency Broadcast MUF Based on LSTM
by
Shengyun Ji, Guojin He, Qiao Yu, Yafei Shi, Jun Hu and Lin Zhao
Atmosphere 2024, 15(5), 569; https://doi.org/10.3390/atmos15050569 - 07 May 2024
Abstract
This paper proposes a short-term forecasting method for high-frequency broadcast Maximum Usable Frequency (MUF) based on Long Short-Term Memory (LSTM) to meet the demand for refined and precise high-frequency broadcast coverage. Based on the existing infrastructure of broadcast and television stations, we established
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This paper proposes a short-term forecasting method for high-frequency broadcast Maximum Usable Frequency (MUF) based on Long Short-Term Memory (LSTM) to meet the demand for refined and precise high-frequency broadcast coverage. Based on the existing infrastructure of broadcast and television stations, we established an experimental verification system to collect data for approximately three years. Two links were selected based on data quality: Urumqi to Lhasa and Lanzhou to Lhasa. A short-term forecast of MUF was conducted using the data from these two links. Comparison and analysis were conducted between the forecasting results of our model and those of the REC533 model. Our proposed method outperforms the REC533 forecasting results overall, with a reduction in root mean square error (RMSE) of 0.66 MHz and an improvement in forecast accuracy of 14.77%. The comparison result demonstrates the feasibility and accuracy of our model.
Full article
(This article belongs to the Special Issue Intelligent Modeling of the Ionosphere and Troposphere for Radio Application)
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Open AccessArticle
Analyses and Simulations of PM2.5 Pollution Characteristics under the Influence of the New Year’s Day Effects in China
by
Qiao Shi, Tangyan Hou, Chengli Wang, Zhe Song, Ningning Yao, Yuhai Sun, Boqiong Jiang, Pengfei Li, Zhibin Wang and Shaocai Yu
Atmosphere 2024, 15(5), 568; https://doi.org/10.3390/atmos15050568 - 03 May 2024
Abstract
Regional haze often occurs after the New Year holiday. To explore the characteristics of PM2.5 pollutions under the influence of the New Year’s Day effect, this study analyzed the spatiotemporal changes relating to PM2.5 during and around the New Year’s Day
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Regional haze often occurs after the New Year holiday. To explore the characteristics of PM2.5 pollutions under the influence of the New Year’s Day effect, this study analyzed the spatiotemporal changes relating to PM2.5 during and around the New Year’s Day holiday in China from 2015 to 2022, and used the Weather Research and Forecasting-Community Multiscale Air Quality (WRF-CMAQ) model to study the effects of human activities and meteorological factors on PM2.5 pollutions, as well as the differences in the contributions of different industries to PM2.5 pollutions. The results show that for the entire study period (i.e., before, during, and after the New Year’s Day holiday) from 2015 to 2022, the average concentrations of PM2.5 in China decreased by 41.9% overall. In 2019~2022, the New Year’s Day effect was significant, meaning that the average concentrations of PM2.5 increased by 18.9~46.8 μg/m3 from before to after the New Year’s Day holiday, with its peak occurring (64.3~74.9 μg/m3) after the holiday. In terms of spatial differences, the average concentrations of PM2.5 were higher in the Beijing–Tianjin–Hebei region, the Yangtze River Delta, and central China. Moreover, the Beijing–Tianjin–Hebei region and its surrounding areas, the Chengdu–Chongqing region, the Fenwei Plain, and the middle reaches of the Yangtze River region were greatly affected by the New Year’s Day effect. Human activities led to higher increases in PM2.5 in Henan, Hubei, Hebei, and Anhui on 3 and 4 January 2022. If the haze was accompanied by cloudy days or weak precipitation, the accumulation of surface water vapor and atmospheric aerosols further increased the possibility of heavy pollution. It was found that, for the entire study period, PM2.5 generated by residential sources contributed the vast majority (60~100 μg/m3) of PM2.5 concentrations, and that the main industry sources that caused changes in time distributions were industrial and transportation sources.
