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Review

Phosphorus-Doped Graphene Electrocatalysts for Oxygen Reduction Reaction

by
Xinxing Zhan
1,
Xin Tong
1,2,*,
Manqi Gu
1,
Juan Tian
1,
Zijian Gao
1,
Liying Ma
1,
Yadian Xie
2,
Zhangsen Chen
3,
Hariprasad Ranganathan
3,
Gaixia Zhang
3 and
Shuhui Sun
3,*
1
School of Chemistry and Material Science, Guizhou Normal University, Guiyang 550001, China
2
Key Laboratory of Low-Dimensional Materials and Big data, Guizhou Minzu University, Guiyang 550025, China
3
Centre Énergie, Matériaux et Télécommunications, Institut National de la Recherche Scientifique (INRS), 1650 Boulevard Lionel-Boulet, Varennes, QC J3X 1P7, Canada
*
Authors to whom correspondence should be addressed.
Nanomaterials 2022, 12(7), 1141; https://doi.org/10.3390/nano12071141
Submission received: 27 February 2022 / Revised: 25 March 2022 / Accepted: 27 March 2022 / Published: 29 March 2022
(This article belongs to the Special Issue Advanced Nanomaterials for Electrochemical Energy Conversion and Storage)
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Abstract

Developing cheap and earth-abundant electrocatalysts with high activity and stability for oxygen reduction reactions (ORRs) is highly desired for the commercial implementation of fuel cells and metal-air batteries. Tremendous efforts have been made on doped-graphene catalysts. However, the progress of phosphorus-doped graphene (P-graphene) for ORRs has rarely been summarized until now. This review focuses on the recent development of P-graphene-based materials, including the various synthesis methods, ORR performance, and ORR mechanism. The applications of single phosphorus atom-doped graphene, phosphorus, nitrogen-codoped graphene (P, N-graphene), as well as phosphorus, multi-atoms codoped graphene (P, X-graphene) as catalysts, supporting materials, and coating materials for ORR are discussed thoroughly. Additionally, the current issues and perspectives for the development of P-graphene materials are proposed.
Keywords: doped graphene; oxygen reduction reaction; phosphorus-doped; codoped doped graphene; oxygen reduction reaction; phosphorus-doped; codoped
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MDPI and ACS Style

Zhan, X.; Tong, X.; Gu, M.; Tian, J.; Gao, Z.; Ma, L.; Xie, Y.; Chen, Z.; Ranganathan, H.; Zhang, G.; et al. Phosphorus-Doped Graphene Electrocatalysts for Oxygen Reduction Reaction. Nanomaterials 2022, 12, 1141. https://doi.org/10.3390/nano12071141

AMA Style

Zhan X, Tong X, Gu M, Tian J, Gao Z, Ma L, Xie Y, Chen Z, Ranganathan H, Zhang G, et al. Phosphorus-Doped Graphene Electrocatalysts for Oxygen Reduction Reaction. Nanomaterials. 2022; 12(7):1141. https://doi.org/10.3390/nano12071141

Chicago/Turabian Style

Zhan, Xinxing, Xin Tong, Manqi Gu, Juan Tian, Zijian Gao, Liying Ma, Yadian Xie, Zhangsen Chen, Hariprasad Ranganathan, Gaixia Zhang, and et al. 2022. "Phosphorus-Doped Graphene Electrocatalysts for Oxygen Reduction Reaction" Nanomaterials 12, no. 7: 1141. https://doi.org/10.3390/nano12071141

APA Style

Zhan, X., Tong, X., Gu, M., Tian, J., Gao, Z., Ma, L., Xie, Y., Chen, Z., Ranganathan, H., Zhang, G., & Sun, S. (2022). Phosphorus-Doped Graphene Electrocatalysts for Oxygen Reduction Reaction. Nanomaterials, 12(7), 1141. https://doi.org/10.3390/nano12071141

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