*Review* **Past, Present and Near Future: An Overview of Closed, Running and Planned Biomethanation Facilities in Europe**

**Máté Zavarkó 1,2, Attila R. Imre 3,4,\*, Gábor Pörzse <sup>5</sup> and Zoltán Csed ˝o 1,2**


**Abstract:** The power-to-methane technology is promising for long-term, high-capacity energy storage. Currently, there are two different industrial-scale methanation methods: the chemical one (based on the Sabatier reaction) and the biological one (using microorganisms for the conversion). The second method can be used not only to methanize the mixture of pure hydrogen and carbon dioxide but also to methanize the hydrogen and carbon dioxide content of low-quality gases, such as biogas or deponia gas, enriching them to natural gas quality; therefore, the applicability of biomethanation is very wide. In this paper, we present an overview of the existing and planned industrial-scale biomethanation facilities in Europe, as well as review the facilities closed in recent years after successful operation in the light of the scientific and socioeconomic context. To outline key directions for further developments, this paper interconnects biomethanation projects with the competitiveness of the energy sector in Europe for the first time in the literature. The results show that future projects should have an integrative view of electrolysis and biomethanation, as well as hydrogen storage and utilization with carbon capture and utilization (HSU&CCU) to increase sectoral competitiveness by enhanced decarbonization.

**Keywords:** biomethanation; power-to-methane; competitiveness; hydrogen utilization; decarbonization; Hungary

#### **1. Introduction**

In line with the long-term strategy of the European Union to become climate-neutral, the energy storage challenge [1] that is induced by volatile renewable electricity production (e.g., with rapidly growing photovoltaic capacities) must be handled [2–4]. Power-to-gas (P2G), and especially power-to-methane (P2M), technologies, however, are capable of providing flexibility [5] and efficient seasonal energy storage [6] with the reuse of CO2 and the utilization of the existing capacities of the natural gas grid [7]. Moreover, these technologies are not only present on a lab-scale or prototype level, but there are examples for commercial-scale implementation, with chemical [8] and biological methanation [9] as well. Widespread utilization of this technology, however, has not happened yet, despite the potential of P2G technologies [10,11]. To accelerate the implementation of the P2M technology on a commercial scale, further R&D&I activities and policy regulations are also needed [7]. Regarding the prior literature in the P2G field, the "research" and the "development" part of the R&D&I are often supported by new technoeconomic research results [12–14]. Moreover, the "innovation" part is already discussed from in-depth management aspects [7,15],

**Citation:** Zavarkó, M.; Imre, A.R.; Pörzse, G.; Csed˝o, Z. Past, Present and Near Future: An Overview of Closed, Running and Planned Biomethanation Facilities in Europe. *Energies* **2021**, *14*, 5591. https:// doi.org/10.3390/en14185591

Academic Editor: Idiano D'Adamo

Received: 29 July 2021 Accepted: 1 September 2021 Published: 7 September 2021

**Publisher's Note:** MDPI stays neutral with regard to jurisdictional claims in published maps and institutional affiliations.

**Copyright:** © 2021 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https:// creativecommons.org/licenses/by/ 4.0/).

and there are also analyses from policy perspectives [6,16]. Nevertheless, there is a lack of a high-level approach which can integrate these aspects for socioeconomic progress. Consequently, this study focuses on P2M facilities with novel biological methanation technology [17] and their potential connection to sectoral competitiveness in Europe.

Compared to previous project reviews [17–20], which have already collected P2M projects including chemical and biological methanation (and other P2X projects, as well), this study has a different approach with the following adjustments:


This competitiveness-oriented approach is unique in the P2G literature. Even though Brunner et al. [21] analyzed the relationships of competitiveness and P2G, it had a different scope: they aimed to compare the competitiveness of different P2G operational concepts. Moreover, research usually focuses on the competitiveness of P2G technologies (e.g., compared to other energy storage technologies) [22,23] but rarely on the competitivenessincreasing opportunities by P2G (or P2M in this study). The importance of this topic, however, derives from the practical need and the context as well—similar to the competitiveness studies in general. For example, Fagerberg [24] argues that the "competitiveness" term also does not originate from theoretical researchers but professionals working around decision makers. The relevance of this topic has similar roots: the European Green Deal mentions several times the importance of supporting the economic competitiveness of the EU [25]. The document also declares that "new technologies, sustainable solutions and disruptive innovation are critical to achieve the objectives of the European Green Deal" (p. 18, [25]). As recent research focusing on biomethanation technology concluded that P2M can be disruptive in the future [15], the research question of this study is the following:

How can future P2M, and especially biomethanation facility development projects, increase sectoral competitiveness in Europe?

