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Article

Numerical Evaluation of a Novel Development Mode for Challenging Oceanic Gas Hydrates Considering Methane Leakage

1
College of Construction Engineering, Jilin University, Changchun 130026, China
2
Key Laboratory of Drilling and Exploitation Technology in Complex Conditions, Ministry of Natural Resources, Changchun 130026, China
3
Shanghai Geotechnical Engineering Detecting Centre Co., Ltd., Shanghai 200436, China
4
Sulige Gas Field Development Company, PetroChina Changqing Oilfield, Xi’an 710018, China
*
Author to whom correspondence should be addressed.
Sustainability 2022, 14(21), 14460; https://doi.org/10.3390/su142114460
Submission received: 26 August 2022 / Revised: 25 October 2022 / Accepted: 1 November 2022 / Published: 3 November 2022
(This article belongs to the Section Environmental Sustainability and Applications)

Abstract

:
The exploitation of challenging oceanic gas hydrate reservoirs with low permeability and permeable boundary layers faces the challenges of methane leakage and low production. Considering this aspect, a novel five-spot injection–production system combined with hydraulic fracturing was proposed. In particular, the potential of this development mode, including hydrate dissociation, gas production, and gas capture, was evaluated in comparison with a three-spot injection–production system. The results showed that increasing the fracture conductivity cannot prevent CH4 leakage in the three-spot, and the leakage accounted for 5.6% of the total gas production, even at the maximum fracture conductivity of 40 D·cm. Additionally, the leakage amount increased as the well spacing increased, and the leakage accounted for 36.7% of the total gas production when the well spacing was 140 m. However, the proposed development mode completely addressed CH4 leakage and significantly increased gas production. The average gas production rate reached 142 m3/d per unit length of the horizontal section, which was expected to reach the commercial threshold. The variance analysis indicated that optimal plans for the challenging hydrates in the Shenhu area were well spacing of 100–120 m and fracture conductivity greater than 20 D·cm.

1. Introduction

Natural gas hydrate (NGH) is a cage-structured crystalline solid formed by natural gas (primarily methane) and water under high pressure and low temperature [1]. The global natural gas reserves in NGH are approximately 2.5–120 × 1015 stm3, nearly twice the total carbon content of fossil fuels [2,3,4]; thus, NGH is generally considered to play a crucial role in future energy supply and climate management [5,6].
NGH is contended to be a challenging natural gas reservoir because its development faces complex phase transition, heat transfer, multiphase flow, formation deformation, and many other challenges, compared with conventional natural gas development [6,7,8,9,10]. According to the reservoir properties and occurrence environment, the challenging NGH reservoirs are characterized by low initial reservoir temperature (CH-k), lack of impermeable boundary layers (CH-b), high hydrate stability (CH-s), and low reservoir permeability (Ch-k) [11]. A vast majority of global oceanic NGH reservoirs have both low reservoir permeability and permeable boundary layers (CH-kb) [12,13], which is the main type of oceanic NGH and the primary target for commercial development.
The premise of efficient gas recovery from NGH reservoirs is to obtain a considerable hydrate decomposition rate. However, the depressurization method, which is generally considered to be the most promising, exhibits a low hydrate decomposition rate and poor gas production in CH-kb [11,14,15]. This is caused by two mechanisms: first, the low reservoir permeability and permeable boundaries inhibit pressure drop transmission and fluid flow [16,17,18]; second, insufficient reservoir sensible heat further reduced the hydrate decomposition capacity [19,20]. Therefore, exploring the efficient development mode of CH-kb has recently become an urgent topic.
Depressurization combined with thermal fluid injection could provide extra heat for hydrate dissociation, which is a promising improved scheme for NGH development [21,22]. In particular, the injection–production system with multiple wells, such as two-spot [23] and three-spot (TS) well patterns [24], significantly increases drainage area and enhances gas recovery, and has been envisaged by Japan for the commercial development of NGH [25]. However, its direct applicability in CH-kb is problematic because the gas released by hydrate thermal decomposition is difficult to pass through the inter-well hydrate undissociated zones where hydrates fill in pores and thereby form barriers to gas production. At present, using hydraulic fracturing (HF), a key stimulation technology in the commercial development of shale and tight gas, to create high conductivity artificial fractures between the injection well (welli) and production well (wellp) is a promising solution. Several numerical simulations confirmed that fractures significantly enhanced hydrate decomposition and gas production capacity, wherein hydraulic fracturing combined with a three-spot well pattern (HF + TS) was used [26,27,28]. However, existing studies have not yet focused on the risk of methane leakage in hydraulic fractured CH-kb. When the hydrate decomposition front breaks through to the permeable boundaries, the gas released by hydrate thermal decomposition escapes into boundary layers under the drive of high injection pressure [29]. This is unfavorable for gas recovery and potentially pollutes the oceanic and atmospheric environment. Recently, methane released by oceanic hydrate dissociation is considered to play an important role in the global carbon cycle, as it is leaking through permeable seabed or natural fractures [30,31,32,33,34]. Furthermore, the massive release of methane induced by NGH development in the future may affect the atmospheric CH4 budget and exacerbate the greenhouse effect [35,36,37]; therefore, there is an urgent need to evaluate the risk of methane leakage in hydraulic fractured CH-kb.
In our previous studies, we successfully addressed methane leakage in the non-fractured CH-kb using a novel five-spot well pattern, wherein two capture wells (wellc) were arranged at the boundary layers to recover the escaped gas [29]. However, because the low reservoir permeability weakens the inter-well interaction, the spacing between injection and production wells is limited to 50 m. Small space well pattern significantly increases the drilling cost, reduces economic benefits, and is not conducive to the commercial development of CH-kb. Given this, a novelty development mode combining hydraulic fracturing and the five-spot injection-production system (HF + FS) is proposed here to address the aforementioned challenges. In this study, the production potential of the proposed development mode (HF + FS) for CH-kb at the SH2 site in the Shenhu area, South China Sea, was evaluated by comparing it with HF + TS. Specifically, the impacts of fracture conductivity (Fc) and well spacing (Ws) on hydrate decomposition, gas production, methane escape, and gas recovery under the two development modes were thoroughly discussed, and ideal development plans were obtained through variance analysis (ANOVA). These findings provide valuable references for the safe and efficient development of CH-kb.

