1. Introduction
Oil still covers about 10% of the heating demand in the world [
1] and 12% in the European Union [
2], yet its use is declining due to the increased fuel cost (e.g., it has more than tripled in the USA since 2000 [
3]) and the high emissions of pollutants and greenhouse gases. The frequent occurrence of leakage episodes from underground storage tanks (USTs) is another major concern due to the consequent expense for tank removal, environmental investigations and possible remediation of soil and groundwater. Interest on this topic was first raised in the Eighties in the USA, as the US Environmental Protection Agency (USEPA) developed a specific program which identified more than 3.5 million USTs [
4]. Since then, more than 500,000 leakage episodes have been observed according to different sources [
5,
6,
7]. As for causes, Ram et al. [
5] found that 74% of fuel releases occur in the tank and/or the pipes, where structural failure (46%), corrosion (27%), and loose fittings (12%) are the most common causes, while the rest is due to incorrect filling operations. The remediation costs for leaking underground storage tanks (LUST) are very large relatively to the small ground volume involved, ranging between 142k
$ and 329k
$ per each site in the USA [
5,
6].
Recently, the GRETA project [
8] addressed the issue of LUST in Aosta Valley (NW Italy) [
9], a small mountainous Italian region (3261 km
2, 128,230 inhabitants) where, as shown later, oil heating is still quite used. Available data on soil and groundwater remediation procedures highlight that 68 suspect or actual leakage episodes occurred between 1999 and 2018, which involved heating fuel tanks, gas stations and other kinds of hydrocarbon storage, as reported in
Table 1. Ten of these 68 sites have been remediated with a median cost of 114k€ which is consistent with data from the USA [
5,
6].
Data highlight that a large share of leaking episodes occurred in gas stations, where possible failures in USTs are more likely to be detected due to the strict monitoring of fillings and sales and to the periodic controls on the structural integrity of the tanks. On the other hand, relatively a few procedures involve heating fuel tanks, which represent almost all USTs but are not subjected to any compulsory monitoring: for these tanks, leaking occurrence has, therefore, generally been revealed by odors or iridescent spots on surficial waters. Regional guidelines have been recently published in the Aosta Valley region aimed at gas stations USTs but containing good practices applicable also to the periodic monitoring of heating oil tanks [
10].
The phase-out of residential oil heating has been addressed in a few studies so far. Hast et al. [
11] found that replacing oil heating in Finland is economically convenient at the end of the operational lifetime of the boiler, while an early replacement strongly depends on the oil price. Most studies agree that the operational costs are the main driver for the choice of alternative heating techniques [
11,
12], although residential users are more likely to consider other factors such as comfort and reliability [
13]. As for environmental impacts of oil heating, Kheirbek et al. [
14] state that phasing it out in New York State and City would avoid 290 premature deaths per year thanks to the reduction of PM 2.5 concentrations. However, the replacing technique should also be considered: for example, shifting 20% of heating systems from oil with wood burning in Thessaloniki resulted in a +52% increase of PM 2.5, which is deemed responsible for about 200 premature deaths per year [
15].
These studies provide a knowledge base for the work presented in this paper, which comprehensively addresses the issue of replacement of oil boilers, with an application to the case study area of Aosta Valley. The practical issues of replacement heating techniques, such as fuel storage, civil engineering works, terminals, and operation are examined to identify potential operating contexts. The environmental impact of heating and domestic hot water (DHW) production is then evaluated through an analysis of greenhouse gas and air pollutant emission factors. Operational costs are estimated based on a research on the Italian market, and trends are identified when available. The return on investment of replacing oil heating is analyzed with reference to two benchmark case studies, i.e., a detached house and a block of flats. The economic results are integrated with an analysis of environmental externalities (greenhouse gases and pollutant emissions) and then discussed, comparing strengths and weaknesses of each heating and DHW production technique and deriving policy recommendation to phase out oil heating.