Figure 1 summarizes (1) why the research is relevant, (2) what is in the focus of the research, and (3) how the research was conducted.

**Figure 1.** Relevance and scope of the research.

In sum, the study has a more future-oriented approach rather than a retrospective one, and this future orientation requires specificity regarding:


Based on the abductive approach of this research with qualitative elements, hypotheses cannot be made, but underlying presumptions as propositional knowledge emerging from prior research [26] can be explicated that will be extended, modified, or developed further by empirical data gathering, analysis, and theory generation. Regarding the fundamental characteristics of the focal technology listed in the first paragraph, the underlying presumption for the research question is that future biomethanation facility development projects would increase sectoral competitiveness in Europe by providing flexibility, seasonal energy storage, and reuse CO2 for synthetic natural gas production, thus integrating renewable energy sources and contributing to decarbonization efforts.

The study is structured as follows. First, the technical background of biological methanation, the research framework, and the applied data gathering and analysis methods are presented. In the Results section, biomethanation facilities are presented and key topics for future projects are revealed. After that, these topics are discussed in-depth according to former literature and research results. Finally, conclusions, limitations, and further research directions are outlined.

#### **2. Materials and Methods**

#### *2.1. Technical Background*

The study focuses on the methanation segment of P2G. In this case, the mixture of H2 (from water electrolysis by renewable electricity) and CO2 (e.g., from biogas, landfill gas or flue gas) can be converted to methane [27]: CO2 + 4H2→CH4 + 2H2O.

There are four different solutions for methanation, two of them are already in use at the commercial scale: chemical and biological methanation. These solutions have different operational characteristics that are thoroughly analyzed in the literature (see, e.g., [19] or [28]). One of the main differences is that while chemical (catalytic) methanation needs high pressure and temperature to reach high CO2 conversion, which can be 50–60% and 80–90% or higher in proper conditions, biological methanation needs lower pressure and temperature (ca. 60–70 ◦C) than catalytic methanation; moreover, the CO2 conversion is often higher than 95% [17,29–32]. Furthermore, in the case of biological methanation, microorganisms catalyze the reaction in a multiphase system because the gaseous H2 and CO2 are dissolved in the liquid phase, in which the Archaea absorb them and produce CH4 [33]. In contrast, chemical methanation needs other types of catalysts, e.g., ruthenium [34] or nickel-based catalysts, that are characterized by high performance and low cost [35]. The catalysts determine different opportunities and limitations as well. For example, fluctuations and impurities are less harmful in case of the biological process with the robust methanogens, thus it can provide simpler applicability in contexts where contaminants (e.g., hydrogen sulfide) must be considered; nevertheless, its main limitation is the gas-to-liquid mass transfer at a relatively low temperature [19].

The "biomethanation" and "biological methanation" terms are often used in case of biogas upgrading, as well, when additional hydrogen injection happens. In this case, hydrogenotrophic methanogens function as a catalyst in a mixed culture, and there is no need for a separate bioreactor and clear culture [36,37]. A novel method for the P2M process is the bioelectrochemical system for electromethanogenesis (EMG-BES). It uses electro-active microorganisms, and the reaction happens only at 25 to 35 ◦C [38].

In the case of the focal biomethanation technology, microorganisms can convert ca. 97–98% of the CO2 into methane during the methanation phase in a separate culture, which is promising regarding the decarbonization efforts. The total efficiency of such

a biomethanation plant (together with the electrolysis step) can be in the range of 55 to 60% [6].

#### *2.2. Research Framework*

While competitiveness is defined from several aspects in the literature [39], an innovation approach must be considered in this study. In this sense, sectoral competitiveness can mean such capabilities which are (partly) created by innovation and which are required for sustained economic growth in an (international) competitive environment [40]. As innovation can be interpreted as a process during which an opportunity becomes a useful solution in practice [41] and can be a positive-sum game because of the complementarities among contributors [42], a network approach can be also important to increase sectoral competitiveness.

Accordingly, as the literature highlights the importance of the know-how transfer among companies, universities, and state administration [40,43], this research not only focuses on biomethanation projects but the main areas on which future work is necessary to contribute to sectoral competitiveness. For this purpose, the projects are interpreted from the aspect of recent scientific research results and EU strategies and policies. Figure 2 illustrates the research framework.