2. Modeling

2.1. Development Plan Design

The implementation of HF + FS includes the following steps: deploying the five-spot well pattern, performing hydraulic fracturing between the welli and wellp, and production with depressurization combined with thermal fluid injection.
As shown in Figure 1, all wells are horizontal and extend along the Y direction. The welli and wellc are arranged by drilling a three-branch horizontal well, wherein the middle section is used for injection, and the upper and lower sections are used for gas capture. Additionally, welli and wellp are connected through a horizontal artificial fracture created by hydraulic fracturing, and its width is 10 mm [38,39]. Due to the lack of engineering cases, the injection pressure and temperature in existing simulations are 16–22 MPa and 30–90 °C, respectively [21,22,23,24,26,27,28,29]. For comparison, we adopted the same injection–production scheme as that in our previous study [29], that is, the injection temperature and pressure were 60 °C and 16 MPa, and the bottom hole pressures of wellp, upper wellc, and lower wellc were 4, 10, and 11 MPa, respectively. Additionally, geomechanical issues are not considered in the model, because current research mainly focuses on CH4 migration and hydrate decomposition behavior under the two development modes.

2.2. Generalization of the Fracture

In this study, the fracture is generalized as porous media with high conductivity, and the multi-flow in the fracture is described as a continuous flow that follows Darcy’s law [40]. Therefore, the two-phase seepage in the matrix and fracture that considers the gravity and capillary forces can be given by Ref. [41]:
F l = k k r l μ l P l ρ l g ,
F i g = k k r g ρ g C i g μ g 1 + ω P g P g ρ g g ,
where F l and F i g are the fluxes of the liquid and gas phases, respectively, wherein l, g, and i represent the liquid phase, gas phase, and gas component, respectively; k is the absolute permeability of the matrix, m2; k r l and k r g are the relative permeabilities; μ l and μ g are the fluid viscosities, Pa·s; P l and P g are the fluid pressures, Pa; ρ l and ρ g are the fluid densities, kg/m3; g is the gravitational acceleration, m/s2; C i g is the mass friction; and ω is the Klinkenberg factor, Pa.
The k r l and k r g are expressed as [41]:
k r l = S l S i r l 1 S i r l n l ,
k r g = S g S i r g 1 S i r g n g ,
where S l and S g are the water and gas saturation, S i r l and S i r g are the irreducible saturation of liquid and gas, n l and n g are the stone indexes of liquid and gas.
The value of P l can be obtained by Ref. [42]:
P l = P g + P c ,
where P c is the capillary pressure, Pa, and is expressed as [43]:
P c = P t S l S i r l 1 S i r l 1 / ϑ 1 1 ϑ ,
where P t is threshold pressure, Pa; and ϑ is the pore structure index.

2.3. Numerical Code

To simulate the production behavior of CH-kb during depressurization and thermal fluid injection, the hydrate reaction based on thermodynamic conditions, mass conservation, energy conservation, and the flux of possible components and phases should be considered. The details of these governing equations have been given in previous studies [23,41]. Several simulators have been developed to solve these governing equations, such as Tough + Hydrate (T + H), and MH21-Hydrate [38]. T + H is developed by Lawrence Berkeley Laboratory and is popular in simulating field-scale hydrate reservoir development [41]. Three forms of heat exchange, heat conduction, heat convection, and heat radiation, are considered in T + H. Heat sources include hydrate reaction heat, phase change latent heat, the sensible heat of the reservoir itself, etc. The fluid flow in T + H follows Darcy’s law, and the convection and molecular diffusion of dissolved gases and inhibitors in water are considered. The code includes four components, including water, CH4, CH4 hydrate, and inhibitor, and four phases, including gas, liquid, ice, and hydrate. Hydrate decomposition is based on the equilibrium model or kinetic model [44]. Therefore, T + H is powerful in modeling non-isothermal hydrate decomposition, phase behavior, heat exchange, and fluid flow in hydrate reservoirs. Furthermore, the reliability of this code has been verified both at the laboratory and field scales [45,46]; thus, T + H is employed in this study.