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(This article belongs to the Section Air Quality)
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Open AccessBrief Report
Why Does the Ensemble Mean of CMIP6 Models Simulate Arctic Temperature More Accurately Than Global Temperature?
by
Petr Chylek, Chris K. Folland, James D. Klett, Muyin Wang, Glen Lesins and Manvendra K. Dubey
Atmosphere 2024, 15(5), 567; https://doi.org/10.3390/atmos15050567 - 03 May 2024
Abstract
An accurate simulation and projection of future warming are needed for a proper policy response to expected climate change. We examine the simulations of the mean global and Arctic surface air temperatures by the CMIP6 (Climate Models Intercomparison Project phase 6) climate models.
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An accurate simulation and projection of future warming are needed for a proper policy response to expected climate change. We examine the simulations of the mean global and Arctic surface air temperatures by the CMIP6 (Climate Models Intercomparison Project phase 6) climate models. Most models overestimate the observed mean global warming. Only seven out of 19 models considered simulate global warming that is within ±15% of the observed warming between the average of the 2014–2023 and 1961–1990 reference period. Ten models overestimate global warming by more than 15% and only one of the models underestimates it by more than 15%. Arctic warming is simulated by the CMIP6 climate models much better than the mean global warming. The reason is an equal spread of over and underestimates of Arctic warming by the models, while most of the models overestimate the mean global warming. Eight models are within ±15% of the observed Arctic warming. Only three models are accurate within ±15% for both mean global and Arctic temperature simulations.
Full article
(This article belongs to the Special Issue Arctic Climate Change: Observations, Modeling, and Arctic Amplification)
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Open AccessArticle
Irrigation Schedule Optimization for Wheat and Sunflower Intercropping under Water Supply Restrictions in Inner Mongolia, China
by
Hexiang Zheng, Hongfei Hou, Jiabin Wu, Delong Tian and Ping Miao
Atmosphere 2024, 15(5), 566; https://doi.org/10.3390/atmos15050566 - 03 May 2024
Abstract
Precise water management is essential for the efficient development of irrigated agricultural crops in the Hetao Irrigation Area of Inner Mongolia. Given the severe water scarcity in the region and the significant use of intercropping as a cropping method, the development of rational
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Precise water management is essential for the efficient development of irrigated agricultural crops in the Hetao Irrigation Area of Inner Mongolia. Given the severe water scarcity in the region and the significant use of intercropping as a cropping method, the development of rational irrigation scheduling is crucial. The objective of this work was to combine the ISAREG model with wheat–sunflower intercropping crops in order to enhance the effectiveness of irrigation scheduling in intercropping systems. This was achieved by changing and verifying crucial parameters for simulating irrigation patterns in intercropping. We conducted an assessment of nine irrigation schedules for a wheat–sunflower intercropping system in order to provide a range of irrigation scenarios that effectively fulfill the water requirements of the system. In light of this, we suggested implementing restrictions on the dates and volumes of irrigation based on the demand for agricultural irrigation. This approach aimed to establish irrigation schedules that are highly efficient and tailored to the specific crops in the area. As a result, we achieved a water use efficiency rate of 100%, saved 28.78% of water resources, optimized crop irrigation schedules, and enhanced crop economics by 6.7%. This study presents a novel and efficient method to optimize agricultural irrigation schedules, boost agricultural water use efficiency, and maximize crop yields in order to promote sustainable agricultural development.