**Figure 2.** Research framework (Orange: Focus of the research; Green: Context of the research).

#### *2.3. Research Methodology, Data Collection, and Analysis*

An abductive approach was followed to answer the research question, which involved iteration between empirical data and theory. It means that empirical data can be analyzed to reveal regularities or phenomena, and then they can be compared to previous research results and theories to explain the revealed phenomena and develop new theories. This abductive approach and the iteration is emphatic in several research methods, such as grounded theory [44], extended case study [45], or more broadly, the abductive theory of method (ATOM) [46]. This research integrates elements from all of these methodological roots. As "ATOM itself as a grounded theory method that explicitly accommodates both quantitative and qualitative outlooks on research" (p. 106, [46]), this research involves both quantitative text analysis and their qualitative interpretation from the aspect of a disruptive technology developer company (an empirical case as a starting point).

The research is partly built on the digital R&D and open innovation platform of Powerto-Gas Hungary Kft., a Hungarian startup that developed an innovative biomethanation P2G prototype in cooperation with Electrochaea GmbH. The startup company consciously manages digital know-how flows within the organization and the inter-organizational network and continuously monitors the international P2G market and research results. On this platform, the company develops different kinds of knowledge elements with the involvement of employees, external professionals, stakeholders, and academic researchers. These knowledge elements include project descriptions, innovational and technological know-hows and analyses, e-learning materials, innovation problems, and ideas to solve them (idea generation). This platform, however, only represents the industrial "lens" for the study because research papers (indicating the scientific context) and EU policies

and strategies (indicating the socioeconomic context) were also collected by the authors, while also considering the suggestions of the stakeholders of the company (interviewees, see below).

Table 1 presents the structure of data collection.

	- a. Scientific research can also affect the planning and implementation of future P2M projects with biological methanation [7]. The authors collected recent research papers and created a long list of potentially relevant publications from the aspect of the company and future biomethanation facility development (*n* > 250). The goal was to provide a broad horizon of opportunities (including power-to-methane (P2M), power-to-hydrogen (P2H), power-to-liquid (P2L), power-to-X (P2X), and carbon capture (CC)) and to avoid unintentionally narrowing the relevant themes, which could have limited the reliability of the research in an abductive sense. After that, the P2H-, P2L-, P2X, and CC-oriented contents were filtered out collaboratively with the interviewees. Facing the limited number of literature analyses focusing only on biological methanation, and as the term "biological methanation" is often used for novel biogas upgrading processes with H2 injection and mixed culture, the potential contribution of biological P2M could be identified more reliably if less restrictions were applied and the whole P2M literature is considered (*n* = 63; see Appendix A).
	- b. In line with the competitiveness approach of the study, the analysis of the project descriptions was compared to EU strategies for carbon-neutrality and their relations to competitiveness.


**Table 1.** Data collection for text analysis.

The research involved quantitative text analysis with the JMP software, which is useful for text mining purposes [51]. After cleaning the data, recoding words and phrases (e.g., plurals, or "ptg" and "p2g" to "power to gas"), word clouds and trend analyses were generated, i.e., exploring the change of the most common terms according to different variables (time horizons, data sources (project descriptions scientific research or

policies), and electrolyzer capacity in case of project descriptions). Moreover, trend analyses were combined with hierarchical clustering to reveal possible important underlying structures [52]. These quantitative analyses, additional qualitative interviews with company employees and stakeholders for interpreting raw data, and iterations with former literature indicated "key topics" for further elaboration. These key topics were iterated by more research results to generate an in-depth understanding and R&D&I directions for future biomethanation projects.

The relevance of these methodological choices is to look at the biomethanation projects not only through the lens of academia, but as a technology developer company as well. Power-to-Gas Hungary Kft. is known for its long-term mission to implement a 10 MWel P2M plant. It would be the largest P2M plant with biological methanation, and the second largest regarding chemical methanation as well [18]; consequently, the potential contribution to sectoral competitiveness is high in its case.

To improve the validity, reliability, and generalizability of the research, the following steps were undertaken:


#### **3. Results**

#### *3.1. Biomethanation Projects and Industrial-Scale Facilities in Europe*

Regarding list of the European P2M projects with biological methanation, while most of the projects were listed in recent reviews of Thema et al. [19] and Bargiacchi [18], there are three projects that were not listed previously.


Table 2 shows these projects with the other projects which are monitored by the company based on accessible information about their capacity or status. Besides these 21 projects, Thema et al. [19] listed other biomethanation (mainly research) projects without sufficient (accessible) information:


Regarding future industrial-scale developments, it can be argued that the capacity of larger biomethanation facilities must reach at least 1 MWel to satisfy the demand for electrolysis and also for methanation, which can exceed even 1000 GWel globally [59], and even over 500 GWel for P2M in very positive scenarios [60]. Based on publicly accessible data, six projects reached or are planned to reach the 1 MWel capacity: Energiepark Pirmasens-Winzeln, BioCat Project, Dietikon Microbenergy, INFINITY 1, Power-to-Gas Hungary plant, and HYCAUNAIS. The first five received a detailed description recently by Bargiacchi [18], while the HYCAUNAIS project was introduced above.

