1. Introduction
The complex interaction of high-power laser with plasma has become a popular research topic due to its various applications in science and technology, including laser-driven inertial confined fusion (ICF) [
1], laser-driven accelerators [
2] and laser machining [
3]. The main research areas have focused on the propagation characteristics of high-power laser beams in plasma [
4,
5,
6]. The Drude model of electrical conduction is extensively considered in this research field [
7,
8]. Sharma et al. [
9] have found that the propagation characteristics of an intense laser beam in plasma depend on the power and width of the beam and the ratio of plasma frequency and light wave frequency. Wang et al. [
10] have investigated the propagation characteristics of a Gaussian laser beam in unmagnetized cold plasmas, based on the theory of ponderomotive nonlinearity. They also applied the Wentzel–Kramers–Brillouin (WKB) method to study the propagation characteristics of a Gaussian laser beam in cold plasma [
11]. However, since the above studies are conducted by only solving the scalar wave equation with complex eikonal function assumption and paraxial approximation, the obtained information about the dynamic laser-plasma interaction is limited. Additionally, the solutions are not accurate enough for tightly focused laser beams whose sizes are in the order of several wavelengths.
In recent decades, the finite-difference time-domain (FDTD) method has become a popular numerical technique in directly solving Maxwell’s curl equations [
12]. The FDTD method also has well-developed techniques for accurately simulating the Drude model [
13,
14,
15] and numerically generating any types of laser beams based on the total-field/scattered-field (TF/SF) technique [
16]. Therefore, the current study evaluates the FDTD method in investigating the propagation characteristics and relevant phenomena of high-power Laguerre-Gaussian laser beams in plasma.
2. Theoretical Background
In physical optics, the complex-form expression of the electric field of a Laguerre-Gaussian beam propagating in the free space under cylindrical coordinates
is given by:
where
is the nominal magnitude of light field of laser beam,
is the wave number of laser beam with wavelength
,
is the radius of beam waist,
is the beam size at distance
from the beam waist with Rayleigh range
,
is the complex beam parameter,
is the Gouy phase shift, and
are the associated Laguerre polynomials. Herewith, each Laguerre-Gaussian beam of
mode is specified by two mode indices, the angular mode index
and the transverse radial mode index
. It is noted that a Laguerre-Gaussian beam degenerates to the fundamental Gaussian beam when
. In this work, we focus on the category of vortex Laguerre-Gaussian laser beams with
. To maintain simplicity without losing generalizability, we investigate the propagation of two typical low-order Laguerre-Gaussian beams in plasma. The first one is the doughnut-shaped
laser beam with electric field written as:
Figure 1 shows the field magnitude and phase distributions of the
laser beam propagating in free space, where
and
are the magnitude and principal argument of the complex electric field
of laser beam given by Equation (1), respectively. The size of beam waist is
as depicted in
Figure 1, where
is the wavelength of laser beam. The distinct doughnut-shaped feature makes it ideal for applications in many areas of optics, such as optical trapping [
17] and optical tweezers [
18].
The second laser beam is the double-ring-shaped Laguerre-Gaussian vortex laser beam of
mode with its electric field given by
according to the associated Laguerre polynomial
.
Figure 2 shows the magnitude and phase distributions of an electric field of the Laguerre-Gaussian laser beam of
mode propagating in free space. Here, a smaller size of beam waist
is applied, which implies a larger diffraction effect as we can see from
Figure 2a. The cross-sectional view of field magnitude distribution
in
Figure 2b shows that the laser beam is double-ring-shaped.