2.4. Initial Conditions and Model Parameters

Post-drilling data at the SH2 site indicates that hydrates occur in argillaceous silt sediment below 185 mbsf (meter below seafloor), with thickness, porosity, and hydrate saturation of 0–40 m, 0.33–0.48, and 26–48%, respectively (40 m, 0.38, and 44%, respectively, in this study) [47]. Core testing revealed that the absolute permeabilities of the overburden, hydrate-bearing layer (HBL), and underburden were 10 mD [48]. Assuming that the reservoir properties are homogeneous along the Y direction, horizontal wells with long production sections are used for gas recovery and fluid injection, thus the thickness of the model in the Y direction could be set to 1 m, as shown in Figure 1.
The reservoir temperature and geothermal gradients were 14.87 °C and 0.047 °C/m, respectively [49]; therefore, the domain temperature can be obtained. The pore water is assumed to be interconnected due to the permeable boundary layers, and the pressure distribution was derived from the reservoir pressure of 14.97 MPa and pressure gradient of 0.01 MPa/m [49]. The temperature and pressure at the upper and lower boundaries of the model are considered constant because HBL is covered by seawater and underlain by enough thick sediment. Based on this, the initial equilibrium state of the reservoir is obtained (Figure 2). The values of other model parameters are listed in Table 1.

2.5. Simulation Scenarios

The fracture conductivity depends on the stress condition, proppant performance, etc., mostly in dozens of D cm [34,35,36,37]. To obtain an ideal development plan, four levels of fracture conductivity are set at 5, 10, 20, and 40 D·cm, and four levels are set at 80, 100, 120, and 140 m for well spacing, as presented in Table 2.

3. Results

3.1. Comparison of Different Development Modes

Based on the simulation results of scenarios 01, 04, and 18#, we compared the production potential of different development modes (TS, HF + TS, HF + FS) for CH-kb.

3.1.1. Spatial Evolution of the Physical Properties

1.
Reservoir temperature evolution
Figure 3 depicts the reservoir temperature evolution in different development modes. In TS, the high-temperature (higher than 30 °C) zone initially spreads circularly around welli (Figure 3a,b). At 1800 d, the thermal decomposition front advanced to the boundaries (Figure 3c), and hot water flowed into the boundary layers, resulting in non-uniform heat diffusion (Figure 3c). Compared to that in TS, the temperature evolution in HF + TS differed considerably. First, hot water mainly flowed into the fracture, resulting in a faster horizontal heat diffusion rate. Second, the hot water injection was strengthened by the fracture, leading to a larger heating area. At 360 d, the horizontal and vertical heating radii are 68 and 9 m, respectively (Figure 3d), which are higher than that at 300 d (7 m) in TS. At 600 d, the high temperature around the wellp indicates that hot water has flowed into it (Figure 3e). This is a phenomenon known as water-flooding in the petroleum industry that dramatically increases the water yield, and the time of occurrence is Tf. At 1800 d, the vertical heating radius reached 44 m (Figure 3f). In HF + FS, vertical heat diffused faster at 600 d (Figure 3h). This is because the low pressure of wellc induces more hot water to migrate vertically. Moreover, since the wellc prevents hot water from passing through the permeable boundaries, the vertical heating radius is still 20 m at 1800 d (Figure 2i). Therefore, the heating efficiency is significantly enhanced by the fracture, and hot water infiltration into the boundary layer is avoided by wellc.
2.
Reservoir pressure evolution
Figure 4 shows the reservoir pressure evolution in different development modes. In TS, two low-pressure (≤13 MPa) zones and a high-pressure (≥15 MPa) zone are formed around wellp and welli (Figure 4a–c), respectively. As the pressure transmission and fluid injection are inhibited by the low reservoir permeability, both the low- and high-pressure zones exhibit a slow diffusion rate. In HF + TS, the high-pressure zone diffuses faster along the fracture (Figure 4d). Moreover, the radius of the low-pressure zone is 48 m at 1800 d (Figure 4f), which is 2.09 times that in TS. At 1800 d, the radius of the high-pressure zone shrinks to 15 m due to the pressure relief (Figure 4f). In HF + FS, the low-pressure transmission of wellp is the same as that in HF + TS, and two low-pressure zones are also formed around wellc, which intersect with the low-pressure zones formed by wellp (Figure 4i). This indicates that the gas is well recovered, thereby relieving the reservoir pressure.
3.
Hydrate saturation evolution
Figure 5 shows the hydrate saturation evolution in different development modes. In TS, the depressurization decomposition zone and thermal decomposition zone expand circularly with a slow expansion rate (Figure 5a,b). At 1800 d, the decomposition radii of the thermal stimulation and depressurization are 13 and 21 m (Figure 5c), respectively, indicating that thermal stimulation has a better hydrate decomposition efficiency. Moreover, the gas leaking into the overburden recombines with free water and re-form hydrates (Figure 5c). In HF + TS, hydrates dissociate rapidly along the fracture, while more hydrates are generated in the overburden (Figure 5d–f). In HF + FS, the hydrate saturation evolution is similar to that in HF + TS, but no hydrate in the overburden (Figure 5g–i). Therefore, the arrangement of wellc effectively avoids the secondary formation of hydrate in the overburden.
4.
Gas saturation evolution
Figure 6 displays the gas saturation evolution in different development modes. In TS, gas saturation evolution is similar to that of hydrate saturation. The gas released by thermal stimulation accumulated at the decomposition front, and can not be produced (Figure 6a–c). Thus, there is no synergy effect between welli and wellp, and thermally decomposed gas migrates into the boundary layer (Figure 6c). In HF + TS, the gas released by thermal stimulation migrates to the wellp through the fracture (Figure 6d–f). However, more gas leaked into the boundary layers (Figure 6d–f), and the farthest vertical escape position was 46 m away from welli (Figure 6f), which was higher than that in TS (35 m). In HF + FS, the gas saturation evolution is similar to that in HF + TS, but there is no methane in the boundary layers (Figure 6g–i). Therefore, methane leakage is addressed by wellc.

