1. Introduction
State-of-the-art conventional accelerators are quite large and expensive to maintain. Decades ago, laser-driven plasma accelerators were proposed as a future alternative by T. Tajima and J. M. Dawson [
1]. Laser–plasma wakefield acceleration (LWFA) is a promising approach for the generation of bright, ultrarelativistic electron beams for numerous applications in a compact manner. The basic principle employs a high-power, ultrashort laser pulse propagating through a low-density gas target generating a plasma wakefield leading to the separation of ions and electrons, thereby building up an electric field of the order of 100
/
. Electrons that are trapped in this wake can be accelerated to energies in the
range over very short distances (10
−2 m range). Their advantages, such as femtosecond pulse duration and high peak currents, make them attractive for a number of scientific and industrial applications [
2,
3,
4,
5].
Generally, 100 TW or even TW-scale laser systems are employed to drive such accelerators. There is a great interest in the pursuit of laser–plasma acceleration reaching electron energies in the
range to drive advanced light sources such as free electron lasers or provide technical and scientific knowledge for linear colliders in high-energy physics [
6]. The realization of such applications relies on Tera- to Peta-Watt-scale laser systems that operate at a few Hertz repetition rates [
7].
However, the required high-power laser systems that are up to date are only available in dedicated laser facilities that can provide the essential research environment. The operation of these systems is very demanding and requires large highly specialized groups with strong expertise. Nevertheless, various applications do not rely on such high-energy electrons. For example, lower-energy electrons (in the range of 10
) can be used in radiobiological experiments to study the effect of fractional dose delivery [
8]. Lower energy electrons can also be used in radiation hardness studies for space electronics [
5] and to investigate the dynamics of matter by ultrafast electron diffraction [
9].
Available laser systems on the 100
scale run at
repetition rates or less and are predominantly based on the Ti:Sapphire technology. However, many applications would benefit from higher repetition rates. Despite providing less energy,
laser systems at
repetition rates combined with a postcompression scheme to reach few-cycle pulses and a tight-focus geometry have already proven their potential for a few
laser–plasma accelerators [
10] and for delivering e-beams with long-term stability [
11]. In addition, recent advances in laser research such as multipass cell postcompression schemes [
12], high-energy optical parametric chirped pulse amplification [
13] (OPCPA), or the use of alternative laser media (e.g., Yb) [
14,
15] are promising developments toward suitable lasers for driving robust and reliable laser–plasma accelerators (LPA) for real-life applications.
In this work, we introduce the e-KAIO (electron Kit-All-in-One), which is a joint effort with the company SourceLAB and a first step towards making LPA technology more accessible to a broader community in scientific research and industry. The main goal of the e-KAIO-beamline is to overcome the current weaknesses of laser–plasma accelerators by mainly employing industrial standard components to realize a much more cost-effective, compact, reliable, and easy-to-use laser–plasma accelerator. To this end, the interaction chamber is combined with an industrial-grade laser system, and possibly, an intermediate postcompression scheme will be added in the future.
Here, the first proof-of-principle experiments are presented, demonstrating the functionality of the e-KAIO chamber. In
Section 2, we discuss the challenges of laser–plasma acceleration (LPA), specifically at high repetition rates, before giving a technical overview of the e-KAIO submodule and its advanced diagnostic, specifically designed for LPA and its application in
Section 3. This includes a detailed characterization of the Coherent Astrella laser system as a driving laser crucial for a controlled laser–plasma interaction. Afterward, we present and discuss our first results in
Section 4 and give an outlook toward future experiments in
Section 5.
2. Design Criteria for LPA at High Repetition Rates
To design a laser–plasma accelerator, it is important to consider the involved scaling laws to estimate the expected electron energies for a given driving laser. Furthermore, there are certain aspects regarding the experimental design when dealing with LPA at high repetition rates that we discuss below.
