Search Results (2)

The study of localized surface plasmons (LSPs) in nanoscale structures is an essential step towards identifying optimal plasmonic modes that can facilitate robust optomechanical coupling and deepen our understanding of light–matter interactions at the nanoscale. This paper investigates, numerically, using the finite element method, LSP modes in a design comprising two coupled nano-ridges deposited on a gold layer with an interposing polymer spacer layer. Such a structure, usually referred to as a particle-on-mirror structure, shows exquisite optical properties at the nanoscale. We first examine the LSP modes of a single nano-ridge through the analysis of its scattering cross-section in the visible and infrared ranges. To enhance the plasmonic response, a thin polymer layer is placed at the middle of the ridge, which introduces additional LSP modes confined within the former. Then, we extend the analysis to the dimer configuration, which exhibits more complex and enhanced plasmonic behavior compared to a single nano-ridge. In particular, the dimer configuration yields LSP resonances with a quality factor enhancement of approximately threefold relative to a single nano-ridge. Furthermore, the presence of the polymer layer within the ridges significantly improves plasmon field localization and the quality factor. These findings underscore the potential of nano-ridge-based structures in advancing optomechanical coupling and offering valuable insights for the development of high-performance acousto-plasmonic devices. In particular, the proposed device could help significantly improve the design of nano-acousto-optic modulators, operating in the visible or in the near-infrared ranges, that require an enhanced light–phonon coupling rate. Full article

A direct comparison of simulation and experimental results of UV laser-induced surface nanostructuring of gold is presented. Theoretical simulations and experiments are performed on an identical spatial scale. The experimental results have been obtained by using a laser wavelength of 248 nm and a pulse length of 1.6 ps. A mask projection setup is applied to generate a spatially periodic intensity profile on a gold surface with a sinusoidal shape and periods of 270 nm, 350 nm, and 500 nm. The formation of structures at the surface upon single pulse irradiation is analyzed by scanning and transmission electron microscopy (SEM and TEM). For the simulations, a hybrid atomistic-continuum model capable of capturing the essential mechanisms responsible for the nanostructuring process is used to model the interaction of the laser pulse with the gold target and the subsequent time evolution of the system. The formation of narrow ridges composed of two colliding side walls is found in the simulation as well as in the experiment and the structures generated as a result of the material processing are categorized depending on the range of applied fluencies and periodicities. Full article