3.1.2. Hydrate Dissociation Behavior

Figure 7 shows the variation of the CH4 released rate (Qr) and hydrate dissociation ratio (Dr) in different development modes, wherein Dr is the ratio between the cumulative decomposed hydrate mass (Md, kg) and the original hydrate mass (Mo, kg) in the reservoir, and is expressed as:
D r = M d M o ,
In TS, Qr is minimum and stable at approximately 50 m3/d. In HF + TS, the variation of Qr exhibited three stages. In the first stage (0–50 d), the stable state of the hydrates was broken instantaneously; thus, the initial Qr value was the highest. In the second stage (50–450 d), Qr stabilized around 200 m3/d. In the third stage (450–1800 d), Qr gradually decreases. This is caused by two factors: first, hot water bursts into the wellp along the fracture, which reduces the heating efficiency. Second, the hydrate decomposition front gradually moves away from the fracture. In HF + FS, the evolution of Qr was similar to that in HF + TS, but it was higher in the first two stages and declined faster in the third stage. This is because the presence of the wellc further strengthened the initial injection, while the subsequent water-flooded further reduced the heating efficiency. The final Dr in TS, HF + TS, and HF + FS is 31%, 93%, and 95%, respectively. This indicates that the final Dr is improved by the fracture, whereas it is barely affected by the existence of wellc.

3.1.3. Gas Production Behavior

Figure 8 displays the variation of the gas production rate (Qp) and cumulative gas production (Vp) in different development modes. In TS, Qp is minimum and totally contributed by depressurization. In HF + TS, affected by Qr, Qp also presents three stages. In the first stage (0–85 d), Qp decreases rapidly. Subsequently (85–374 d), gas migrates to wellp; thus, Qp increases and reaches its peak of 143 m3/d, which is 5.72 times that in TS. In the third stage (374–1800 d), the decrease of Qr leads to a decrease in Qp. For HF + FS, the variation of Qp is similar to that in HF + TS. Attributed to the gas recovery by wellc, the maximum Qp reaches 203 m3/d, which is 1.43 times that in HF + TS. The final Vp in HF + FS is 20.75 × 104 m3, which is 5.47 and 1.18 times of TS and HF + TS, respectively. Therefore, wellc and the fracture synergistically enhance the production.

3.1.4. Methane Leakage, Gas Capture, and Recovery Efficiency

The volume of methane leakage (Vl, m3) consists of two parts: the volume of free gas in the boundary layers ( V l f , m3) and the volume of gas trapped in re-formed hydrates ( V l h , m3), and is expressed as:
V l = V l f + V l h ,
To characterize the methane capture ability of wellc, the cumulative gas production of wellc was defined as the volume of captured gas (Vc). Recovery efficiency (Re) is defined as the ratio between cumulative gas production (Vp, m3) and the volume of gas released by hydrate decomposition (Vr, m3), and is expressed as:
R e = V p V r ,
Figure 9 depicts Vl in TS and HF + TS, Vc in HF + FS, and Re in different development modes at 1800 d. The Vl in TS and HF + TS are 15,080 and 18,389 m3, respectively, indicating that CH4 leakage is aggravated by the fracture. The Vc in HF + FS is 40,750 m3 and there is no CH4 leakage, which is consistent with the gas distribution shown in Figure 7i. Moreover, Vc is higher than Vl, indicating that wellc also enhances Vp. The Re in HF + FS is 0.93, an increase of 0.14 and 0.42 relative to TS and HF + TS, respectively. Therefore, HF + FS is a better development mode for CH-kb. It is important to note that 7% of the gas was trapped in the reservoir at 1800 d (Figure 6i). To avoid methane leakage, depressurized production can be maintained until free gas is completely produced.