Depending on the experimental conditions, there are several different regimes where electrons can be accelerated effectively. Subrelativistic electron beams with relatively low charge can be produced utilizing the density down-ramp injection [
16], when working with laser pulses of a few
at tens of
pulse duration. Using ultra-high-density gas targets, the authors of Salehi et al. [
17] were able to produce relativistic electron beams at
repetition rate operating in the self-modulated regime. The resulting electron beam is fairly divergent and has a Maxwellian distribution. To reduce the energy spread of the electron beam it is favorable to work in the so-called blow-out or bubble regime [
18,
19,
20,
21]. The resulting electron beams typically have a small divergence while still maintaining relativistic energies, which makes them highly suitable for numerous applications. Provided the electron injection is properly controlled, the scaling law of Lu [
22] can be used to predict the acceleration gradients generated in such strongly nonlinear plasma wakefields. To optimize the output energies, the experimental conditions have to be tuned for the laser pulse to be in resonance with the created plasma cavity. Assuming a near-spherical shape of
R (given by half the plasma wavelength
) both the transverse and longitudinal pulse size have to be of similar dimension, i.e.,
, where
c is the speed of light,
the pulse duration, and
the beam waist. By matching the transverse dimension of the laser pulse and the plasma cavity, one ensures that the ponderomotive force exerted on the electrons is balanced by the Coulomb force of the ions inside the plasma cavity. In addition, the laser–plasma interaction leads to etching via energy depletion and redshift of the pulse over a length
. Ideally, this pulse degradation is limited to the time that the electron bunch is in phase with the plasma wakefield within the distance
-leading to the second condition
. When both conditions are met, the maximum wakefield amplitude is
, where
is the cold wavebreaking field,
the electron mass,
the plasma frequency, and
the normalized vector potential of the driving laser of frequency
. The maximum electron energy gain is then given by
In addition to the spatial resonance discussed, the above laser propagation plays a crucial role as the dephasing length usually exceeds the Rayleigh range given by the chosen focus geometry. To extend the interaction length (such that maximum electron energy gain can be reached), one utilizes the effect of self-focusing which counteracts the diffraction effects and helps to maintain the transverse and longitudinal resonance. For self-focusing to occur, the peak power
P of the laser pulse should exceed the usual threshold for relativistic self-focusing
, which is
. As found by Lu et al. [
22], when working in the bubble regime, this condition has to be altered to
, as the wakefield has a predominant effect on the propagation.
Following the scaling laws, one usually finds that for laser systems operating at repetition rate, the resonance conditions place high demands on the experimental conditions.
Due to the limited pulse energy of high repetition rate laser systems, one usually has to work in a tight focusing geometry to reach the limit of relativistic self-focusing, which is a requirement for electron injection in any regime. At very high target pressures (
), electron injection can be achieved even for pulse energies of a few mJ [
17] and pulse durations around ~30
even outside the bubble regime. To optimize the electron acceleration and beam quality, an additional postcompression scheme has to be employed to work in the bubble regime by lowering the pulse duration. In the extreme limit, this means working in the few-cycle regime, where effects based on the carrier-envelope phase (CEP) can modify the electron output characteristics [
23]. For a given pulse energy
and
at a fixed value for
, one can find the required beam waist
and pulse duration
. The lower the pulse energy, the shorter the focus geometry and pulse duration that have to be chosen, leading to dephasing and Rayleigh lengths of tens of
. Consequently, the gas targets used should have density gradients of similar dimensions or even smaller to optimize the coupling of the laser into the jet and avoid ionization-induced defocusing [
24]. In addition, the electron density needs to be on the order of
ne = 10
20 cm
−3 to reach the resonant regime as
. To ensure the laser does not damage the gas nozzle, the interaction region should be at least 100
above, which can be realized by using super-sonic or shocked nozzles [
25]. Extensive diagnostics must be implemented to check the target and plasma density distribution above the jet. In addition, a pump–probe line is needed to observe the plasma processes with sufficiently good temporal resolution and check the target condition between successive laser interactions (no preionization). Finally, the target gas should flow continuously to allow operation at high repetition rates while maintaining an ambient pressure of 10
−2 inside the interaction chamber.
An example of possible experimental conditions in the bubble regime is given in
Table 1.
3. e-KAIO Chamber and Laser–Plasma Diagnostics
The progress of laser–plasma accelerators in the last decades has established this technology as a potential candidate for future accelerators, not only for research but also for industrial and societal applications. The numerous advantages of LPA-produced electron beams (micrometer-scale source size, femtosecond pulse durations, high peak currents) make them ideally suited to ultrafast electron diffraction, nondestructive imaging, radiobiology, or space radiation production. At a high repetition rate, LPA electron sources are particularly appealing, as they offer long-term stability and real-time access to statistics [
26], enabling efficient complex parametric studies (e.g., in radiobiology [
27]). This is supported by the fast progress in laser development, as by now there are multiple industrial-grade laser systems that are suitable as potential drivers at
repetition rates. These laser systems offer high reliability and ease of use, while still fulfilling the demanding output requirements for driving LPA.
Nowadays, LPA sources can be found mostly in the scientific community as operating these highly complex systems requires a lot of expertise and experience. Thus, implementing LPA sources at high repetition rates for applications remains challenging, as LPAs require laser drivers with both high average and high peak power, high-performance vacuum handling to manage the large target gas loads, and adequate management of large data sets generated during measurement runs.