**Table 2.** European biomethanation projects with sufficient accessible information about capacity or status, based on [18,19] and own research.


#### *3.2. Key Topics of Future Implementation*

In the following section, key topics are identified based on the quantitative text analysis, interviews, and the literature, for which overarching R&D&I directions will be suggested in the Discussion section.

3.2.1. Key Topic 1: The Role of Biomethanation in the Hydrogen Economy

Based on the short summaries of the listed projects (ca. 1–3 pages, 2501 total terms, 14,573 total tokens), the most common word is "hydrogen". Similar influential words are "carbon dioxide" and "methane" (see Figure 3). This result refers to the importance of input factors in the biomethanation sector, and even though it is not particularly surprising, the relative dominance of hydrogen against the other key terms (e.g., methane, storage, biogas, natural gas) is conspicuous. Regarding the trend and advancements towards the

hydrogen economy [85], the hydrogen orientation can be justified, but it can also be asked, for example, what could the role of biomethanation (biomethane or SNG production) be in the hydrogen economy? This might require further analysis later, based on other research results and EU policies.

**Figure 3.** Word cloud from biomethanation project descriptions.

In addition to taking a static "snapshot" of the content of the biomethanation project descriptions (Key topic 1), quantitative characteristics of the projects provide opportunities for deeper insights. The next section (Key topic 2) considers the size of the facility (indicated by the capacity of the electrolyzer), while after that, Key topic 3 analyzes trends according to the start of the project (year).

3.2.2. Key Topic 2: Opening New Ways besides Biogas Plants to Store More Renewable Electricity/Hydrogen

The terms that appeared at least 15 times in the project descriptions were analyzed according to the size of the biomethanation facility. It can show how the focus of the R&D&I activities changes (or does not change) with the deployment of larger facilities. Considering the lessons of the interpreting interviews as well, Figure 4 suggests the following:


The importance of the results shown by Figure 4 is that they interconnect the past and the future of biomethanation technology development from a purely technical aspect (without considering the time horizon, which is presented in the next section). Less abstractly, different issues are important at the small and large scales, and the gaps between these issues might generate new areas for research. Regarding the listed (a) and (b) points above, a step is missing between the efficient process in kW-scale with CO2 from biogas and the purpose of storing high volumes of renewable electricity in the form of SNG in MW-scale. This missing step seems to be the sourcing of CO2 in large volumes to develop multi-MW biomethanation plants. Accordingly, it is worth analyzing that if biogas plants cannot provide enough carbon dioxide for large-scale P2M plants [15], which could convert the vast volume of renewable electricity produced by wind or solar parks, what solutions can help to increase the capacity of biomethanation facilities to multi-MWel level, which are needed in the future [59].

**Figure 4.** Appearance of the most common terms according to the size of the planned/implemented biomethanation facility. For example, the term "storage" appeared in project descriptions of biomethanation plants, which were 1.3 MWel on average.

3.2.3. Key Topic 3: From Technology Development towards Achieving "Future" Benefits

The most common terms of the project descriptions may change according to the start year of the projects, not only their capacity. Accordingly, Figure 5 shows constellation plots of a hierarchical cluster analysis which might reveal some underlying structures (e.g., main terms of past and present; based on the 75 most common terms). Based on the collaborative interpretation with the interviewees, Figure 5 shows the following:


"electricity", and producing "green methane", "biomethane", or other "fuels" that fit the "infrastructure" to fight "climate" change.

**Figure 5.** Constellation plots showing clusters of terms according to the project starts.

3.2.4. Key Topic 4: Future Project Planning in Line with Scientific Advancements and Policy Objectives

Based on the abstracts of the selected publications, a slightly different scheme can be seen on the word cloud than in the case of the biomethanation project descriptions. For example, while hydrogen and carbon dioxide are apparently important, carbon dioxide appears more often in case research papers, while hydrogen utilization appears more often in case of the project descriptions. Scientific research, however, deals more with the operative questions of the "system", the "process", or the "reactor", while biomethanation project descriptions write about "using" the "technology" for "energy storage" and the "production" of methane.