3.2. The Effect of Fracture Conductivity

Scenarios 02–05, 10, 14, 18, and 22# simulated the production behavior of the two development modes (HF + TS, HF + FS) with different fracture conductivity at the well spacing of 100 m. By comparing these simulation results, the effect of fracture conductivity on production behavior is analyzed.

3.2.1. Hydrate Dissociation Behavior

Figure 10 depicts the variation of Qr in HF + TS and HF + FS at different Fc. In HF + TS, Qr varies gently around 90 m3/d when Fc is 5 D·cm, which is similar to that in TS, indicating that an Fc value of 5 D·cm is insufficient for gas migration. When Fc is 10 D·cm, Tf is 1000 d. For Fc of 20 and 40 D·cm, Tf further increases to 400 and 70 d, respectively. Additionally, Qr at 1800 d is lower when Fc ≥ 20 D·cm than that when Fc ≤10 D·cm. This is attributed to the inadequacy of remaining hydrates for the gas supply when Fc ≥ 20 D·cm. In HF + FS, Qr is higher at the early stage of production and lower at the later stage of production. The final Dr values in HF + TS are 0.51, 0.82, 0.93, and 0.96 for Fc of 5, 10, 20, and 40 D·cm, respectively (Figure 11), indicating that Dr increases as Fc increases, but the increased rate gradually decreases. The final Dr in HF + FS and HF + TS are almost the same, thus the existence of wellc has little effect on hydrate decomposition.

3.2.2. Gas Production Behavior

Figure 12 depicts the variation of Qp in HF + TS and HF + FS at different Fc. In HF + TS, Qp is lower than 50 m3/d and gradually decreases when the Fc is 5 D·cm. When Fc is 10 D·cm, Qp shows a downward trend in the first 750 d as the gas released by thermal stimulation does not migrate to the wellp. Subsequently, Qp increases and peaks at 85 m3/d. When Fc is 20 and 40 D·cm, the gas migration speed is faster; thus, Qp starts to rise at 100 and 45 d, showing peak values of 143 and 232 m3/d, respectively. In HF + FS, Qp is higher and shows a period of increase even at a low Fc value. Figure 13 shows that the final Vp values in HF + TS and HF + FS are 5.64 and 10.52, 12.93 and 17.56, 17.46 and 20.75, and 19.94 and 22.26 × 104 m3 for Fc values of 5, 10, 20, and 40 D·cm, respectively. That is, the final Vp increases with increasing Fc. Compared to HF + TS, the final Vp values in HF + FS increased by 86%, 35%, 18%, and 11%, respectively, indicating that the contribution of wellc to Vp is greater at a lower Fc value.

3.2.3. Methane Leakage, Gas Capture, and Recovery Efficiency

Figure 14 displays the variation of Vl, Vc, and Re with Fc. Notably, Vl and Vc initially increase and subsequently decrease with the increase in Fc. This can be explained by the impacts of Fc on hydrate decomposition and gas migration. In particular, increasing Fc in the range of 5–10 D·cm significantly improved the hydrate decomposition efficiency, while the gas migration capacity was insufficient, thereby exacerbating the CH4 leakage. When Fc > 20 D·cm, the improvement of the gas migration capacity is more significant than the increase in Qr; thus, more gas was produced by wellp, which decreased the Vl and Vc values. However, a leakage volume of 11,236 m3 still exists at the highest Fc, indicating that the reduction of Vl by increasing the Fc is unsatisfactory. Additionally, Vc was higher than Vl, indicating that all escaped gas was recovered by wellc.
Re increases with increasing Fc while the increased rate decreases gradually. Additionally, the Re values in HF + FS increased by 0.31, 0.21, 0.14, and 0.10 compared to those in HF + TS at Fc of 5, 10, 20, and 40 D·cm, respectively. This indicated that the contribution of wellc to Re decreases as Fc increases.

3.3. The Effect of Well Spacing

Based on the simulation results of scenarios 04, 06–08, and 17–20#, we compared the impacts of Ws on the production potential of HF + TS and HF + FS.

3.3.1. Hydrate Dissociation Behavior

Figure 15 displays the variation of Qr in HF + TS and HF + FS at different Ws. In the first 450 days, Qr decreased as Ws increased. This is attributed to the lower pressure gradient in the fracture, which reduces the fluid flow velocity. Under the same Ws, the Qr in HF + FS in the first 450 days was higher than that in HF + TS, but it dropped sharply after 450 days. Figure 16 shows that the final Dr values in HF + TS and HF + FS are 0.98 and 0.98 (Ws = 80 m), 0.93 and 0.95 (Ws = 100 m), 0.83 and 0.87 (Ws = 120 m), and 0.70 and 0.72 (Ws = 140 m), respectively. This indicated that the Dr decreases as Ws increases, whereas the existence of wellc negligibly affected the final Dr.