The novel e-KAIO-beamline aims at addressing these challenges by combining three key ingredients: (i) an industrial high average power laser system, (ii) a versatile temporal pulse postcompression stage, and (iii) a compact electron accelerator module with an integrated user interface and data management system. The e-KAIO-beamline approach is compatible with a wide range of commercial laser platforms, as it is modular and features versatile postcompression based on multipass cell technology. Secondary electron and betatron radiation production is coupled to an automatic high repetition rate data acquisition program, which monitors and logs all relevant parameters during day-long experimental runs.
In the following, we discuss two major subcomponents of the e-KAIO-beamline, focusing on the e-KAIO chamber itself and the Astrella laser system by Coherent as a potential driver for LPA.
3.1. Interaction Chamber
The e-KAIO chamber is designed to produce
level electron beams at
when the accelerator is driven by few
and few
relativistic laser pulses. A user-friendly system allows fine adjustment of the central parameters essential for high-quality beams. These parameters include among other things the control of the laser beam alignment, the control of focal spot quality, the control of gas jet position, density, and profile, and the electron spectrometer dispersion. Depending on the pulse length of the driving laser beam, different regimes of the laser–plasma interaction can be reached, thus offering different electron output characteristics as discussed in
Section 2 above. The e-KAIO is versatile and can be used in combination with different driving lasers and used for various applications. In the following, we discuss the different subcomponents of the system and show how it is perfectly adapted to tackle the challenges of high-repetition-rate LPA.
The e-KAIO vacuum chamber is shown in
Figure 1 and can be operated even in small experimental areas. The vacuum chamber itself is carried by an outer support structure, and the inner breadboard is mechanically isolated from the chamber walls by flexible bellows to reduce vibrations produced by the pumping system or the surroundings. The dimensions of the vacuum chamber itself are 500 mm × 900 mm × 450
, and the optical entrance window supports beam diameters up to
. The e-KAIO chamber provides multiple diagnostics for monitoring the laser beam or studying the electron beam. The optical diagnostics are installed outside of the chamber including six CCD cameras that are connected to the KAIO control computer. A detailed overview is shown in
Figure 2. The input beam is recorded by two reference CCDs which can be used for alignment references, thus enabling a quick realignment procedure from day-to-day operation. In addition, the references can be used for active (automatized) beam stabilization as they are coupled to piezo-motors controlling the position and pointing of the input beam. In this mode, the drift or misalignment of the laser beam will be corrected automatically by moving the pico-motors of the two last mirrors before the focusing off-axis parabola. This option is useful during the pumping of the chamber under conditions of strong vibrations and/or mechanical stress, as well as during long-term system operation. The alignment references are shown in the upper left of
Figure 3, and the integrated signal of one of the cameras can be used to track the average power stability of the laser. In addition, the deviation from the set reference can be recorded to investigate the beam drift and pointing under different conditions. For prealignment purposes, the e-KAIO chamber is equipped with a red alignment laser diode, which has the same path and close central wavelength as the actual femtosecond laser. This allows one to align equipment without having to use a high-intensity laser. The mirrors and off-axis parabola used for focusing the beam are motorized and can be positioned via the control unit and the dedicated computer. The beam is focused by a
or
off-axis-parabola and the attenuated focal spot can be imaged by an objective when the flip mirror in front of the gas jet is up. The gas jet is installed on a 3-directional translation stage and can be moved with micrometer precision. During the interaction of the high-intensity laser beam and the gas jet electrons are accelerated which follow the axis of the main laser beam direction. These electrons are detected via a scintillator (Hamamatsu FOS J6677) screen, and the converted visible light is further recorded by a CCD camera after passing an interference filter. Additionally, a magnetic spectrometer can be implemented in the electron beam axis as needed.
The spectrometer consists of a pinhole and a pair of permanent magnets positioned on individual translation stages. By adjusting the distance of the magnets, the magnetic field strength can be adjusted to vary the electron dispersion. The field strength is precalibrated, and the dispersion axis is shown in the user interface (upper right in
Figure 3). At the back of the interaction chamber are multiple vacuum flanges as a feed-through for additional diagnostic, to connect a beamline for further manipulation of the electron beam, or to measure the source output (such as beam charge).
3.2. User Interface and Data Acquisition
The e-KAIO beamline has a Graphic User Interface (GUI) that allows online control of all parameters and data acquisition. In
Figure 3, the user-friendly GUI overview of the e-KAIO chamber is shown. The interface supports the multiple CCD cameras, the several motorized translation stages, the piezo-motors for driving the mirrors, and also the data acquisition and storing. The interface not only allows monitoring and adjusting the parameters but also has a quick analysis of the focal spot and electron density, for instance. Similarly to the INSIGHT algorithm, the e-KAIO software (version 1.0) has an implemented GS algorithm to measure the spectrally averaged wavefront of the laser beam. The recorded images and values are stored in HDF5 files giving the possibility to store large amounts of data. To reproduce and keep track of the experimental conditions used, a tagging function is included in the HDF5 file-saving option.
