In this section a few aspects of the role of particles in the thermal interaction between two homothermal regions, advected by a statistically steady homogeneous and isotropic velocity field, will be discussed from the data obtained from a set of direct numerical simulations. Given the large set of parameters, the discussion will focus on the role of particle inertia, and not on the Reynolds and Prandtl numbers or on the volume fraction. Therefore, all simulations have been carried out at the same Taylor microscale Reynolds number
, at a fixed Prandtl number
. Particle volume fraction has been set equal to
in all the simulations. The density ratio is set as
, corresponding to the one of water particles in air, so that particle relaxation times are varied by changing the particle size and the specific heat ratio
between the particles and fluid. Anyway, only the relaxation times of particles matter, and the values of a particle’s parameters have been chosen such that we could explore the behaviour of the system for Stokes numbers up to 6 and thermal Stokes numbers up to 10 in both the one- and two-way coupling regimes. However, differently from previous studies on this problem [
19,
20,
22] which kept the ratio
constant, we consider inertia and thermal inertia as independent parameters, thus St and
are varied independently.
The interface which initially separates the two homothermal regions is spread by the turbulent velocity field and evolves into a thermal mixing layer characterized by a high temperature variance and a strong intermittency at its borders [
32]. As we have shown in [
20], the region where the temperature is not uniform and the two zones interact has a thickness which grows in time and, after a few eddy turnover times
, where
ℓ is the integral scale of the flow and
the root mean square of velocity fluctuations, the mean temperature of the fluid shows, up to the numerical uncertainty, a self-similar profile. This allows us to define a measure of the thickness of the interaction layer from the mean temperature
of the carrier fluid as
to be used as the length scale of the layer [
20]. When the fluid and particle second-order moments are rescaled using the temperature difference
and the thickness
as scales, all profiles tend to collapse into a single curve, i.e., this interaction zone develops in a self-similar way, up to the numerical uncertainty. This lengthscale
shows a
diffusive growth. Particles which move across this non-homothermal layer experience a strong mean temperature gradient, leading to high temperature derivatives, whose distribution is strongly intermittent with large non-Gaussian tails.
Figure 1 shows an example of spatial distribution of the convective heat flux and the particle temperature variance, normalized with the mixing layer thickness
, when
. Both the variance and the temperature–velocity correlation have a maximum for
, where the mean temperature gradient is largest. The temperature gradient across the mixing layer is of order
, so that the large scales of the flow, of the order of the integral scale
ℓ, perceive a temperature difference of order
, which is the expected scale of temperature fluctuations inside the mixing layer. Therefore, if
is the root mean square of the fluid velocity fluctuations, the
correlation can dimensionally scale only as
, while the temperature variance should scale as
. All the curves of both moments are very close for
, almost collapsing within the limits of the noise associated with their computation. This also implies a self-similar or almost self-similar behaviour of particle second-order moments, a feature already observed in [
20]. Therefore, it is possible to average in time all the rescaled moments. In the following, we will discuss the properties of the mixing layer by considering all moments in the centre of the mixing layer. Given the almost self-similar behaviour, this is representative of the entire layer.
This interaction or, broadly speaking, thermal mixing layer (in the sense of [
20,
32,
33]) is characterized also by the onset of a significant velocity–temperature correlation, which is responsible for most of the transfer of enthalpy across the layer, since, by averaging Equation (
3), the mean heat flux in the inhomogeneous direction
is given by
or, in dimensionless form (see
Appendix A for the dimensionless form of the equations according to the adimensionalization (
7)),
where the first term is the mean temperature diffusion, the second the convective heat flux and the third the particle contribution to the mean heat transfer. Since
is the only length-scale of the problem,
is the scale of the heat flux in static conditions. A Nusselt number can be defined as the ratio between this flux, computed in the mixing centre,
and
. By using the definition of
, Equation (
8), this is equal to the diffusive term in (
9) when the flux is computed in the mixing centre, so that the Nusselt number is
Therefore, the re-scaled fluid and particle temperature–velocity correlation, see, e.g.,
Figure 1a, give just the fluid and particle contribution to the Nusselt number of this flow configuration.
Particles have a dual role in the interaction between the two regions, which globally manifests itself with a transfer of heat from one to the other: a direct role, as their motion counteracts the enthalpy transfer, and an indirect role, due to the modulation of temperature and velocity fluctuations of the carrier fluid. Therefore, both one- and two-way thermally coupled regimes are considered, because their differences allow to evidence the role of particle feedback in the flow, i.e., the indirect role of particles. Since the coupling between the convective heat transfer and particles creates a very complex scenario, as stated in
Section 2, we do not consider the particle momentum feedback, which has a minor role [
15,
16,
17] in homogeneous flows, and neither do we consider collisions between particles, whose effect have been documented in [
21,
22].
