*2.1. Materials*

The chemicals used in the present study were all of analytical grade and supplied by Aldrich, Gillingham, UK. They included cobalt acetate Co(ac)2·4H2O, nickel acetate Ni(ac)2·4H2O and zirconium(IV)-butoxide Zr(BuO)<sup>4</sup> (80 wt % solution in 1-butanol). Aluminum tri-sec.-butylate Al(sec.-BuO)<sup>3</sup> was supplied by Merck, Southampton, UK.