3.3.2. Gas Production Behavior

Figure 17 shows the variation of Qp in HF + TS and HF + FS at different Ws. When Ws is 80 m, Qp increased the fastest at the initial production stage, while it declines the most rapidly after 450 days. This is because when Ws is too small, production wells are flooded earlier and there is not enough hydrate to maintain long-term production. In HF + FS, the variation in Qp presents three phases. However, in HF + TS, the pressure gradient in the fracture was insufficient for gas migration when Ws ≥120 m, thus, Qp is lower and there is no rising phase. The final Vp values in HF + FS were 18.62, 20.75, 21.19, and 18.70 × 104 m3 at Ws values of 80, 100, 120, and 140 m, respectively. These values were 1.05, 1.19, 1.47, and 1.67 times those in HF + TS (Figure 18), indicating that the enhancement of the Vp increases as Ws increases. Additionally, the reasonable Ws should be 100–120 m because Vp under this condition is more attractive

3.3.3. Methane Leakage, Gas Capture, and Recovery Efficiency

Figure 19 depicts the variation of Vl, Vc, and Re with Ws. Notably, Vl and Vc increase with increasing Ws, indicating that the methane leakage is aggravated after increasing the Ws. Furthermore, Vc is higher than Vl even at Ws of 140 m, indicating no CH4 leakage in HF + FS. The Re values in HF + TS and HF + FS are 0.91 and 1, 0.79 and 0.93, 0.6 and 0.86, and 0.54 and 0.79 at Ws values of 80, 100, 120, and 140 m, respectively. Thus, with increasing Ws, more gas is trapped, and the contribution of wellc to Re is greater.

3.4. Variance Analysis

Analysis of variance (ANOVA) can examine the significance of the difference between the means of the factors [50]. In this study, a two-factor mixed variance model is established through the “aov” function in the “R language” (https://www.r-project.org/ (accessed on 18 June 2022)). The Vp, Vc, and Re values of 300, 600, 900, 1200, 1500, and 1800 d in HF + FS are considered evaluation indicators, and Fc and Ws are the independent variables. Thus, the significance of Fc and Ws are obtained, as shown in Figure 20. Additionally, the main effect and interaction effect of Fc and Ws were visualized, as shown in Figure 21.

3.4.1. Gas Production

As shown in Figure 20a, the significance of Fc to Vp is highest in the entire production period, and the significance level of Ws is lower and gradually decreases as the production progresses. Thus, Fc has a more significant impact on Vp. Moreover, Fc has a positive effect on Vp, whereas Ws has a negative effect on it, except at Ws of 80 m (Figure 21a–c). Thus, it is necessary to further improve Fc to overcome the negative effects of Ws to enhance production. For the current simulations, the average Qp per unit horizontal section length is higher than 100 m3/d when Fc ≥ 20 D·cm, and a horizontal section length of 600 m can reach the commercial threshold of 60,000 m3/d [25,48,49].

3.4.2. Gas Capture

Figure 20b exhibits the significance level of Fc to Vc is highest at 300 d, which subsequently becomes insignificant at 900 d. The significance level of Ws increases gradually and reaches the maximum at 1200 d. Thus, the initial and final Vc values are mainly controlled by Fc and Ws, respectively. As shown in Figure 21d, Fc has a positive effect on Vc at 300 d, indicating that the rapid decomposition of hydrate caused by the fracture increased the risk of CH4 leakage. After 900 d (Figure 21e,f), Ws exhibited a positive effect on Vc. Furthermore, the effect of Fc on Vc changed from positive to negative as the production progresses. This is because the thermal decomposition front gradually moves away from wellc, and more gas is produced when Fc is higher. Therefore, a higher Fc reduces Vc, while the necessity of deploying wellc increases under larger Ws.

3.4.3. Recovery Efficiency

As shown in Figure 20c, both Fc and Ws are insignificant to Re at the initial stage, and their significance levels were enhanced as the production progresses. Moreover, the significance level of Ws is higher than that of Fs, indicating that Ws have a more significant impact on Re. Additionally, the negative effect of Ws on Re and the positive effect of Fc on Re become increasingly clear as the production progresses (Figure 21g–i). Therefore, a higher Re can be obtained with a smaller Ws and a greater Fc, e.g., Re values were higher than 0.85 for Ws ≤ 120 m and Fc ≥ 20 D·cm.