Full article
(This article belongs to the Special Issue Agrometeorology, Agricultural Water Management and Impacts of Extreme Events (2nd Edition))
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Open AccessArticle
Visualising Daily PM10 Pollution in an Open-Cut Mining Valley of New South Wales, Australia—Part I: Identification of Spatial and Temporal Variation Patterns
by
Ningbo Jiang, Matthew L. Riley, Merched Azzi, Praveen Puppala, Hiep Nguyen Duc and Giovanni Di Virgilio
Atmosphere 2024, 15(5), 565; https://doi.org/10.3390/atmos15050565 - 02 May 2024
Abstract
The Upper Hunter Valley is a major coal mining area containing approximately 40% of the currently identified total coal reserves in New South Wales (NSW), Australia. Due to the ongoing increase in mining activities, PM10 (airborne particles with an aerodynamic diameter of less
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The Upper Hunter Valley is a major coal mining area containing approximately 40% of the currently identified total coal reserves in New South Wales (NSW), Australia. Due to the ongoing increase in mining activities, PM10 (airborne particles with an aerodynamic diameter of less than 10 micrometres) pollution has become a major air quality concern in local communities. This paper summarises the spatial and temporal variability modes of PM10 pollution in the region, based on long-term multi-site monitoring data and the application of the rotated principal component analysis (RPCA) and wavelet analysis techniques. RPCA identified two distinct air quality clusters/subregions in the valley: one in the west/northwest and the other in the southeast. Wavelet analysis revealed the annual cycle to be the most persistent temporal mode of PM10 variability in both subregions, with intermittent signals also observed at time scales of around 120, 30~90, and under 30 days. How these variation modes are related to the effects of local PM10 emissions and the influence of meteorology at different time scales deserves further attention in future work. The findings will be used in air quality reporting and forecasting in NSW. The methodology and results can also be useful for air quality research in similar regions elsewhere.
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(This article belongs to the Section Aerosols)
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Open AccessArticle
Wide and Deep Learning Model for Satellite-Based Real-Time Aerosol Retrievals in China
by
Nana Luo, Junxiao Zou, Zhou Zang, Tianyi Chen and Xing Yan
Atmosphere 2024, 15(5), 564; https://doi.org/10.3390/atmos15050564 - 30 Apr 2024
Abstract
Machine learning methods have been recognized as rapid methods for satellite-based aerosol retrievals but have not been widely applied in geostationary satellites. In this study, we developed a wide and deep learning model to retrieve the aerosol optical depth (AOD) using Himawari-8. Compared
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Machine learning methods have been recognized as rapid methods for satellite-based aerosol retrievals but have not been widely applied in geostationary satellites. In this study, we developed a wide and deep learning model to retrieve the aerosol optical depth (AOD) using Himawari-8. Compared to traditional deep learning methods, we embedded a “wide” modeling component and tested the proposed model across China using independent training (2016–2018) and test (2019) datasets. The results showed that the “wide” model improves the accuracy and enhances model interpretability. The estimates exhibited better accuracy (R2 = 0.81, root-mean-square errors (RMSEs) = 0.19, and within the estimated error (EE) = 63%) than those of the deep-only models (R2 = 0.78, RMSE = 0.21, within the EE = 58%). In comparison with extreme gradient boosting (XGBoost) and Himawari-8 V2.1 AOD products, there were also significant improvements. In addition to higher accuracy, the interpretability of the proposed model was superior to that of the deep-only model. Compared with other seasons, higher contributions of spring to the AOD concentrations were interpreted. Based on the application of the wide and deep learning model, the near-real-time variation of the AOD over China could be captured with an ultrafine temporal resolution.
Full article
(This article belongs to the Special Issue Natural Sources Aerosol Remote Monitoring (2nd Edition))
Open AccessArticle
Impact of COVID-19 Lockdown on Inhaled Toxic Elements in PM2.5 in Beijing: Composition Characterization and Source-Specific Health Risks Assessment
by
Mingsheng Zhao, Lihong Ren, Xiaoyang Yang, Yuanguan Gao, Gang Li and Yani Liu
Atmosphere 2024, 15(5), 563; https://doi.org/10.3390/atmos15050563 - 30 Apr 2024
Abstract
In early 2020, China experienced a mass outbreak of a novel coronavirus disease (COVID-19). With an aim to evaluate the impact of emission variations on toxic element species in PM2.5 and the health risks associated with inhalation exposure during COVID-19, we collected
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In early 2020, China experienced a mass outbreak of a novel coronavirus disease (COVID-19). With an aim to evaluate the impact of emission variations on toxic element species in PM2.5 and the health risks associated with inhalation exposure during COVID-19, we collected PM2.5 filter samples in Beijing from January 1 to February 28, 2020. Positive matrix factorization (PMF) and a health risk (HR) assessment model were used to assess the health risks of the toxic elements and critical risk sources. The total concentration of eight toxic elements (Se, Cd, Pb, Zn, As, Cu, Ni, and Cr) in Beijing showed a trend of first increasing and then decreasing: full lockdown (322.9 ng m−3) > pre-lockdown (264.2 ng m−3) > partial lockdown (245.3 ng m−3). During the lockdown period, stringent control measures resulted in significant reductions (6−20%) in Zn, Pb, Cd, and Ni levels, while concentrations of Se, As, Cu, and Cr were unexpectedly elevated (14−348%). A total of five sources was identified: traffic emission, coal combustion, dust emission, industrial emission and mixed source of biomass burning and firework combustion. Total carcinogenic risk (TCR) of the selected toxic elements exceeded the US EPA limits for children and adults. As and Cr (IV) were the main contributors to non-carcinogenic and carcinogenic risks, respectively. For source-resolved risks, coal combustion was the main contributor to HI (43%), while industrial emissions were the main cause of TCR (45%). Additionally, increased contributions from coal combustion, biomass burning, and firework combustion during the full lockdown elevated the HI and TCR values.