2. Technical Analysis of Replacement Options for Oil Heating
Aosta Valley is a mountainous region with an average elevation of about 2100 m a.s.l. and a semi-continental, temperate to cold climate [
16]. Rainfall ranges from about 600 mm/year in the bottom valley to 1800 mm/year on the highest peaks, with a regional average of 950 mm/year and a clear correlation with altitude [
16]. Heating degree-days according to the Eurostat method [
17] range from 2400–2800 HDD in the bottom valley from Pont-Saint-Martin to Aosta, where most of the population lives, to more than 5000 HDD in the highest settlements such as Valtournenche [
18] (
Figure 1). These climatic factors explain why Aosta Valley is the Italian region with the highest heating expense per family in Italy [
19]. Getting into the detail of the energy sources used for heating, it turns out that oil is a residual option which is adopted in the case gas is not available [
2,
20]. Indeed, gas in Italy is much cheaper than oil since taxation on heating oil was raised in the mid-eighties [
20]. Data on the diffusion of gas grids highlight that 50 of 74 municipalities of Aosta Valley do not have any methane grid [
21], with a total population of about 27384 inhabitants (i.e., 21.4% of the population of Aosta Valley); the other 24 municipalities, mostly in the bottom valley from Pont-Saint-Martin to Saint-Pierre (
Figure 1), are partially covered by the methane pipelines and a lower usage of oil boilers which is limited to the areas not covered by the methane grid.
Therefore, the solutions considered in view of the phase-out of oil heating are the following: LPG boilers, wood-fueled (logs, chips, and pellets) boilers, and different kinds of heat pumps i.e., air-source (ASHP), ground-coupled heat pumps (GCHP), and groundwater heat pumps (GWHP).
The LPG boiler is the most similar technical solution to oil heating, since it provides unattended boiler operation with a single (or a few) tank refilling for each heating season, avoiding the more frequent maintenance operations required by wood-fueled boilers. In the case of leakage from LPG storage tanks (both above and underground) the fuel does not penetrate the ground and groundwater, and this prevents the contamination of the underground. On the other hand, LPG has the same GHG emissions of oil (as shown later in
Section 3) and it is the most expensive heating fuel. A new tank (above or underground) must also be installed to switch from oil to LPG.
Wood-fueled heating has become very popular in recent years in Italy, and in Aosta Valley it is used by almost half of the population according to national statistics [
19]. Three main kinds of wood fuel are available on the market: logs, chips, and pellets. Wood logs have the main advantage of possible self-production, which dramatically reduces their cost, but the hand loading of wood makes them unpractical for large size plants, e.g., for a block of flats. Wood chips are very cheap, they can be produced too, optimally exploiting forestry residues. The automatic loading makes them practical also for large-size systems such as district heating. Yet wood chips require large storage spaces, which could make them unpractical for residential application: about 1 m
3 of storage volume is required for 1 MWh of heat, i.e., 10 times the value heating oil. Wood pellets and logs are much denser, requiring respectively 0.35 m
3 and 0.45 m
3 of storage volume per MWh.
Wood pellet boilers combine the advantages of the automatic loading and the relatively small storage spaces required. They are generally sold in small bags of 15 kg, thus limiting dust and sawdust in the storage room. These practical advantages, combined with an affordable price, have contributed to the large diffusion of this fuel in the 2000’s, particularly in Italy which has become the second consumer (and the first importer) in the world [
23].
Both LPG and wood biomass boilers can be adapted to any kind of hydronic and aeraulic heating terminal, with no interventions nor replacement required, which is the main technical drawback of heat pumps. Indeed, the efficiency of heat pumps strongly depends on the operating temperature of the heating terminals. Radiant panels are the most suitable terminals, and fan coils provide a good performance too, while heat pumps are hardly suitable for high-temperature radiators, which are still the most used heating terminals. However, radiator over-sizing, building retrofitting and heat pump control could greatly improve heat pump efficiency [
24,
25].
