Collaborative Purification of Tert-Butanol and N2O over Fe/Co-Zeolite Catalysts
Abstract
:1. Introduction
2. Materials and Methods
2.1. Catalyst Preparation
2.2. Catalytic Performance Tests
2.3. Catalyst Characterization
3. Results and Discussion
3.1. Characterization
3.1.1. XRD
3.1.2. N2 Adsorption/Desorption
3.1.3. XPS
3.1.4. UV−Vis
3.1.5. Temperature−Programmed Reduction by Hydrogen
3.2. Activity Measurement
3.2.1. Activity Comparison on Different Fe Zeolite Catalysts
3.2.2. Activity Comparison of Different Co Zeolite Catalysts
3.2.3. Activity Comparison of Fe-BEA with Different Concentrations
3.2.4. Activity Comparison of Co-BEA with Different Concentrations
4. Conclusions
Supplementary Materials
Author Contributions
Funding
Institutional Review Board Statement
Informed Consent Statement
Data Availability Statement
Acknowledgments
Conflicts of Interest
References
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Samples | Surface Area m2/g | Micropore Volume cm3/g | Average Pore Diameter nm |
---|---|---|---|
H-BEA | 562.0 | 0.18 | 15.0 |
0.25% Fe-BEA | 490.1 | 0.14 | 14.0 |
0.5% Fe-BEA | 463.7 | 0.15 | 15.8 |
1% Fe-BEA | 449.8 | 0.13 | 14.7 |
1.5% Fe-BEA | 414.7 | 0.11 | 13.2 |
2% Fe-BEA | 421.1 | 0.15 | 15.2 |
0.25% Co-BEA | 544.31 | 0.17 | 16.70 |
0.5% Co-BEA | 561.71 | 0.17 | 14.85 |
1% Co-BEA | 471.31 | 0.14 | 15.80 |
1.5% Co-BEA | 488.65 | 0.14 | 15.79 |
2% Co-BEA | 483.66 | 0.13 | 14.09 |
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Wu, R.; Liu, N.; Dai, C.; Xu, R.; Wang, N.; Yu, G.; Chen, B. Collaborative Purification of Tert-Butanol and N2O over Fe/Co-Zeolite Catalysts. Int. J. Environ. Res. Public Health 2023, 20, 4902. https://doi.org/10.3390/ijerph20064902
Wu R, Liu N, Dai C, Xu R, Wang N, Yu G, Chen B. Collaborative Purification of Tert-Butanol and N2O over Fe/Co-Zeolite Catalysts. International Journal of Environmental Research and Public Health. 2023; 20(6):4902. https://doi.org/10.3390/ijerph20064902
Chicago/Turabian StyleWu, Ruiqi, Ning Liu, Chengna Dai, Ruinian Xu, Ning Wang, Gangqiang Yu, and Biaohua Chen. 2023. "Collaborative Purification of Tert-Butanol and N2O over Fe/Co-Zeolite Catalysts" International Journal of Environmental Research and Public Health 20, no. 6: 4902. https://doi.org/10.3390/ijerph20064902