A 12-year analysis, from 2005 to 2016, of atmospheric aerosol optical properties focusing for the first time on Northeast Brazil (NEB) was performed based on four different remote sensing datasets: the Moderate Resolution Imaging Spectroradiometer (MODIS), the Aerosol Robotic Network (AERONET), the Cloud-Aerosol LIDAR with Orthogonal Polarization (CALIOP) and a ground-based Lidar from Natal. We evaluated and identified distinct aerosol types, considering Aerosol Optical Depth (AOD) and Angström Exponent (AE). All analyses show that over the NEB, a low aerosol scenario prevails, while there are two distinct seasons of more elevated AOD that occur every year, from August to October and January to March. According to MODIS, AOD values ranges from 0.04 to 0.52 over the region with a mean of 0.20 and occasionally isolated outliers of up to 1.21. Aerosol types were identified as sea spray, biomass burning, and dust aerosols mostly transported from tropical Africa. Three case studies on days with elevated AOD were performed. All cases identified the same aerosol types and modeled HYSPLIT backward trajectories confirmed their source-dependent origins. This analysis is motivated by the implementation of an atmospheric chemistry model with an advanced data assimilation system that will use the observational database over NEB with the model to overcome high uncertainties in the model results induced by still unvalidated emission inventories. Full article

The impact of absorbing aerosols on climate is complex, with their potential positive or negative forcing, depending on many factors, including their height distribution and reflective properties of the underlying background. Measurement data is very limited, due to insufficient remote sensing methods dedicated to the retrieval of their vertical distribution. Columnar values of absorbing aerosol optical depth (AAOD) and single scattering albedo (SSA) are retrieved by the Aerosol Robotic Network (AERONET). However, the number of available results is low due to sky condition and aerosol optical depth (AOD) limitation. Presented research describes results of field campaigns in Strzyżów (South-East Poland, Eastern Europe) dedicated to the comparison of the absorption coefficient and SSA measurements performed with on-ground in-situ devices (aethalomter, nephelometer), small unmanned aerial system (UAS) carrying micro-aethalometer, as well as with lidar/ceilometer. An important aspect is the comparison of measurement results with those delivered by AERONET. Correlation of absorption to scattering coefficients measured on ground (0.79) and correlation of extinction on ground to AOD measured by AERONET (0.77) was visibly higher than correlation between AOD and AAOD retrieved by AERONET (0.56). Columnar SSA was weakly correlated with ground SSA (higher values of columnar SSA), which were mainly explained by hygroscopic effects, increasing scattering coefficient in ambient (wet conditions), and partly high uncertainty of SSA retrieval. AAOD derived with the use of profiles from UAS up to PBL height, was estimated to contribute in average to 37% of the total AAOD. A method of AAOD estimation, in the whole troposphere, with use of measured vertical profiles of absorption coefficient and extinction coefficient profiles from lidars was proposed. AAOD measured with this method has poor correlation with AERONET data, however for some measurements, within PBL, AAOD was higher than reported by AERONET, suggesting potential underestimation in photometric measurement under particular conditions. Correlation of absorption coefficient in profile to on ground measurements decrease with altitude. Measurements of SSA from drones agree well with ground measurements and are lower than results from AERONET, which suggests a larger contribution of absorbing aerosols. As an alternative for AAOD estimation in case of lack of AERONET AAOD data simple models are proposed, which base on AOD scaling with SSA measured with different methods. Proposed solution increase potential of absorption coefficient measurements in vertical profiles and columns of the atmosphere. Presented solutions make measurements of absorption coefficients in vertical profiles more affordable and allow rough estimation of columnar values for the whole atmosphere. Full article

We analyzed a June 2018 Nanjing, China haze event using ground-based and spaceborne sensors, combined with sounding and HYSPLIT backward trajectory data, with the ground-based and spaceborne sensor data exhibiting good consistency. Water vapor content showed significant positive correlation with AOD (aerosol optical depth), and AOD measured in urban and industrial areas was much higher compared to other similar zones. The afternoon convection caused the aerosol uplift during the haze event. Higher aerosol concentration was detected below 2 km. Due to the summer afternoon convective movement, pollutants at high altitude were dominated by small particles, while the overall pollutant mix was dominated by mixed aerosols. During a stable period over June 11–18, a single, near-surface inversion layer, and occasional two inversion layers, stopped pollutant dispersal, with only very stable ocean air mass transport in the southeast direction available. The Air Quality Index drop which took place during June 28–30 was caused by two inversion layers, combined with the immigration of pollutants from inland air masses. Full article

The moderate resolution and imaging spectroradiometer (MODIS) level 2 operational aerosol products that are based on the dark target (DT) method over vegetated regions and the enhanced deep blue (DB) algorithms over bright pixels provide daily global aerosol optical depth (AOD). However, increasing the data coverage by merging the DT and DB merged AOD product has recently become the focus of research. Therefore, this study aims to improve the merged AOD performance by introducing a new regression method (DTBRG), depending on the normalized difference vegetation index values when DT and DB AOD are valid. The DTBRG AOD is validated on a global scale while using aerosol robot network AOD measurements. Merged AOD550s from the MODIS official method and Bilal’s customized methods are evaluated for the same period for comparison. The inter-comparison of merged AOD550s from different methods with an equal number of coincident observations demonstrates that the DTBRG method performs better than the MODIS official algorithm with increased expected error (83% versus 76%), R (0.92 versus 0.90), and decreased bias (−0.001 versus 0.012). Therefore, it can be operationally used for global merged aerosol retrievals. Full article