4. Discussion

The previous study has obtained the optimal development plan of FS for non-hydraulically fractured reservoirs [29]. To evaluate the production potential of the proposed development mode in this study, the development indicators of the two are compared, as shown in Figure 22. The fracture conductivity and well spacing of the proposed development mode used for comparison here are 40 D·cm and 120 m, respectively. It can be seen that the well spacing is 50 m in a non-hydraulically fractured reservoir, which is only 41.7% of that in a hydraulically fractured reservoir. The cumulative gas production in hydraulically fractured reservoir is 243.2 × 103m3, which is 3.1 times of non-hydraulically fractured reservoir. The volume of captured gas increases from 22.9 to 43.1 × 103m3, indicating that there is a greater risk of gas escape in hydraulically fractured reservoir. Additionally, the recovery efficiency increases by 6.3% after fracturing, and the horizontal well section length required to reach the commercial gas production level is reduced from 1362 m to 444 m. Therefore, the proposed development mode is helpful to reduce drilling costs and improve the economics of challenging hydrate development.
It is important to note that the present simulations were conducted under an ideal fracture morphology as field trials of hydraulic fracturing in hydrate reservoirs have not yet been carried out. In fact, for weakly consolidated hydrate reservoirs, it is generally considered that hydraulic fracturing is challenging, and the fracture propagation patterns are complex due to the inhomogeneous hydrates in sediments [51,52,53]. Thus, it is necessary to further evaluate the effect of fracturing morphology on reservoir stimulation and methane leakage. Additionally, various injection-production well patterns, such as two-, three-, five-, seven-, and nine-spot, have been designed in conventional oil and gas development, and there is an optimal matching relationship between fracture distribution and injection–production system [54,55,56]. Unlike conventional oil and gas, the design of hydrate development mode needs to consider the methane leakage due to the lack of impermeable boundaries. Furthermore, the methane escape behavior is affected by reservoir-cover conditions and injection–production parameters. Consequently, to safely and efficiently recover methane from challenging hydrates, the applicability of different development modes to challenging hydrates with various occurrence conditions should be further explored.

5. Conclusions

In this study, we compared the production potential of the three-spot and five-spot well patterns for hydraulically fractured CH-kb reservoirs. The effects of fracture conductivity and well spacing on methane leakage and gas production were investigated. The main conclusions are as follows.
  • For the three-spot well pattern, there was considerable methane leakage into the permeable boundary layers. The leakage volume increases as the well spacing increases and reaches 46,341 m3 when the well spacing is 140 m. The impact of fracture conductivity on methane leakage shows two opposite stages: when the fracture conductivity is lower than 20 D·cm, the leakage volume increases as the fracture conductivity increases; when the fracture conductivity is higher than 20 D·cm, the opposite is true. However, enhancing the fracture conductivity can not prevent methane leakage, as a leakage volume of 11,236 m3 was observed at the greatest fracture conductivity of 40 D·cm.
  • The proposed five-spot well pattern combined with hydraulic fracturing could realize the safe development of CH-kb under a large well spacing. Even at the well spacing of 140 m, there is still no methane leakage. Additionally, increasing the well spacing increased the risk of methane leakage. Consequently, deploying capture wells is crucial for expanding safe well spacing.
  • Compared with the three-spot, the five-spot further increases the gas production and recovery and is expected to meet the commercial production threshold of hydrates. In the current simulations, the five-spot maximizes total gas production and recovery efficiency by 87 and 31%, respectively, compared to the three-spot. The average gas production rate reached 142 m3/d per unit horizontal section length, and a horizontal section length of 425 m was estimated to meet the commercial threshold.
  • The development mode of hydraulic fracturing combined with the five-spot well pattern enhances the production potential of CH-kb while addressing methane leakage, which is safe and efficient for the development of low-permeable hydrate reservoirs with permeable boundary layers. In particular, a comprehensive analysis of gas production, methane capture, and gas recovery indicates that the CH-kb hydrate reservoir at the SH2 site in the Shenhu area is suitable for a well spacing of 100–120 m and fracture conductivity greater than 20 D·cm.

Author Contributions

Conceptualization, S.N. and C.C.; methodology, S.N. and M.C.; software, S.N. and M.C.; validation, M.C. and J.S.; formal analysis, S.N. and M.C.; investigation, J.S.; resources, C.C.; data curation, J.S. and Y.W.; writing—original draft preparation, S.N.; writing—review and editing, S.N.; visualization, Y.W. and Y.M.; supervision, C.C.; project administration, C.C.; funding acquisition, C.C. All authors have read and agreed to the published version of the manuscript.

Funding

This research was funded by National Natural Science Foundation of China, grant number 41672361.

Institutional Review Board Statement

Not applicable.

Informed Consent Statement

Not applicable.

Data Availability Statement

The data presented in this study are available on request from the corresponding author.

Conflicts of Interest

The authors declare no conflict of interest.