Full article
(This article belongs to the Section Air Quality and Human Health)
Open AccessReview
Climate Change, Air Pollution, and Human Health in the Kruger to Canyons Biosphere Region, South Africa, and Amazonas, Brazil: A Narrative Review
by
Monika dos Santos
Atmosphere 2024, 15(5), 562; https://doi.org/10.3390/atmos15050562 - 30 Apr 2024
Abstract
There is a 50% possibility that global temperatures will have risen by more than 5 °C by the year 2100. As demands on Earth’s systems grow more unsustainable, human security is clearly at stake. This narrative review provides an overview and synthesis of
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There is a 50% possibility that global temperatures will have risen by more than 5 °C by the year 2100. As demands on Earth’s systems grow more unsustainable, human security is clearly at stake. This narrative review provides an overview and synthesis of findings in relation to climate change, air pollution, and human health within the Global South context, focusing on case study geographic locations in South Africa and Brazil. Two case study regions—the Kruger to Canyons Biosphere region of South Africa and the Amazon region of Brazil—were the subjects of PubMed literature searches. Technical reports, policy briefs, and grey literature were also narratively synthesized. The burning of wood for fuel, as witnessed in Agincourt, and forest fires, such as those seen in the Amazon rainforest, release air pollutants such as methane and black carbon, which are strong short-lived climate pollutants (SLCPs) which fuel climate change and adversely affect human health. SLCPs have a brief lifetime in the atmosphere, but they frequently have a far larger potential for global warming than carbon dioxide (CO2). Most air pollution in geographic case study areas, that are home to human settlements, is due to the burning of wood and other biomasses that are pollutants. These areas are seen to be important for climate and health responses, and if constructive action is taken to switch to other modes of electricity generation (such as solar power) and the prevention of deforestation, the worst of the impacts may still be mitigated in these regions. Authorities should also establish a monitoring strategy for air quality, as well as enforce air quality regulations that safeguard public health.
Full article
(This article belongs to the Special Issue Climate Change, Air Pollution and Human Health: Past, Present and Future)
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Open AccessArticle
Volcanic Glass as a Proxy for Paleotopography Suggests New Features in Late-Miocene Oregon
by
Julian Cohen, John Bershaw and Richard Hugo
Atmosphere 2024, 15(5), 561; https://doi.org/10.3390/atmos15050561 - 30 Apr 2024
Abstract
Volcanic glass has been used extensively as a paleoaltimeter. Deuterium (2H) concentrations in glass have been found to be stable over geologic timescales, making δ2H (also known as δD) a reliable proxy for ancient water chemistry. However, continued work
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Volcanic glass has been used extensively as a paleoaltimeter. Deuterium (2H) concentrations in glass have been found to be stable over geologic timescales, making δ2H (also known as δD) a reliable proxy for ancient water chemistry. However, continued work revolves around better understanding how different factors affect preserved water in volcanic ash. Here, we analyze δD in the Rattlesnake Tuff (RST), a widespread ca. 7 Ma ash-flow tuff, and create a paleoisoscape to assess variations in δD across Oregon during that time. To this end, 16 ash samples were collected across central and eastern Oregon from various flow units within the RST. Samples were analyzed for δD using a temperature conversion elemental analyzer (TC/EA) connected to a mass spectrometer and elemental composition using a scanning electron microscope (SEM). We compared the isotopic results to modern water and published ancient water proxy data to better constrain changes in climate and topography across Oregon throughout the Neogene. We also estimated wt. % H2O by calculating excess (non-stoichiometric) oxygen from SEM elemental data. We did not observe significant variations in δD among the flow units from single locations, nor was there a significant relationship between the prepared glass shard composition and wt. % H2O or δD, supporting the use of volcanic glass as a reliable paleoenvironmental indicator. Our results show significant spatial variation in δDwater values of RST, ranging from −107‰ to −154‰. δD values of ancient glass were similar to modern water near the Cascade Mountains but became relatively negative to the east near the inferred eruptive center of the RST, suggesting that a significant topographic feature existed in the vicinity of the RST eruptive center that has since subsided.