The Arabian Peninsula is one of the world’s largest sources of mineral dust that includes several major population hotspots. However, until now, few studies have performed a comprehensive quantification of the long-term variability of aerosol species in this region. In this study, the speciation, variability, and distribution of aerosol optical depth over the Arabian Peninsula during 2005–2015 is analyzed by using the modern-era retrospective analysis for research and applications, Version 2 (MERRA-2) model together with satellite retrieved data and AERONET observations and focusing on nine large cities in the region (Dammam, Doha, Dubai, Jeddah, Kuwait, Manama, Muscat, Riyadh, and Sanaa). Over the past decade, the mean annual aerosol optical thickness (AOT) values were in the range of 0.3–0.5, which is attributed to both mineral dust (60–70%) and anthropogenic activities (20–30%). An increase in AOT values between 2005 and 2009 is attributed to increased dust generation from the Sahel region in Northern Africa, and the Fertile Crescent (Syria, Iraq, Jordan) due to an extended dry period. Reductions in local urban emissions are still considered to be efficient measures to improve air quality in these population centers despite the significant contribution of desert dust in the total particulate matter levels in the region. Full article

In this paper, the feasibility of retrieving the aerosol fine-mode fraction (FMF) from ground-based sky light measurements is investigated. An inversion algorithm, based on the optimal estimation (OE) theory, is presented to retrieve FMF from single-viewing multi-spectral radiance measurements and to evaluate the impact of utilization of near-infrared (NIR) measurements at a wavelength of 1610 nm in aerosol remote sensing. Self-consistency tests based on synthetic data produced a mean relative retrieval error of 4.5%, which represented the good performance of the OE inversion algorithm. The proposed algorithm was also performed on real data taken from field experiments in Beijing during a haze pollution event. The correlation coefficients (R) for the retrieved aerosol volume fine-mode fraction (FMF_v) and optical fine-mode fraction (FMF_o) against AErosol RObotic NETwork (AERONET) products were 0.94 and 0.95 respectively, and the mean residual error was 4.95%. Consequently, the inversion of FMF_v and FMF_o could be well constrained by single-viewing multi-spectral radiance measurement. In addition, by introducing measurements of 1610 nm wavelength into the retrieval, the validation results showed a significant improvement in the R value for FMF_o (from 0.89–0.94). These results confirm the high value of NIR measurements for the retrieval of coarse mode aerosols. Full article

We herein present the spectral linear particle depolarization ratios (δ_p) from an Aerosol Robotics NETwork (AERONET) sun/sky radiometer with respect to the aerosol type. AERONET observation sites, which are representative of each aerosol type, were selected for our study. The observation data were filtered using the Ångström exponent (Å), fine-mode fraction (FMF) and single scattering albedo (ω) to ensure that the obtained values of δ_p were representative of each aerosol condition. We report the spectral δ_p values provided in the recently released AERONET version 3 inversion product for observation of the following aerosol types: dust, polluted dust, smoke, non-absorbing, moderately-absorbing and high-absorbing pollution. The AERONET-derived δ_p values were generally within the range of the δ_p values measured from lidar observations for each aerosol type. In addition, it was found that the spectral variation of δ_p differed according to the aerosol type. From the obtained results, we concluded that our findings provide potential insight into the identification and classification of aerosol types using remote sensing techniques. Full article

Vipava valley in Slovenia is a representative hot-spot for complex mixtures of different aerosol types of both anthropogenic and natural origin. Aerosol loading distributions and optical properties were investigated using a two-wavelength polarization Raman LiDAR, which provided extinction coefficient, backscatter coefficient, depolarization ratio, backscatter Ångström exponent and LiDAR ratio profiles. Two different representative meteorological situations were investigated to explore the possibility of identifying aerosol types present in the valley. In the first case, we investigated the effect of strong downslope (Bora) wind on aerosol structures and characteristics. In addition to observing Kelvin–Helmholtz instability above the valley, at the height of the adjacent mountain ridge, we found new evidence for Bora-induced processes which inject soil dust aerosols into the free troposphere up to twice the height of the planetary boundary layer (PBL). In the second case, we investigated aerosol properties and distributions in stable weather conditions. From the observed stratified vertical aerosol structure and specific optical properties of different layers we identified predominant aerosol types in these layers. Full article

The article is aimed at presenting a semi-empirical model coded and computed in the programming language Python, which utilizes data gathered with a standard biaxial elastic lidar platform in order to calculate the altitude profiles of the structure coefficients of the atmospheric refraction index $C_N^2\left(z\right)$ and other associated turbulence parameters. Additionally, the model can be used to calculate the PBL (Planetary Boundary Layer) height, and other parameters typically employed in the field of astronomy. Solving the Fernard–Klett inversion by correlating sun-photometer data obtained through our AERONET site with lidar data, it can yield the atmospheric extinction and backscatter profiles $\alpha \left(z\right)$ and $\beta \left(z\right)$ , and thus obtain the atmospheric optical depth. Finally, several theoretical notions of interest that utilize the solved parameters are presented, such as approximated relations between $C_N^2\left(z\right)$ and the atmospheric temperature profile $T\left(z\right)$ , and between the scintillation of backscattered lidar signal and the average wind speed profile $U\left(z\right)$ . These obtained profiles and parameters also have several environmental applications that are connected directly and indirectly to human health and well-being, ranging from understanding the transport of aerosols in the atmosphere and minimizing the errors in measuring it, to predicting extreme, and potentially-damaging, meteorological events. Full article