The dynamic interaction of laser beams with plasma is complex and dependent on the level of laser power [
19]. When the intensity of the incident laser beam is low, the charged particles such as ions and electrons in plasma driven by the light fields are oscillating around their nearly-fixed oscillation centers. Therefore, the spatial distribution of the electron density keeps nearly unchanged. However, when the light intensity is extremely high, the spatially-inhomogeneous light beam exerts a significant nonlinear Lorentz force, called the ponderomotive force, on the charged particles in the plasma. Since the ponderomotive force scales with the inverse of particle mass, the ponderomotive effect on ions is generally negligible with respect to that of electrons. Thus, the electron density in plasma is manifestly changed by such a force until the balance is restored with the plasma pressure gradient force. According to the theory of ponderomotive nonlinearity, the redistributed electron density is exponentially dependent on the square of light-field magnitude
and is given by [
20]:
where
is the initial spatial distribution of electron density before the presence of laser beam,
is the square of light-field magnitude,
is the electron temperature of plasma in unit of kelvin,
is Boltzmann’s constant,
is the angular frequency of laser beam, and the coefficient
is defined for the sake of conciseness of following equations.
On the other hand, the electromagnetic properties of plasma are usually described by the famous Drude model of permittivity:
where
is permittivity of free space,
is the plasma frequency and
is the collision frequency. Theoretical derivations [
7,
11] demonstrated that
and
both are proportional to the electron density
. Therefore, for high-power laser beam incidence, both the plasma frequency and collision frequency are modulated by the square of field magnitude as follows:
and
where
and
are the initial plasma frequency and collision frequency before the incidence of laser beam. Thus, the modified Drude model of permittivity for describing the interaction of high-power laser beams with plasma is given by
As apparent in Equation (8), such a physical model of permittivity for plasma is related to the light intensity of laser beam. Therefore, it is a nonlinear and space-dependent model. According to the electromagnetic theory, the refractive index of a medium is
, where
and
are the relative permittivity and relative permeability of the medium, respectively. Since the relative permeability of plasma is usually defaulted to unit one
in the regime of optical frequencies, the complex refractive index of plasma is accordingly expressed as
which also reflects the dispersion and dissipation characteristics of the plasma.
3. Numerical Methodology
The Laguerre-Gaussian laser beams are numerically generated by utilizing the FDTD method based on the total field/scattering field (TF/SF) source condition [
12,
16]. It is possible to generate any types of laser beams with predefined pattern and parameters using this technique. Within the framework of FDTD method, assuming that the TF/SF interface is perpendicular to the
axis and locates at
, the
component of scattering magnetic field
on the plane
at time instant
can be updated by:
where the first item on the right side of (10) is the FDTD updating equation for
and the last item is the
component of the electric field of the to-be-generated laser beam,
Similarly, the
component of scattering magnetic field:
where the last item is the
component of the electric field of the to-be-generated laser beam:
Typically, the TF/SF interface is set at or near the plane of beam waist for convenience purposes, where the electric field has the simplest expression and there is no component of electric field.
The bilinear transform (BT) approach [
13] can be used to implement the complex dispersive model given by Equation (8) via the numerical implementation of the constitutive equation,
, within the frame work of FDTD method. The BT approach is not only accurate, but also stable with a stability limit that is equal to the Courant stability limit,
, where
is the shortest side of Yee cell,
is the speed of light, and
is the dimensionality of the simulated problem. In fact, we can first introduce the auxiliary quantity:
so that:
Subsequently, by applying the bilinear transformation
to transform Equation (15) from the frequency domain to the Z domain and noting that
and
, we have the updating equation for the discrete time-domain relationship between
and
:
where
,
, and
with
. By substituting Equation (16) into Equation (15), we have the final updating equation for
:
after some mathematical manipulation. However, the coefficients
,
, and
are dependent on
that is related to
. Thus, we also need to extract the parameter
. According to the time-harmonic property of a coherent laser beam,
can be numerically extracted by applying the composite trapezoidal rule within the discrete framework of FDTD method [
20],
where
is an even number of time steps per period of laser oscillation.