Figure 6 shows the comparison of the most common terms of research papers, project descriptions, and EU policies. In line with the mentioned trends, carbon dioxide (N = 116), hydrogen (101), methane (92), system (79), and power-to-gas (77) were the most dominant in a quantitative sense, in case of the abstracts of research papers. Project descriptions were also focused on these three terms, but with others: hydrogen (104), methane (90), carbon dioxide (80), use (80), energy (77), and gas (77).

**Figure 6.** Comparing the word clouds of biomethanation project descriptions, P2M publications, and relevant EU policies.

In contrast to that, regarding the EU policies and strategies, the most common terms are energy (157), greenhouse gas emissions (88), economy (87), reduce (69), sectors (68), and sustainable (68). Accordingly, the main objective is to "reduce" the "greenhouse gas emissions" (GHG) through a "sustainable" "transition" with more "renewable energies". The "economy" and increasing "competitiveness" in a "global" "environment", however, is also important while fighting "climate change". For example, the document called "A Clean Planet for All" by the European Commission refers to competitiveness already in its subtitle: "A European strategic long-term vision for a prosperous, modern, competitive and climate neutral economy" [47]. The European Green Deal "aims to transform the EU into a fair and prosperous society, with a modern, resource-efficient and competitive economy" (p. 2, [48]).

These results suggest that scientific research, industrial project development, and policies have common points, e.g., the GHG-reduction induces the scientific research on carbon capture and utilization (CCU) solutions and their industrial application at biomethanation facilities. These high-level interconnections, however, should be analyzed in-depth to identify how sectoral competitiveness can be supported in practice by new biomethanation facility development projects.

#### **4. Discussion**

In the following, possible R&D&I directions will be presented for the identified key topics. These directions are based on the European context on the one hand, and the mentioned EU documents and the extensive studies of the European STORE&GO project [86] were analyzed. This project included three P2G demonstration plants, and its studies are heavily based on empirical data, as well.

On the other hand, the Hungarian context was also considered. It was important because the whole research followed an abductive approach in which the aspect of the Hungarian technology developer company is central. In addition, the capacity of the gas-grid of Hungary—compared to most other European countries—is quite high, which is an important factor to choose P2M-based long-term energy storage. Consequently, its national environment must be taken into account to contextualize findings. Since the National Energy Strategy 2030 of Hungary states that the implementation of the strategy contributes to the improvement of Hungary's competitiveness (p. 13, [87]) and identifies the direct value-creating potential of power-to-gas in energy storage (p. 39), the contribution for competitiveness by P2M seems clear by deductive reasoning. Based on the abductive methodology, however, it must be supported by more empirical evidence and prior research results.

In the following, overarching directions are presented along with the key topics for future biomethanation facilities, which can directly or indirectly increase sectoral competitiveness.

#### *4.1. Key Topic 1: The Role of Biomethanation in the Hydrogen Economy—An Integrative View of Electrolysis and Biomethanation for Carbon-Neutral Energy Production, Flexibility Services, and Hydrogen Storage and Utilization*

Hydrogen is explicitly considered as a "priority area" (p. 8, [48]) in the EU. The more hydrogen is produced in the hydrogen economy, the higher the need will be to store or utilize it efficiently, especially because there are safety limits to the injection hydrogen into the natural gas grid [88,89]. Biomethanation can function as a chemical method for hydrogen storing and/or utilization "tool" in the form of methane (SNG) in high amounts and for a long term, or it can be a middle step towards utilization in other forms (e.g., LNG). This is also in line with EU strategies, for example: "Sustainable renewable heating will continue to play a major role and gas, including liquefied natural gas, mixed with hydrogen, or e-methane produced from renewable electricity and biogas mixtures could all play a key role in existing buildings as well as in many industrial applications" (p. 8, [47]). Biomethanation can be also dynamically coupled with electrolyzers because microorganisms are capable to produce methane in seconds [6] (unlike chemical methanation)—this means additional flexibility beyond the electrolysis for the coupled electricity and gas sector.

In the European context, flexibility by electrolysis and biomethanation can have a beneficial effect on the operation of the network. The presence of 7.2 GWel P2M could significantly reduce the peak (~45%) and duration (>95%) of the imbalance. Due to P2M installation, reverse energy flow could be reduced by 67% or even 100% [90]. Furthermore, the prevalence of green methane is also expected. By 2030, according to scenarios that can be considered optimistic in this regard, the 4% share could increase to 12% [91]. With P2M technology, the ratio of imported gas and total gas consumption could be reduced by up to 30–40% by 2050 [92]

In the Hungarian context, carbon-neutral methane production can also reduce natural gas imports, which is relevant because ca. 80% of the natural gas demand is covered by imports (p. 14). Encouraging the use of biogas, biomethane and non-natural-gas-based hydrogen (p. 12) also include the production of these energy sources. Hydrogen and methane can be used to produce biofuels or "green" fuels, which can be the part of the green transportation program (p. 13, [87]).