Air-source heat pumps are the most widespread, covering 80% of the European heat pump market [
26], due to the lower cost of installation compared to the geothermal ones. In addition, the need for space to install ground heat exchangers or wells for geothermal heat pumps could switch the choice to air-source ones, e.g., in the case of an autonomous installation in a block of flats. The main drawbacks of air-source heat pumps are the noise [
27,
28], the reduction of thermal power delivered at low air temperatures and, in the presence of moist air, frosting [
29,
30]. Geothermal heat pumps use ground (ground-coupled, GCHP) or groundwater (GWHP) as a heat source or sink [
31,
32]. The need for borehole heat exchangers (BHEs) or wells increases the installation costs, but geothermal heat pumps are far more efficient than air-source ones [
33]. Ground-coupled heat pumps (GCHPs), also known as closed-loop geothermal heat pumps, exchange heat with the ground through a closed pipe loop buried in the ground, usually in vertical boreholes drilled on purpose and called borehole heat exchangers (BHEs). Groundwater Heat Pumps (GWHPs), also known as open-loop geothermal heat pumps, exchange heat directly with groundwater abstracted by one or more wells; after the heat exchange takes place, water usually gets disposed into the same aquifer. This practice is allowed by the Italian law [
34] but not in the Aosta Valley region, and this represents a major barrier to the diffusion of open-loop geothermal systems in a territory which would have a great potential for this technique [
35,
36].
The use of air-source heat pumps (ASHPs) dedicated to the production of DHW has grown recently due to their relatively low cost and high efficiency [
26]. The DHW heat pump could be a viable solution for both wood-fueled boilers, allowing to have them switched off out of the heating season, and for all kinds of centralized space heating systems, for the separate production of DHW.
3. GHG and Pollutant Emission Factors of Different Heating Techniques
Aside from the prevention of soil and groundwater pollution, the replacement of oil heating systems reduces greenhouse gases (GHG) and air pollutant emissions.
Table 2 reports a comparison of CO
2 and pollutants emission factors related to different kinds of boilers, derived from the LCA database GEMIS 4.95–Global Emissions Model for integrated Systems [
37]. GEMIS considers biomasses as carbon neutral (0 gCO
2/kWh
th), although this assumption is not shared in related literature; for this reason, we considered other sources [
38,
39] to derive CO
2 emission factors for wood logs, chips, and pellets.
The comparison among fuels highlights that oil and LPG are the most carbon-intensive fuels, followed by methane (−12.7%), which is reported in
Table 2 as a term of comparison but is not considered as a replacement option for oil: indeed, methane in Italy is much cheaper than oil for heating (−41%), and it requires a minimal investment for the replacement of the boiler. For this reason, as shown above, a negligible number of oil boilers is present in areas covered by the methane grid.
The CO
2 emission factors of fossil fuels provided by different sources vary in small ranges, since such emissions are almost exclusively due to their combustion. On the other hand, the carbon footprint of wood and derivates depends on transport distances and on the energy used for the transformation operations of wood (sawing, chipping, and pellettization), while CO
2 emissions of wood combustion are considered as perfectly compensated by those removed by trees during their life cycle. Regarding pellet and wood chips, we have considered the values provided by Sjølie and Solberg [
39] who analyzed the production of pellets with Canadian wood exported in Norway. They derive an emission factor between 113 and 482 kgCO
2/ton of pellets, equal to 22–93 gCO
2/kWh
th assuming a typical Lower Heating Value (LHV) of 5.2 kWh/kg of pellets. The lowest value (22 gCO
2/kWh
th), based on an on-site production in Norway and truck transportation to Germany (from Averøy to Hamburg, about 1300 km), could be considered as representative of the Italian situation, where 81% of pellets are imported, mostly from Austria (28%) and other EU countries (40%) within 1500 km distance from Aosta Valley [
40]. The CO
2 footprint of wood chips could be estimated to 100 kgCO
2/ton of pellets (i.e., 19 gCO
2/kWh
th) by removing the contribution of the transformation of wood chips into pellets (13 kgCO
2/tons pellets). As a simplifying assumption, we assume that the mass reduction in the transformation from moist chips to pellets is perfectly compensated by the increase of LHV. Regarding wood logs, Klein et al. [
38] found CO
2 emission factors for different wood types in Bavaria (Germany) ranging between 9 and 15 kgCO
2/m
3 of dry wood, i.e., about 2–6 gCO
2/kWh
th. For this study, we adopted the highest value (6 gCO
2/kWh
th) considering a short supply chain with a negligible transport contribution to CO
2 emissions. The values of CO
2 emission factors assigned to wood-fueled boilers are in the orders of magnitude provided by other literature sources [
41,
42] and, unless we consider very long supply chains (e.g., American or Asian raw wood), the abatement of CO
2 emissions exceeds 80% with respect to methane, LPG, and oil.