Full article
(This article belongs to the Section Climatology)
Open AccessArticle
A Year-Long Measurement and Source Contributions of Volatile Organic Compounds in Nanning, South China
by
Ying Wu, Zhaoyu Mo, Qinqin Wu, Yongji Fan, Xuemei Chen, Hongjiao Li, Hua Lin, Xishou Huang, Hualei Tang, Donglan Liao, Huilin Liu and Ziwei Mo
Atmosphere 2024, 15(5), 560; https://doi.org/10.3390/atmos15050560 (registering DOI) - 30 Apr 2024
Abstract
Severe ozone (O3) pollution has been recorded in China in recent years. The key precursor, volatile organic compounds (VOCs), is still not well understood in Nanning, which is a less developed city compared to other megacities in China. In this study,
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Severe ozone (O3) pollution has been recorded in China in recent years. The key precursor, volatile organic compounds (VOCs), is still not well understood in Nanning, which is a less developed city compared to other megacities in China. In this study, a year-long measurement of VOCs was conducted from 1 October 2020 to 30 September 2021, to characterize the ambient variations and apportion the source contributions of VOCs. The daily-averaged concentration of VOCs was measured to be 26.4 ppb, ranging from 3.2 ppb to 136.2 ppb across the whole year. Alkanes and oxygenated VOCs (OVOCs) were major species, contributing 46.9% and 25.2% of total VOC concentrations, respectively. Propane, ethane, and ethanol were the most abundant in Nanning, which differed from the other significant species, such as toluene (3.7 ppb) in Guangzhou, ethylene (3.8 ppb) in Nanjing, and isopentane (5.5 ppb), in Chengdu. The positive matrix factorization (PMF) model resolved six source factors, including vehicular emission (contributing 33% of total VOCs), NG and LPG combustion (19%), fuel burning (17%), solvent use (16%), industry emission (10%), and biogenic emission (5%). This indicated that Nanning was less affected by industrial emission compared with other megacities of China, with industry contributing 12–50%. Ethylene, m/p-xylene, butane, propylene, and isoprene were key species determined by ozone formation potential (OFP) analysis, which should be priority-controlled. The variations in estimated OFP and observed O3 concentrations were significantly different, suggesting that VOC reactivity-based strategies as well as meteorological and NOx effects should be considered collectively in controlling O3 pollution. This study presents a year-long dataset of VOC measurements in Nanning, which gives valuable implications for VOC control in terms of key sources and reactive species and is also beneficial to the formulation of effective ozone control strategies in other less developed regions of China.