#### *4.2. Key Topic 2: Opening New Ways besides Biogas Plants to Store More Renewable Electricity/Hydrogen—Enhanced Decarbonization by the Co-Specialization with Carbon Capture Technologies*

Decarbonization is one of the main objectives in the EU, as "further decarbonising the energy system is critical to reach climate objectives in 2030 and 2050" (p. 6, [48]). In this area, an important challenge emerges in case of biomethanation because methanation requires efficiently useable CO2 sources, which are reachable at biogas or bioethanol plants, but these plants sometimes do not have a close connection to the natural gas grid for energy storage, nor enough CO2 for multi-MWel P2M plants [6]. Moreover, carbon capture solutions for flue gas are considered expensive and immature in commercial-scale yet [15], despite the numerous research on different CC solutions (e.g., post-combustion [93] or oxyfuelcombustion [94]). A promising direction can be, however, the joint R&D on carbon capture technologies and biomethanation, similar to the research of Bailera et al. [95,96]. In addition to the co-specialization of resources, technologies can lead to competitive advantages in general in a competitive environment [97], and the context is also supporting this purpose. For example, by implementing P2M systems, pollutant emissions can be reduced, thus their environmental impact is positive and most of the positives can be detected in the field of climate change [98]. Synthetic methane offers outstanding greenhouse gas savings when biogenic carbon dioxide sources have been used in the methanation process or when hydrogen is generated by electrolysis by renewable energy [99], but it can be further be enhanced with efficient carbon capture solutions for flue gas.

Strictly speaking, P2M is not carbon-neutral because, during the use of biomethane, the previously "captured" CO2 will be emitted again. However, one should realize, for example, that by using the flue gas of an energy-producing gas turbine for methanization and by reusing the new biomethane again in the same gas turbine, one carbon atom will be used twice (or thrice or even more) before emitting it as CO2.

In the Hungarian context, by 2030, 90% of domestic electricity production is planned to be CO2 emission-free (p. 42). Installation alongside GHG-intensive industrial activities and the use of industrial carbon dioxide are also promising in the methanation step, to increase the competitiveness of GHG-intensive industrial activities (p. 50). The production and purification of biogas can also contribute to the achievement of decarbonization goals (p. 20, [87]), and it is particularly true if carbon dioxide can be converted into methane.

#### *4.3. Key Topic 3: From Technology Development towards Achieving "Future" Benefits—Finding Ways for Realizing and Communicating Business, Societal and Residential Value Creation*

Research results suggest that even though there is still a need for research on biological methanation to increase its TRL [100], it is already worthwhile to analyze how future biomethanation can achieve future socioeconomic benefits. Realizing benefits is possible by scaling up the technology, but it requires capital investments, the returns of which might not meet the expectations of market players in the present [6,7]. Consequently, supporting regulations and profitable business models must be developed to "attract support from "patient" capital (i.e., long-term venture capital)" (p. 24, [47]), but significant public funding could be also necessary to scale up the technology. Public funding, however, can be justified if broad social and residential benefits are also explicit. Research results of the STORE&GO project show, for example, that a potential supply shock in the energy market will have less of an impact on social welfare if P2M technology is used [98]. Moreover, solar parks and P2M infrastructure increase the acceptance of the energy system by local energy communities [101].

In Hungary, rapidly growing photovoltaic capacities to 6000 MW by 2030 is a priority (p. 14), which can be technically supported by the integration function of P2M technology. Converting surplus electricity to methane and its storage, however, can be important from broader socioeconomic aspects as well, because it can contribute to the affordable and steady energy supply (p. 10, [87]).

#### *4.4. Key Topic 4: Future Project Planning in Line with Scientific Advancements and Policy Objectives—Building and Supporting Innovation Ecosystems for Efficient Know-How Transfer*