Methane and nitrous oxide emissions were also considered to assess the total GHG effect as CO
2 equivalent. The 20-years GWP values provided by the AP5 report of the International Panel on Climate Change [
43], i.e., 84 for methane (CH
4) and 264 for nitrous oxide (N
2O). As show in
Table 2, emissions from fossil fuels and wood pellets are slightly increased, while a noticeable increase occurs for wood logs and chips due to the higher emissions of methane.
Other environmental factors should, however, be considered in the evaluation of different fuels. Wood biomasses are responsible for high emissions of air pollutants such as SO
2 (with emissions similar to those of oil boilers), NO
x, CO, VOC etc. The highest concern is raised by particulate matters, and numerous studies highlighted the impact of wood burning on air quality and their adverse impact on health. In the Po Plain, the contribution of wood burning to high air concentrations of PM10 and PM2.5 is in the order of 50% during winter time [
44,
45,
46]. However, large differences in pollutant emissions are observed among different wood fuels: wood logs produce CO emissions of about 30–100 times higher compared to both fossil fuels and chips/pellets (
Table 3), as they are generally characterized by a poor combustion (e.g., wrong regulation of excess air); a similar difference between wood and fossil fuels is observed for VOC emissions.
A further factor to be considered when evaluating wood biomass boilers is the time variation of pollutant emissions. A number of experimental studies agree that cold starts are critical for pollutant emissions [
47,
48,
49], and hence, an accurate sizing of the heat storage tank could reduce the incidence of such conditions, with noticeable gains in energy efficiency and air quality impact [
50]. This fact supports the advisability of using a separate DHW generator to avoid powering boilers for short cycles and out of the heating season. For this reason, a heat pump dedicated to the DHW production was included in all the technical solutions proposed in the economic feasibility analysis of
Section 4.
The replacement of fossil fuels with wood biomasses has a few criticalities such as feedstock availability, supply chain and air quality impact. In addition, the relatively low value of volumetric LHV, and hence, the need for large storage spaces, could be an issue for their implementation in urban areas. For this reason, heat pumps rather than wood-fueled boilers should be regarded as the real mass-scale implementable technology to increase the share of renewable heat sources and, since they have no pollutant emissions on site, they are particularly suitable for air pollution offset purposes in urban areas.
The emission factors with heat pumps are reported in
Table 4 (greenhouse gases) and
Table 5 (air pollutants) and have been calculated with the following formula:
where
is the GHG/pollutant emission factor of the Italian grid reported in Ref. [
51] and
is the seasonal performance factor of the heat pump type considered, i.e., ground-coupled heat pump (GCHP, SPF = 4), groundwater heat pump (GWHP, SPF = 4.8), and air-source heat pump for heating (Heating ASHP, SPF = 2.5) and for DHW production (DHW ASHP, SPF = 2.8). The SPF of the air-source heat pump for DHW production has been set slightly higher than for heating: indeed, although the condensation temperature for DHW is higher (DHW is stored at 55 °C, compared to low-temperature radiators which operate at 40–45 °C), this kind of heat pump also operates out of the Winter season, when the higher outdoor temperature allows higher SPF values to be achieved. Since heating ASHPs also include the DHW production, the electric consumption to cover the DHW demand was calculated considering the related SPF value (i.e., SPF = 2.8 instead of SPF = 2.5 of the heat pump in heating mode). For the other heat pump types (ground-coupled and groundwater), the SPF values were kept the same for heating and for DHW since the heat source temperature is much less variable than the air.