3.1. Temperature and Velocity Moments in Terms of Particle Time Derivatives
Given the flow inhomogeneity and unsteadiness, in the following we consider conditional averages at a given time and position
along the inhomogeneous direction, i.e., we define, for any function
f of the state of the particle,
where
is the statistical average and we define the fluctuation of
f as
. We will now express the average temperature fluctuations and the heat flux in terms of the time derivatives of particle velocity (i.e., the acceleration) and temperature. By subtracting from (
4) its conditional average, the particle temperature and velocity fluctuations can be expressed in terms of the fluctuations of the time derivatives, i.e.,
where fluid velocity and temperature are to be computed at particle position. In the following, we will skip the apex from all moments that are second order or higher to keep notations simple. By multiplying the particle temperature fluctuation (
12) equation by
and
and conditionally averaging, we have
Therefore, the ratio of particle temperature variance to fluid temperature variance at particle position is
while, by multiplying (
12) by the temperature derivative and conditionally averaging, we have instead a relation for the variance of the temperature derivative,
Equations (
15) and (
16) are general and can help to analyze the role of particle thermal inertia in the fluid and particle temperature statistics. Given the self-similarity of the flow [
20], this ratio is independent from the position
and time
t. In the following, we will use it to discuss the behaviour of the flow in the central region of the mixing layer, in a thin region, of a thickness much less than
, where variance and heat flux have their maximum [
20]. All data presented in the figures refer to this zone, because the relative homogeneity of the flow in this zone [
32] allows for the reduction in noise in the processing of numerical data.
A few pieces of information can be directly inferred from these equations, in particular as regards the limiting cases. In the zero-thermal inertia limit,
, particle temperature variance and fluid temperature variance become the same, independently from the momentum relaxation time. On the other hand, in the opposite limit
, the ratio is equal to
. This shows the importance of particle temperature derivatives in the determination of particle temperature fluctuations. As discussed by Carbone et al. [
16] and Béc et al. [
18], particle thermal acceleration is responsible for particle–fluid small-scale thermal coupling even in the one-way coupling regime.
Indeed, they discussed the small-scale fluid–particle interaction on the basis of the statistics of the particle thermal acceleration
in one- and two-way coupling, leading to the conclusion that particle inertia generates a multifractal behaviour, as indicated by Lagrangian temperature structure functions. Such a lack of smoothness, defined by [
16] as thermal caustics, dominates at small scales, where particle temperature differences at small separation rapidly increase as the Stokes number and the thermal Stokes number are increased. Béc et al. [
18] related the onset of the fluid temperature fronts along a particle’s Lagrangian path to the dynamics of particle temperature acceleration, whose non-Gaussian statistics leads to multifractal behaviour. Note that at a fixed Stokes number we can use (
14) to understand the effect of particle thermal inertia at a very high thermal Stokes number. Even if particle inertia does not appear explicitly in Equations (
13)–(
15), inertia influences particle trajectories and therefore the fluid temperature at a particle’s position.
Figure 2a shows that the ratio of variances increases with
for any Stokes number at large
, i.e., at least when
, but the slope reduces at higher inertia, so that at fixed
,
Figure 2b, it always reduces if
. On the contrary, at low thermal inertia,
, particle temperature variance always remains lower than fluid temperature variance and approaches it in the
limit. In the one-way coupling regime, the denominator of (
15) is a function of St only, and increases with St (
Figure 3b) so that the thermal inertia acts only on
in the numerator (
Figure 3a).
In the two-way coupling case (
Figure 4), the growth with the thermal Stokes number is much faster, because the particles enhance the dissipation of fluid temperature variance [
16], and this effect grows monotonically with their thermal inertia. This is essentially in agreement with our previous results [
20], but in those works the ratio between particle thermal inertia and inertia is kept constant, so that an increase in inertia is associated with an increase in thermal inertia, and no independent limit with respect to each variable is possible. At very small St, when
increases, the particle variance deviates from the fluid temperature variance. The effect of thermal inertia is dominant over the particle inertia in all ranges of Stokes number. Particle temperature variance is maximum for small particles with large thermal inertia (i.e.,
and
), as the lag between
T and
induced by a large
allows for large particle temperatures deviations from the mean temperature of particles coming from the two homothermal regions. The minimum particle temperature variance occurs when particle relaxation time increases,
, for an intermediate thermal Stokes number, as
makes its variance equal to that one of the flow, and
makes it increase.