4. Simulation Results
The propagation characteristics of the
-polarized high-power
laser beam in plasma is first modeled and simulated. The laser beam used is as the one depicted in
Figure 1, where the beam waist
with the wavelength
in the ultraviolet region. The nominal electric field of the laser beam is
, which is feasible and practicable in modern giant laser facilities [
1]. The total three-dimensional computational region for the following FDTD simulations is
in the
,
, and
directions and is surrounded by perfectly matched layers (PMLs). A cubic Yee cell with size
is applied for the space discretization. The initial electron density of simulated plasma is spatially homogeneous with
and the collision frequency is
. As the interaction process is simulated in a relatively short time
for a total of 3000 time steps, a constant electron temperature
is also considered.
Figure 3a,b show the simulation results for the longitudinal views of the redistributed light field magnitude of high-power doughnut-shaped
laser beam on the
and
planes, respectively, when it propagates in plasma.
Figure 4a–f show the cross-sectional views of light field magnitude of
laser beam at several propagation distances
,
,
,
,
and
from the beam waist. The dynamic interaction process between the
laser beam and plasma are vividly recorded in
Videos S1 and S2. See
Supplementary Videos S1 and S2 for details.
Secondly, the propagation characteristics of the
-polarized high-power
laser beam in plasma is modeled and simulated. The investigated laser beam is as the one depicted in
Figure 2 and the parameters for wavelength and light-field intensity are the same as those of the
laser beam. The parameters for FDTD simulations and plasma parameters are also the same as the first numerical example.
Figure 5a,b show the simulation results for the longitudinal views of the redistributed light field magnitude of high-power double-ring-shaped
laser beam on the
and
planes, respectively, when it is propagating in plasma.
Figure 6a–f show the cross-sectional views of light field magnitude of
laser beam at several specified propagation distances
,
,
,
,
and
from the beam waist. The dynamic interaction process between the
laser beam and plasma are vividly recorded in
Videos S3 and S4. See
Supplementary Videos S3 and S4 for details.
5. Discussion
From
Figure 3 and
Figure 5, it is noted that the self-focusing and absorption phenomena of high-power laser beams in plasma are evident as compared with those propagating in free space as illustrated in
Figure 1 and
Figure 2. The physical model of permittivity with ponderomotive nonlinearity given by Equation (8) determines that the refractive index of plasma is smaller at the place where the light intensity is lower and larger where the light intensity is stronger. The ensuing inhomogeneous distribution of refractive-index attribute to the self-focusing effect and the laser beam is therefore focused when this effect overly counteracts the natural diffractive divergence of the laser beam. This is apparent from
Figure 4 and
Figure 6 in which the cross-sectional profiles of the light fields of
and
vortex laser beams within the plasma first experienced self-focusing and then stochastic absorption.
Video S2 and Video S4 vividly displayed the rotations and temporal evolutions of the cross-sectional light fields of
and
laser beams, which demonstrate the vortex features of the LG laser beams. We also note that the field distributions of the
and
planes are different from each other since the two laser beams are both linearly polarized in the
direction.
We also highlight the ribbons with half-wavelength intervals in
Figure 3 and
Figure 5. Since the incident laser beams are assumed spatially coherent, the transient light intensity proportional to
is also harmonic with a half-wavelength period. In each half period of space, the electrons at the place with high transient light intensity are pushed to the place with low transient light intensity. According to Equations (4) and (9), this intensifies the difference of refractive indices at the two places and the half-wavelength electron-free elongated cavities are formed. The ensuing high reflection of light at the walls of cavities causes the ribbon phenomenon. Moreover, the speckles found in
Figure 4 and
Figure 6 can be attributed to the Rayleigh-Taylor fluid mechanics instability [
19] under the local oscillation electronic acceleration mechanism. Once the initial laser beam has a small-scale perturbation or is disturbed by the unevenly medium when it propagates in the plasma, a rapid light intensity growth will occur in the near region that forms a speckle in the cross-sectional patter of the laser beam. It can be estimated that different modulation effects of light fields can be achieved by using LG laser beams of other polarization states, such as the radial and azimuthal polarizations. Thus, the plasma can serve as a new medium for modulating the LG beams into the desired field patterns.