Full article
(This article belongs to the Special Issue Urban VOC Emission, Transport, and Chemistry (VOC/ETC))
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Open AccessArticle
Analysis of Ozone Pollution Characteristics, Meteorological Effects, and Transport Sources in Zhuzhou, China
by
Bei Yan, Jia Luo, Min Zhang, Yi Zhang, Tongjue Xiao, Lu Wang, Bo Liu, Yunjuan Han, Gongxiu He, Lili Yang and Zhihong Huang
Atmosphere 2024, 15(5), 559; https://doi.org/10.3390/atmos15050559 - 30 Apr 2024
Abstract
Based on the hourly surface ozone (O3) observations and meteorological data from Zhuzhou in 2021, the pollution characteristics and influencing factors of O3 in Zhuzhou were investigated in the study. In addition, the Potential Source Contribution Function (PSCF) and Concentration
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Based on the hourly surface ozone (O3) observations and meteorological data from Zhuzhou in 2021, the pollution characteristics and influencing factors of O3 in Zhuzhou were investigated in the study. In addition, the Potential Source Contribution Function (PSCF) and Concentration Weighted Trajectory (CWT) analysis methods were employed to analyze the transmission paths and potential pollution sources of O3 pollution in Zhuzhou. The results showed that the total number of days with O3 exceeding the standard at all monitoring stations in Zhuzhou was 142 days in 2021. The overall air quality was less affected by SO2, NO2, and CO, and the trend of O3 pollution was still increasing. The concentrations of O3, CO, and NO2 varied significantly in different months, and the variation of O3 exhibited a “double-peak” pattern, with the peak value occurring in September. The O3 concentration in urban areas was significantly higher than that in suburban areas. Meteorological conditions had a significant impact on the degree of O3 pollution in Zhuzhou. The average wind speed in Zhuzhou throughout the year was 1.7 m/s, and the prevailing wind direction in summer was southeast, with a frequency of 16%. O3 pollution was mainly transported by short-distance airflow during the over-standard periods in 2021, accounting for 37.64%. The main source of O3 pollutant was from Jiangxi Province in the east, with the shortest distance of regional transport and the highest O3 concentration. In addition, transportation from central Guangdong Province, western Jiangxi Province, and central Hubei Province also had a significant impact.
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(This article belongs to the Special Issue Air Pollution in Urban and Regional Level: Sources, Sinks and Transportation (2nd Edition))
Open AccessArticle
The Wind Profile Characteristics of Super Typhoon Lekima Based on Field Measurement
by
Yanru Wang, Qianqian Qi, Shuqin Zheng, Bin Fu, Maoyu Zhang, Xu Wang, Chuanxiong Zhang and Lei Zhou
Atmosphere 2024, 15(5), 558; https://doi.org/10.3390/atmos15050558 - 30 Apr 2024
Abstract
Many cities in coastal areas are prone to typhoon disasters due to their location on the Pacific storm path, and the direct effect of catastrophic winds can lead to the destruction of low-rise buildings and severe damage to high-rise structures. The purpose of
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Many cities in coastal areas are prone to typhoon disasters due to their location on the Pacific storm path, and the direct effect of catastrophic winds can lead to the destruction of low-rise buildings and severe damage to high-rise structures. The purpose of this study was to enhance the understanding of boundary layer wind profiles of strong typhoons in coastal areas and reduce property losses and casualties caused by wind disasters. Based on the field measurements of wind profile acoustic radar in coastal areas, the variation characteristics of the boundary layer wind profile during the passage of super typhoon Lekima were first studied in depth, and the evolution law of the typhoon boundary layer profile was summarized. Then, the effects of typhoon horizontal structure, topography, wind speed, and time distance on the characteristics of the typhoon profile were discussed, respectively. Finally, the evolution characteristics of wind profile parameters were obtained by fitting three wind profile theoretical models. Due to the strong variability of typhoon profile morphology, the theoretical model of wind profile is only applicable to the wind profile from the bottom to the low-level jet height of typhoons, while wind parameters are closely related to the spatial location of the typhoon wind field.
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(This article belongs to the Topic Condition Perception and Performance Evaluation of Engineering Structures)
Open AccessArticle
Estimating Concurrent Probabilities of Compound Extremes: An Analysis of Temperature and Rainfall Events in the Limpopo Lowveld Region of South Africa
by
Caston Sigauke and Thakhani Ravele
Atmosphere 2024, 15(5), 557; https://doi.org/10.3390/atmos15050557 - 30 Apr 2024
Abstract
In recent years, there has been increasing interest in the joint modelling of compound extreme events such as high temperatures and low rainfall. The increase in the frequency of occurrence of these events in many regions has necessitated the development of models for
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In recent years, there has been increasing interest in the joint modelling of compound extreme events such as high temperatures and low rainfall. The increase in the frequency of occurrence of these events in many regions has necessitated the development of models for estimating the concurrent probabilities of such compound extreme events. The current study discusses an application of copula models in predicting the concurrent probabilities of compound low rainfall and high-temperature events using data from the Lowveld region of the Limpopo province in South Africa. The second stage discussed two indicators for monitoring compound high temperature and low rainfall events. Empirical results from the study show that elevations ranging from 100–350 m, 350–700 m and 700–1200 m exhibit varying probabilities of experiencing drought, with mild droughts having approximately 64%, 66%, and 65% chances, moderate droughts around 36%, 39%, and 38%, and severe droughts at approximately 16%, 19%, and 18%, respectively. Furthermore, the logistic regression models incorporating the southern oscillation index as a covariate yielded comparable results of copula-based models. The methodology discussed in this paper is robust and can be applied to similar datasets in any regional setting globally. These findings could be useful to disaster management decision makers, helping them formulate effective mitigation strategies and emergency response plans.