It should be noted that, in the two-way coupling regime, i.e., when the thermal feedback
is not neglected, the interplay in Equation (
15) is much more complex because
T is no longer independent from
so that numerator and denominator are coupled. The modulation of fluid temperature fluctuations implies that, even in the thermal ballistic limit
, the ratio
has no unique limit.
The effect of particle modulation of fluid fluctuations can be understood by comparing the fluid temperature variance in the one- and two- way coupling regimes, as in
Figure 5, which shows the ratio of the variance between the two regimes, as a function of St and
. The feedback of small particles, such that
and
, produces an increase in the fluid temperature variance, while larger particles with
,
always damp the fluid temperature fluctuations. This effect is more pronounced at large
, while the modulation of the flow temperature variance by particles is almost ineffective for
.
An equation for the ratio between particle and fluid variance in a homogeneous and isotropic flow has been proposed by [
34] on the basis of a Langevin equation for fluid temperature fluctuations and by [
16] from the properties of the general solution of the quasi-linear equation of particle temperature and the statistics of temperature increments at very small and very large time separations. In both cases an increase in thermal inertia always led to a reduction in the
ratio, as a larger inertia acts as a filter for the ambient fluctuations of
T seen by the particle during its trajectory, so that
where
is the time-scale of fluid temperature fluctuations sampled by the particle, proportional to the large-scale eddy turnover time
and
is a dimensionless coefficient, equal to 1 in [
16], which in [
34] depends on the “actual situation of the turbulence”, i.e., it is a fitting coefficient of the Langevin model which takes into account the effect of the finite Reynolds number on the temporal scale seen by an advected scalar. On the opposite, in the present flow configuration, a larger inertia allows more and more particles coming from one of the two homogeneous regions to keep their original temperature while they cross the thermal mixing layer, thus increasing the temperature variance inside the layer. Therefore, the presence of a temperature gradient imposed by the initial conditions, which creates a large-scale modulation of temperature on a length-scale
, prevails on the small-scale effects of spatial clustering of particles at local temperature fronts located in the high-strain regions by velocity fluctuations.
3.2. Velocity–Temperature Correlation
The same argument can be used to discuss the role of inertia on the velocity–temperature correlations, which define the heat transfer across the inhomogeneous layer. Indeed, by multiplying Equations (
11) and (
12) and taking the conditional average, one has
which could be conveniently divided by the fluid temperature–velocity correlation to obtain
Therefore, the particle contribution to the heat flux can be decomposed in terms of the correlations between the particle derivatives and between them and the fluid velocity and temperature fluctuations.
The ratio expressed in Equation (
18) is directly linked to the particle contribution to the heat flux across the thermal mixing layer, as detailed in Equation (
9) with respect to the convective heat flux and, as such, is one of the main objects of any modelling. The decomposition of the flux, as presented in Equation (
17), allows for an understanding of how particle heat flux is affected by the particle inertia and thermal inertia, both of which modulate particle velocity and temperature time derivatives. An overview of the correlation ratio (
18) is depicted in
Figure 6,
Figure 7 and
Figure 8.
Figure 6 portrays an overall view of the ratio between particle velocity–temperature correlation and fluid velocity–temperature correlation derived from 256 simulations in the one-way coupling regime and 221 simulations in the two-way coupling regimes.
This ratio consistently increases monotonically with thermal inertia (i.e.,
) at any given Stokes number, reaching an asymptotic limit dependent on the Stokes number. Particle inertia (i.e., St) makes this ratio peak when the particle relaxation time is of the same order as the Kolmogorov microscale (i.e.,
), a situation where particles are expulsed from the small-scale vortex cores. This is even more clearly visible in
Figure 7a, where each curve corresponds to a single Stokes number. Anyway, the limit for large Stokes number is always higher than one, that is, when the thermal Stokes number is large enough, particle velocity–temperature correlation becomes larger than the fluid–velocity correlation. By fitting the available data, the transition condition
, shown by the dashed line in
Figure 6, can be expressed as
with
,
and
in the one-way coupling regime, and
,
and
in the two-way coupling regime up to
, which then tends to be linear for
, with
when the curve is fitted for
. Any Stokes number below this threshold produces an increase in the correlation ratio, whereas for Stokes numbers larger than this threshold the ratio is below one. Thus, given
, it is possible to infer that, in the ballistic limit
, particle velocity and temperature consistently tend to decorrelate, irrespective of particle thermal inertia. However, in the thermal ballistic limit
, a notable correlation persists, consistently surpassing the fluid correlation, especially at a Stokes number around one. This decorrelation process operates at a slower pace in the two-way coupling regime due to the particle’s thermal feedback altering fluid temperature along its trajectory. Particularly, in this regime, the modulation of fluid temperature fluctuations by particles leads to a reduction in the convective heat flux
, as observed in [
20]. Simulating
is not possible in the two-way coupling scenario because the number of particles
scales as
, diverging for
. Consequently, only
could be represented in
Figure 7. This limitation is not present in the one-way coupling regime, because particles do not influence either each other nor the fluid phase, so that their actual number is irrelevant.