3.3. Laser System and Diagnostics
The first experimental studies were carried out with the Astrella laser provided by Coherent. This Astrella laser combines industry-leading performance and durability. Having a tabletop, one-box size enables the availability for various applications and operating conditions. The Astrella laser system delivers up to 9
/pulse and a pulse range of 35–100 fs at a repetition rate of 1
. The nominal beam diameter is around
at a divergence angle of
1–2 mrad. Different measurements were performed employing various devices to characterize the laser system. We found a relative average power stability of ±3.8% using the alignment reference CCD (limited by vibrations and airflow in the lab). A more representative (nonlinear) measurement was found using the TIPTOE background measurement ionization yield, which was stable within a standard deviation of ±2.1%. Temporal characterization is achieved using TIPTOE [
28], which is a broadband time-domain autocorrelator. By adapting the scanning range of the device, one can either characterize the main pulse to obtain access to the temporal shape and its spectral phase, or one can scan a wider temporal window to check the
contrast.
The pulse measurements are plotted in
Figure 4. The strong third-order dispersion of the spectral phase (b) limits the pulse duration to
and leads to additional side peaks after the main pulse (a).
Figure 5 shows the temporal contrast of the Astrella laser pulse determined with the TIPTOE device. The three differently colored traces represent measurements that were performed within two months. The laser system is proven to be stable within its specifications, and the contrast measurements were reproducible. Assuming a peak intensity of 1 × 10
18 W cm
−2, the temporal contrast is reasonably good to prevent preionization of the gas target between two consecutive shots when using helium or argon.
The measurements taken by TIPTOE provide a spatially averaged signal, since the device integrates over the entire ionization volume at the laser focus. Thus, the measurements are insensitive to any spatiotemporal couplings (STCs). For this reason, another device, the so-called INSIGHT [
29] (SourceLab), was used to characterize the spatiotemporal distribution of the laser pulses. The INSIGHT measurements are performed by focusing the laser beam using a
achromatic lens, and a spatially resolved spectrum is taken at the focus and one each before and after at approximately
. The spectrally resolved wavefront can be recovered using an adapted version of the Gerchberg–Saxton (GS) iterative algorithm [
30]. In
Figure 4c, the three-dimensional spectrally resolved focus is shown. The spectral components are well aligned along the propagation axis, which indicates there are no significant STCs such as pulse front tilt or higher-order effects, which reduce the far-field intensity.
5. Conclusions and Outlook
We present the e-KAIO chamber, a submodule for the e-KAIO-beamline, a versatile electron accelerator for various applications. Our first proof-of-principles experiments demonstrated the capability of the e-KAIO chamber to accommodate an industrialized laser system. The first results show that the alignment and data acquisition using the e-KAIO chamber is straightforward and can be easily carried out in different laboratories or working environments. To achieve shorter pulse duration and higher intensities, it is foreseen to repeat the experiments with a postcompression stage. This implies that, by using higher intensities at shorter pulse durations, it is possible to reach the point where the laser and target parameters interact in a way that is conducive to effective electron acceleration. The experimental results are listed in
Table 2 below. The first line summarizes the experimental results of this paper. The focal intensity (or normalized vector potential
) is mainly limited by the OAP’s aberrations and the laser pulse’s third-order dispersion. This also limits the self-focusing
(
in the bubble regime) at the measured target pressures, which is essential for electron injection. A first step toward low-energy electron acceleration (
level) working in the self-injection regime would be the optimization of the focal spot and the pulse duration down to 30
, while increasing the target pressure. A further increase in the plasma density could be reached by using molecular nitrogen as the target gas (10 electrons per molecule). Potential experimental parameters are given in the third line of
Table 2. To reach electron energies in the
range, a postcompression scheme needs to be implemented to reach the bubble or resonant regime (second line in
Table 2). A multi-pass-cell postcompression scheme with a total transmission of around 80% is planned for future experiments.
The e-KAIO interaction chamber is a first step in reaching the goal of a table-top laser–plasma electron accelerator on a university scale accessible for different potential applications. It can provide a structural change in the availability of laser–plasma accelerators that will advance the research and progress of developing a system suitable for industrial applications. This will give opportunities to drive the research forward and make electron accelerators available on a smaller scale. Therefore, research and applications will advance further.