GHG emissions of heat pumps are not only due to the electricity used to feed them, but also to other factors among which refrigerant leaks are the most relevant, i.e., 10% of GHG emissions in a GCHP if R-134a (GWP = 1430) is used [
52]. However, as the global warming power of heat pumps is going to be dramatically reduced in the future with the F-gas EU directive [
53], the contribution of refrigerant losses to GHG emissions will move from marginal to negligible and it was therefore neglected in this study.
The reduction of CO
2 by using heat pumps ranges from 54% to 76% compared to oil boilers, depending on the heat source (air, ground, ground water). These results are consistent with other studies on heat pumps with reference to the Italian electrical grid [
52,
54,
55]. Other GHG like methane and nitrous oxide are abated by more than 90%. In addition, the GHG emission factor of electricity has declined of 32% between 2005 and 2016 [
51] (
Figure 2), thanks to the progressive phase out of liquid and solid fossil fuels in its production process, and a further reduction of GHG emissions is expected in the future, since the Italian government recently pledged to completely phase out coal as a source of energy by 2025 [
56]. When compared to fossil fuels, GHG reductions achievable by using heat pumps systems are therefore likely to increase in the foreseeable future.
Compared to oil boilers, heat pumps also show reduced global emissions of SOx (83 ÷ 91%), NOx (38 ÷ 68%), PM10 (37 ÷ 67%) and CO (26 ÷ 61%), while they increased non-methane volatile organic compounds (NMVOC) emissions (58 ÷ 205%), due to the contribution of waste combustion in the electricity mix. NMVOC emissions due to heat pump systems are, however, much lower than those caused by biomass boilers and in the order of those of LPG boilers (−19% to 55%).
5. Discussion
The technical, environmental and economic analyses reported in the previous chapter provide an information basis to support the choice of the most suitable technique to replace oil heating.
The evaluation of technical issues depends on the utilization context of the heating system since choice factors have different weights depending on the target user. For example, a number of recent studies on heat pump uptake highlighted that residential users are keener on choosing the heating technique based on perceived reliability and ease of installation rather than financial criteria [
62,
63] which, on the other hand, are the most important driver for heating choices in the commercial and industrial sectors [
13]. Literature in this field agrees on the fact that large installation costs are a strong drawback for heating technologies, even in the case of substantial reduction of the operational costs and reasonable payback times [
13,
62,
63].
Heat pumps could be the most technically suitable heating technology for most of users since they combine no need for fuel refill nor storage, no attendance, and the least safety issue; however, the difficulty to integrate them in existing buildings (i.e., fitting them into the available space and coupling them with high temperature radiators, which are still the most used terminals) is a major obstacle to their diffusion, along with noise issues for the air-source type. On the other hand, fuel refill and storage are the main drawdowns for biomass boilers, along with the time-consuming management of the system (i.e., maintenance, boiler refill etc.).
The economic evaluation of technical solutions highlights that the initial investment may be the strongest barrier for the diffusion of both wood biomass boilers and heat pumps. Payback times are made attractive (3 to 8 years) by the Italian governmental incentives for energy refurbishment. These incentives are also granted to fossil fuel boilers if they meet certain efficiency criteria [
60]: removing fossil fuel boilers from incentive schemes would further encourage the phase-out of oil at the end of the technical lifetime of the boiler.
Wood biomass boilers have lower costs of installation and shorter payback times compared to heat pumps, and this is a particularly strong driver for the choice of the heating technique.