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(This article belongs to the Special Issue Extreme Weather Events in a Warming Climate)
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Open AccessArticle
FY-4A Measurement of Cloud-Seeding Effect and Validation of a Catalyst T&D Algorithm
by
Liangrui Yan, Yuquan Zhou, Yixuan Wu, Miao Cai, Chong Peng, Can Song, Shuoyin Liu and Yubao Liu
Atmosphere 2024, 15(5), 556; https://doi.org/10.3390/atmos15050556 - 30 Apr 2024
Abstract
The transport and dispersion (T&D) of catalyst particles seeded by weather modification aircraft is crucial for assessing their weather modification effects. This study investigates the capabilities of the Chinese geostationary weather satellite FY-4A for identifying the physical response of cloud seeding with AgI-based
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The transport and dispersion (T&D) of catalyst particles seeded by weather modification aircraft is crucial for assessing their weather modification effects. This study investigates the capabilities of the Chinese geostationary weather satellite FY-4A for identifying the physical response of cloud seeding with AgI-based catalysts and continuously monitoring its evolution for a weather event that occurred on 15 December 2019 in Henan Province, China. Satellite measurements are also used to verify an operational catalyst T&D algorithm. The results show that FY-4A exhibits a remarkable capability of identifying the cloud-seeding tracks and continuously tracing their evolution for a period of over 3 h. About 60 min after the cloud seeding, the cloud crystallization track became clear in the FY-4A tri-channel composite cloud image and lasted for about 218 min. During this time period, the cloud track moved with the cloud system about 153 km downstream (northeast of the operation area). An operational catalyst T&D model was run to simulate the cloud track, and the outputs were extensively compared with the satellite observations. It was found that the forecast cloud track closely agreed with the satellite observations in terms of the track widths, morphology, and movement. Finally, the FY-4A measurements show that there were significant differences in the microphysical properties across the cloud track. The effective cloud radius inside the cloud track was up to 15 μm larger than that of the surrounding clouds; the cloud optical thickness was about 30 μm smaller; and the cloud-top heights inside the cloud track were up to 1 km lower. These features indicate that the cloud-seeding catalysts led to the development of ice-phase processes within the supercooled cloud, with the formation of large ice particles and some precipitation sedimentation.
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(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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Open AccessArticle
Evaluating Phoenix Metropolitan Area Ozone Behavior Using Ground-Based Sampling, Modeling, and Satellite Retrievals
by
Jason A. Miech, Pierre Herckes, Matthew P. Fraser, Avelino F. Arellano, Mohammad Amin Mirrezaei and Yafang Guo
Atmosphere 2024, 15(5), 555; https://doi.org/10.3390/atmos15050555 - 30 Apr 2024
Abstract
An oxidizing and harmful pollutant gas, tropospheric ozone is a product of a complex set of photochemical reactions that can make it difficult to enact effective control measures. A better understanding of its precursors including volatile organic compounds (VOCs) and nitrogen oxides (NO
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An oxidizing and harmful pollutant gas, tropospheric ozone is a product of a complex set of photochemical reactions that can make it difficult to enact effective control measures. A better understanding of its precursors including volatile organic compounds (VOCs) and nitrogen oxides (NOx) and their spatial distribution can enable policymakers to focus their control efforts. In this study we used low-cost sensors (LCSs) to increase the spatial resolution of an existing NO2 monitoring network in addition to VOC sampling to better understand summer ozone formation in Maricopa County, Arizona, and observed that afternoon O3 values at the downwind sites were significantly correlated, ~0.27, to the morning NO2 × rate values at the urban sites. Additionally, we looked at the impact of wildfire smoke on ozone exceedances and compared non-smoke days to smoke days. The average O3 on smoke days was approximately 20% higher than on non-smoke days, however, the average NO2 concentration multiplied by estimated photolysis rate (NO2 × rate) values were only 2% higher on smoke days. Finally, we evaluated the ozone sensitivity of the region by calculating HCHO/NO2 ratios using three different datasets: ground, satellite, and model. Although the satellite dataset produced higher HCHO/NO2 ratios than the other datasets, when the proper regime thresholds are applied the three datasets consistently show transition and VOC-limited O3 production regimes over the Phoenix metro area. This suggests a need to implement more VOC emission controls in order to reach O3 attainment in the county.