Most of the biomethanation projects are realized in consortia of heterogeneous stakeholders, such as universities, startups, and large energy companies, while funding is often provided by the state administration [17,18]. As such, an inter-organizational network can have heterogeneous stakeholders, and an R&D&I ecosystem might be needed to bring and hold them together. An innovation ecosystem is a dynamic and adaptive system, the participants of which have different roles, motivations, and capabilities, but they all contribute to the success of an innovation process [102]. It means that an innovation ecosystem can involve not only companies from a certain sector but also from supporting sectors and regulators, since government policies also affect competitiveness [103]. Accordingly, the literature deals with the state support of R&D&I ecosystems as well. For example, government interventions that focus resources for grand challenges such as climate change facilitate the formation of networks beyond sectors and encourage scientific and technological improvements and the introduction of new or existing technologies [104]. These ecosystems can be the key for the economic growth after the COVID-19 pandemic according to the World Economic Forum, who also stated that supporting ecosystems can contain incentives for venture capital investments, R&D process and spreading new technologies [105]. Even though "green" R&D and creating balance among economic, ecological, and societal aspects must be supported by public financial sources, recent empirical studies showed that advancement in one dimension (e.g., ecological) does not necessarily happen at the cost of another dimension (e.g., economic) [106]. Biomethanation-focused innovation ecosystems may obtain support from the Horizon Europe programme, in which "partnerships with industry and Member States will support research and innovation on transport, including batteries, clean hydrogen, low-carbon steel making, circular bio-based sectors and the built environment" (p. 18, [49]).

Consequently, know-how transfer in biomethanation-focused innovation ecosystems with startups, universities, and state administrations can facilitate the previous three R&D&I directions. Figure 7 summarizes the findings and shows them according to the research framework.

**Figure 7.** Findings aligned by the research framework (Orange: Focus of the research; Green: Context of the research; Red: Key topics; Blue: Suggested R&D&I directions).

#### *4.5. Comparing the Results to Other Relevant Topics*

As stated before, the list of the analyzed project descriptions and research papers was formulated from the viewpoint of a startup company (which might contribute to sectoral competitiveness with the deployment of large biomethanation plants). In addition, raw text data and interview data were iterated with former theories and research results. This approach, on the one hand, can be considered as a pragmatist one, which is in line with the roots of competitiveness studies [24], and one aimed to generate conclusions representing "cognitive usefulness in the world" (p. 18, [46]) and actionable knowledge [107]. This actionable knowledge is represented by the suggested R&D&I directions. Moreover, the conclusions would be supported by the coherence theories of truth, as well, according to which the propositions must be coherent with other scientific propositions [46]. This is because the empirical data was processed with comparisons with previous research results.

On the other hand, findings generated by this approach cannot cover every aspect and do not mean a positivist, general, theory [44]. It means that because of this abductive methodological approach, there can be areas that did not emerge during the research, i.e., the empirical data did not orient the parts of the ATOM, such as phenomena detection, analyses, and theory development [46]. Consequently, even though the synthesis of new empirical data and former research results into a coherent (but not full) set of theoretical propositions, it is worth comparing the results to some other topics which might be considered "key topics" in different contexts.

For example, (1) circular economy models can be relevant. Based on the analysis of Kircherrr et al. [108] on circular economy definitions, the main elements are central in circular economy models: the combination of reduction, reuse and recycling, and systemic shifts. These elements can be supported by biomethane production with P2M technology, as follows:


Taking a closer look at biomethanation, research on the relationship with circular economy outlined some opportunities and challenges already. Baena-Moreno et al. [109] discussed that the combination of biological processes and renewable energy production can be the main pillar of the paradigm shift towards the circular economy, but incentives and/or cost-reduction-oriented technology developments are still needed. In a similar area, Eggemann et al. [110] argued that power-to-fuel processes producing methanol can contribute to the circular economy, but technology adoption might be influenced by the economic performance of these systems compared to other technological options. D'Adamo et al. [111] showed how biomethane can integrate effective management of renewable energies and municipal waste, thus contributing to the circular economy development. Their research leads to another important area of potential competitiveness developments, as well. The authors pointed out that biomethane can be used as fuel for vehicles, so (2) the green revolution in the transportation sector might be also supported by converting biowaste into clean fuels [111]. For example, biomethane can be compressed (CNG) or liquefied (LNG) for these purposes. Finally, competitiveness can be researched from (3) policy perspectives. Wall et al. [112] pointed out that recent EU legislation incites third-generation biofuels, and it creates a foundation for the integration of different solutions, e.g., anaerobic digestion, gasification, P2G, or algae as feedstock. Nevertheless, there is still further need for policy interventions to support green transitions with biomethane, for example, fueling stations in the case of the transportation sector [111], feed-in tariffs supporting seasonal energy storage [6], or carbon taxes [7] or certifications for green premiums [113] influencing the diffusion of the biomethanation technology and the production of biomethane.