Replacing oil boilers has multiple environmental benefits, namely i) the removal of the threat to groundwater resources represented by USTs, ii) the reduction of greenhouse gas emissions and iii) the reduction of air pollutant emissions. With the current energy mix adopted in Italy, wood biomass still is less carbon-intensive than heat pumps, although this advantage is likely to further decrease in the future due to the progressive increase of the use of renewables to produce electricity. On the other hand, as highlighted previously, boilers using wood biomass (especially wood logs) have very large particulate, CO and VOC emissions. This is a particularly important issue in Aosta Valley, which has unfavorable conditions for air quality due to the confinement effect of mountain chains. The latest yearly report on air quality by ARPA Valle d’Aosta (2018, [
64]) shows yearly average PM10 of about 20 µg/m
3 in the monitored sites in the bottom valley (Aosta and Donnas): while this value is well below the legislative threshold of 40 µg/m
3, wood biomass heating is responsible for more than 70% of these emissions. Also, wood burning has a major contribution to PAH, SO
x and CO concentrations. A further increase of the use of wood biomass should therefore be accompanied by strong policy actions to upgrade existing boilers and reduce impacts on the air quality in this region.
Considering technical issues, economic viability, GHG and air pollutant emissions, heat pumps prove to be the most suitable solution for replacing oil heating systems in Aosta Valley. Among them, air-source heat pumps have lower installation costs, but their efficiency could greatly be impaired by icing, which may occur when the evaporator temperature is below 0 °C and the dew point of air [
30]. In addition, very low air temperatures reached during winter could make the operation of air-source heat pump critical due to the reduction of the delivered power and of the SPF. These two factors should be taken into great consideration especially in the Aosta Valley, since oil boilers to be replaced are often located at high elevations with a cold climate. Ground-source heat pumps are not affected by seasonal variations of the air temperature, with a consequent efficiency gain over air-source heat pumps. In addition, most of the territory of the Aosta Valley has a high potential for heat exchange with BHEs [
35] both in the bottom valley, where the alluvial sediments have a medium-high thermal conductivity and medium-high temperature, and at higher elevations, where the high thermal conductivity of rocks compensates the negative effect of lower subsurface temperatures [
35,
36]. The Aosta Valley already has 43 BHE systems installed [
35], among which a plant operating at 2400 m a.s.l. in Cervinia [
65] which is, to our knowledge, the highest in the world for a GSHP. Also, a few alluvial plains are present (Aosta, Pont-Saint-Martin, Issogne-Verres), where 24 GWHPs have already been installed [
35]. In particular, the Aosta plain has a great potential for development of open-loop systems [
36,
66,
67].
6. Conclusions
Although declining, oil heating systems are still quite commonly used, especially in scarcely populated areas not reached by gas pipelines. Most of oil heating systems use USTs, which represent one of the most used potential groundwater contamination sources. This issue has been addressed since the early 80’s in the USA and, more recently, in Europe. In Italy, a recent study conducted on the Aosta Valley region revealed that 68 (suspect) UST leakage episodes have occurred between 1999 and 2018, of which ten were remediated. A relevant share of gas station tanks had leakage issues, while relatively few spills were found from heating oil tanks, which are much more numerous. This could be attributed to the absence of any compulsory monitoring on heating USTs, contrary to gas stations, and highlights the need to both implement periodic controls on all hydrocarbon storage tanks and to proceed to a rapid phase-out of oil heating, the impact of which is not limited to soil and groundwater. Oil is among the most carbon-intensive fuels and has a noticeable impact on air quality, especially PM10 and SOx emissions.
The techno–economic feasibility of alternatives to oil heating was therefore examined, with reference to Italian unit costs of energy and incentive schemes. Wood logs and chips boilers are the cheapest and least carbon-intensive alternatives, but their impact on air quality is to be considered critical, and their need for large storage spaces could be a strong limiting factor for large buildings plants. On the other hand, heat pumps are more expensive and have longer payback times compared to wood fuels, but they produce no emissions on site, and present dramatically reduced GHG and pollutant emissions on a global scale; in addition, they do not require fuel storage. Payback times for the replacing of oil boilers range between 6 and 16 years without considering incentives, and from about 3–8 years considering Italian current incentives for residential buildings. Including solar thermal panels to integrate the DHW production of the heat pump, as well as a photovoltaic system which could partially cover the electric demand of the heat pump, has a similar payback time (6–9 years considering incentives).
These figures confirm the economic feasibility of a rapid phase-out of oil heating systems in Aosta Valley and in other Italian regions.