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(This article belongs to the Section Air Quality)
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Open AccessArticle
Distinguishing Saharan Dust Plume Sources in the Tropical Atlantic Using Elemental Indicators
by
Daniel E. Yeager and Vernon R. Morris
Atmosphere 2024, 15(5), 554; https://doi.org/10.3390/atmos15050554 - 30 Apr 2024
Abstract
The Sahara Desert is the largest contributor of global atmospheric dust aerosols impacting regional climate, health, and ecosystems. The climate effects of these dust aerosols remain uncertain due, in part, to climate model uncertainty of Saharan source region contributions and aerosol microphysical properties.
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The Sahara Desert is the largest contributor of global atmospheric dust aerosols impacting regional climate, health, and ecosystems. The climate effects of these dust aerosols remain uncertain due, in part, to climate model uncertainty of Saharan source region contributions and aerosol microphysical properties. This study distinguishes source region elemental signatures of Saharan dust aerosols sampled during the 2015 Aerosols Ocean Sciences Expedition (AEROSE) in the tropical Atlantic. During the 4-week campaign, cascade impactors size-dependently collected airborne Saharan dust particulate upon glass microfiber filters. Inductively Coupled Plasma Mass Spectrometry (ICP-MS) analysis differentiated metal isotope concentrations within filter samples from various AEROSE dust sampling periods. Back-trajectory analysis and NOAA satellite aerosol optical depth retrievals confirmed source regions of AEROSE ’15 dust samples. Pearson correlational statistics of source region activity and dust isotope concentrations distinguished the elemental signatures of North African potential source areas (PSAs). This study confirmed that elemental indicators of these PSAs remain detectable within dust samples collected far into the marine boundary layer of the tropical Atlantic. Changes detected in dust elemental indicators occurred on sub-weekly timescales across relatively small sampling distances along the 23W parallel of the tropical Atlantic. PSA-2 emissions, covering the western coast of the Sahara, were very strongly correlated (R2 > 0.79) with Ca-44 isotope ratios in AEROSE dust samples; PSA-2.5 emissions, covering eastern Mauritania and western Mali, were very strongly correlated with K-39 ratios; PSA-3 emissions, spanning southwestern Algeria and eastern Mali, were very strongly correlated with Fe-57 and Ti-48 ratios. The abundance of Ca isotopes from PSA-2 was attributed to calcite minerals from dry lakebeds and phosphorous mining activities in Western Sahara, based on source region analysis. The correlation between K isotope ratios and PSA-2.5 was a likely indicator of illite minerals near the El Djouf Desert region, according to corroboration with mineral mapping studies. Fe and Ti ratio correlations with PSA-3 observed in this study were likely indicators of iron and titanium oxides from Sahelian sources still detectable in Atlantic Ocean observations. The rapid changes in isotope chemistry found in AEROSE dust samples provide a unique marker of Saharan source regions and their relative contributions to desert outflows in the Atlantic. These elemental indicators provide source region apportionments of Sahara Desert aerosol flux and deposition into the Atlantic Ocean, as well as a basis for model and satellite validation of Saharan dust emissions for regional climate assessments.
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(This article belongs to the Section Aerosols)
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