These areas (circular economy, green transportation, impact of policies) did not emerge empirically during this research, but their related research results are mostly in line with the key topics and/or suggested R&D&I directions. For example, circular economy development is often focused on decarbonization which can be supported by the co-specialization of biomethanation and carbon capture technologies. Regarding green transportation, finding the role of biomethane in an area dominated by electric and hydrogen vehicles is also an important task, while incitive policies are important in the case of the formation of efficient national or international innovation ecosystems as well. The main novelty of the findings compared to previous literature, however, is related to the urged adaptation to the hydrogen economy and carbon capture of the future biomethanation project planning, as discussed below.

#### **5. Conclusions**

This research aimed to answer how could future biomethanation facility development projects increase the sectoral competitiveness in Europe. The propositional knowledge of the research based on prior literature was that future biomethanation facility development projects would increase sectoral competitiveness in Europe by providing flexibility, seasonal energy storage, and the reuse of CO2 for synthetic natural gas production, thus integrating renewable energy sources and contributing to decarbonization efforts. Based on the empirical data collection, analysis, and iterative theory generation, however, this proposition must be modified. It viewed the relationship of biomethanation projects and sectoral competitiveness too narrowly, and ignored their contribution to the hydrogen economy and the synergies with another technology development area: carbon capture. The specific conclusion for this proposition is that in addition to the important energy storage potential, biomethanation facilities would increase sectoral competitiveness mainly due to their connective role between the two most important terms (or areas) of European strategies about economic and environmental progress: hydrogen economy and decarbonization.

Findings suggest that by building on the know-how of past and present projects, future biomethanation projects could take significant steps towards multi-MWel capacities. Moreover, they should take these steps to satisfy the growing demand for their outputs and positive externalities. These improvements could support sectoral competitiveness in Europe if these projects have an integrative view of electrolysis and biomethanation for carbon-neutral energy production, flexibility of services, and hydrogen storage and utilization. In other words, biomethanation should be interpreted in the future as a hydrogen storage and utilization (HSU) solution, on the one hand. On the other hand, as biogas plants sometimes cannot provide enough CO2 for multi-MWel plants, enhanced decarbonization can be only achieved by co-specialization with carbon capture technologies. Consequently, future industry-scale biomethanation facilities should integrate hydrogen storage and utilization and carbon capture and utilization functions (HSU&CCU) to increase sectoral competitiveness in Europe. This direction, however, requires strategic alignment and know-how transfer among universities, startups, large energy companies, and state administration in biomethanation-focused innovation ecosystems.

The main limitation of the research is that it was built on abductive methodology, i.e., conclusions are not confirmed in a positivist sense by testing hypotheses. Because of the specific environment and the integrative, high-level of the analysis, the study might not cover every aspect of biomethanation technology development and competitiveness. For example, future research could identify the competitiveness-increasing potential of biomethanation in future energy systems, or maybe compare it to the potential of chemical methanation. The abductively revealed key topics, however, such as the role of biomethanation in the hydrogen economy or integration with carbon capture technologies, the alignment of technology development, scientific research, and policies might induce other thoughts and future research that facilitates the broad utilization of this innovative technology.

**Author Contributions:** Conceptualization, A.R.I. and Z.C.; methodology, M.Z. and G.P.; validation, A.R.I. and Z.C., formal analysis, G.P. and M.Z.; investigation, A.R.I., G.P., Z.C. and M.Z.; data curation, M.Z.; writing—original draft preparation, G.P. and M.Z.; writing—review and editing, A.R.I. and

Z.C.; visualization, M.Z.; supervision, A.R.I.; project administration, Z.C. All authors have read and agreed to the published version of the manuscript.

**Funding:** This research received no external funding.

**Acknowledgments:** The authors would like to thank Hiventures Zrt./State Fund for Research and Development and Innovation for their investment that enabled this research. This work was prepared with the professional support of the doctoral student scholarship program of the Co-Operative Doctoral Program of the Ministry of Innovation and Technology financed from the National Research, Development and Innovation Fund. Part of this work was performed in the frame of the 2020- 3.1.1-ZFR-KVG-2020-00006 project, implemented with the support provided from the National Research, Development and Innovation Fund of Hungary, financed under the 2020-3.1.2-ZFR-KVG funding scheme.

**Conflicts of Interest:** Two of the authors perform their P2G research at Corvinus University of Budapest, and they have founded the innovative startup company Power-to-Gas Hungary Kft. in order to perform industrial R&D and further develop the technology in pre-commercial and commercial environments.

#### **Abbreviations**


#### **Appendix A**

**Table A1.** Selected publications for quantitative text analysis.



**Table A1.** *Cont.*




#### **Table A1.** *Cont.*

#### **References**