The data presented in [
20], where the ratio
was kept fixed, correspond to a diagonal cut in
Figure 6. Since
the higher the ratio of particle to fluid specific heat, the higher the overall correlation levels between particle temperature and velocity, because a lower portion of the map in
Figure 6 is sampled. To keep constant the ratio between
and St implies to fix the particle material while allowing the size to change so that, for any kind of particle, there is a critical Stokes number above which the correlation is lower than the fluid temperature–velocity correlation, and for increasing Stokes velocity and temperature, always decorrelate. This could not be seen in [
20] because the maximum simulated Stokes number was equal to 3.
In the two-way coupling regime, particle feedback tends to increase the ratio (
18), but most of the variations can be attributed to the resulting damping of fluid correlations (
Figure 7b) and not to an increase in particle correlations. This damping is an effect of particle preferential concentration near the temperature fronts, as described by [
16,
18] in homogeneous turbulence, which smooths the fluid temperature gradients. Indeed, only for a Stokes number larger than one is there a small range of
at which particle modulation of fluid fluctuations produces a slight increment in the fluid temperature–velocity correlation, which in all other situations is always reduced. This damping effect produces an overall reduction in the fluid heat flux across the thermal mixing layer except at low inertia.
To unravel how particle inertia and thermal inertia influence the heat transfer, we examine numerical simulation data by dissecting temperature–velocity correlation
using the decomposition of Equation (
18). The three addends outlined in Equation (
18) are shown in
Figure 9 and
Figure 10a for the one-way coupling case. The first term, depicted in
Figure 10a, is a function of St only in the one-way coupling regime, as particle velocity and fluid temperature are independent of particle thermal inertia in that case. Its magnitude diminishes with increasing St and exhibits a negative value, akin to the second term, shown in
Figure 9b. This term,
, displays a mild dependence on both St and
, varying no more than 2% within the investigated parameter range. Both these terms, in accordance with Equation (
18)’s signs, contribute to building the particle temperature–velocity correlation, thereby elevating heat transfer. Overall, their sum decreases with the Stokes number, with a minor influence of the thermal Stokes number. On the other hand, the third addend in Equation (
18), proportional to the correlation between the particle acceleration
and the temperature derivative
(
Figure 9a), is negative due to the presence of a mean temperature gradient. This term tends to diminish the
correlation, exhibiting more pronounced effects at lower Stokes numbers and diminishing with increasing St and
. These variations are more gradual than the first term, thus allowing for maximal correlation around
. However, it is responsible for the decorrelation at large St, given the strong dependence of the correlation between particle acceleration and temperature on St. This gradual reduction in the correlation with
is far less pronounced than the reduction in the thermal time derivative variance, as shown in
Figure 10b. The temperature time derivative variance increases with the Stokes number but reduces with the thermal Stokes number. It is worth noting that, based on Equation (
16), the temperature derivative variance is proportional to the difference between the correlation of fluid temperature and the temperature time derivative and the correlation between the particle temperature and the temperature time derivative. In homogeneous turbulence, the presence of a smooth temperature field leads to a finite limit of the variance of
for small thermal Stokes numbers [
16]. Conversely, in the opposite limit, with very large thermal inertia, the acceleration integral tends to be dominated by uncorrelated temperature increments, causing its variance to decrease as
[
16,
18]. The data illustrated in
Figure 10b indicate a low thermal inertia finite limit at all simulated Stokes numbers, suggesting a smooth temperature field. Meanwhile, the behaviour in the self-similar stage in the presence of high thermal inertia demonstrates the presence of well-mixed regions within the thermal mixing layer core, approaching the
asymptotic scaling found in homogeneous turbulence.