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Figure 1. (a) FS under the 3D view; (b) HF + FS and (c) HF + TS under the cross-sectional view of x-z.
Figure 1. (a) FS under the 3D view; (b) HF + FS and (c) HF + TS under the cross-sectional view of x-z.
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Figure 2. The initial equilibrium of the reservoir, including reservoir temperature (a), pressure (b), and hydrate distribution (c).
Figure 2. The initial equilibrium of the reservoir, including reservoir temperature (a), pressure (b), and hydrate distribution (c).
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Figure 3. Reservoir temperature evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d, where “d” means “days”, and the fracture is located at Z = 50 m in subgraph (di).
Figure 3. Reservoir temperature evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d, where “d” means “days”, and the fracture is located at Z = 50 m in subgraph (di).
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Figure 4. Reservoir pressure evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d. The fracture is located at Z = 50 m in subgraph (di).
Figure 4. Reservoir pressure evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d. The fracture is located at Z = 50 m in subgraph (di).
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Figure 5. Hydrate saturation evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d. The fracture is located at Z = 50 m in subgraph (di).
Figure 5. Hydrate saturation evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d. The fracture is located at Z = 50 m in subgraph (di).
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Figure 6. Gas saturation evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d. The fracture is located at Z = 50 m in subgraph (di).
Figure 6. Gas saturation evolution: in TS at (a) 300, (b) 600, and (c) 1800 d; in HF + TS at (d) 300, (e) 600, and (f) 1800 d; and in HF + FS at (g) 300, (h) 600, and (i) 1800 d. The fracture is located at Z = 50 m in subgraph (di).
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Figure 7. Qr and Dr variation in different development modes.
Figure 7. Qr and Dr variation in different development modes.
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Figure 8. Qp and Vp variation in different development modes.
Figure 8. Qp and Vp variation in different development modes.
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Figure 9. Vl in TS and HF + TS, Vc in HF + FS, and Re in the different development modes.
Figure 9. Vl in TS and HF + TS, Vc in HF + FS, and Re in the different development modes.
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Figure 10. The variation of Qr in HF + TS and HF + FS at different Fc.
Figure 10. The variation of Qr in HF + TS and HF + FS at different Fc.
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Figure 11. The variation of Dr in HF + TS and HF + FS at different Fc.
Figure 11. The variation of Dr in HF + TS and HF + FS at different Fc.
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Figure 12. The variation of Qp in HF + TS and HF + FS at different Fc.
Figure 12. The variation of Qp in HF + TS and HF + FS at different Fc.
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Figure 13. The variation of Vp in HF + TS and HF + FS at different Fc.
Figure 13. The variation of Vp in HF + TS and HF + FS at different Fc.
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Figure 14. The variation of Vl, Vc, and Re with Fc.
Figure 14. The variation of Vl, Vc, and Re with Fc.
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Figure 15. The variation of Qr in HF + TS and HF + FS at different Ws.
Figure 15. The variation of Qr in HF + TS and HF + FS at different Ws.
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Figure 16. The variation of Dr in HF + TS and HF + FS at different Ws.
Figure 16. The variation of Dr in HF + TS and HF + FS at different Ws.
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Figure 17. The variation of Qp in HF + TS and HF + FS at different Ws.
Figure 17. The variation of Qp in HF + TS and HF + FS at different Ws.
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Figure 18. The variation of Vp in HF + TS and HF + FS at different Ws.
Figure 18. The variation of Vp in HF + TS and HF + FS at different Ws.
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Figure 19. The variation of Vl, Vc, and Re with Ws.
Figure 19. The variation of Vl, Vc, and Re with Ws.
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Figure 20. The evolution of significance levels of Ws and Fc for (a) Vp, (b) Vc, and (c) Re. Significance levels and their codes: most ‘***’; moderate ‘**’; significant ‘*’; insignificant ‘_’ and ‘ ’.
Figure 20. The evolution of significance levels of Ws and Fc for (a) Vp, (b) Vc, and (c) Re. Significance levels and their codes: most ‘***’; moderate ‘**’; significant ‘*’; insignificant ‘_’ and ‘ ’.
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Figure 21. Main effect and interaction effect of Ws and Fc: to Vp at (a) 300, (b) 900, and (c) 1800 d; to Vc at (d) 300, (e) 900, and (f) 1800 d; and to Re at (g) 300, (h) 900, and (i) 1800 d. In each subgraph, the up-left and down-right describe the interaction effect, and the up-right and the down-left describe the main effect.
Figure 21. Main effect and interaction effect of Ws and Fc: to Vp at (a) 300, (b) 900, and (c) 1800 d; to Vc at (d) 300, (e) 900, and (f) 1800 d; and to Re at (g) 300, (h) 900, and (i) 1800 d. In each subgraph, the up-left and down-right describe the interaction effect, and the up-right and the down-left describe the main effect.
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Figure 22. Comparison of development indicators between the non hydraulically fractured reservoir and hydraulically fractured reservoir using FS.
Figure 22. Comparison of development indicators between the non hydraulically fractured reservoir and hydraulically fractured reservoir using FS.
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Table 1. Model parameters.
Table 1. Model parameters.
ParametersValue
Formation thickness (Overlayer, HBL, and underlayer)30, 40, 30 m [26]
Intrinsic permeability of wells1 × 10−9 m2 (=1000 D) [11]
Intrinsic porosity of wells1 [11]
Initial water saturation (Overlayer, HBL, and underlayer)1, 0.56, 1
Porewater salinity (Overlayer, HBL, and underlayer)0.03
Gas compositionCH4 100%
Dry thermal conductivity (All deposits)1 W/m/K
Wet thermal conductivity (All deposits)3.10 W/m/K
Grain density (All deposits)2600 kg/m3
Grain-specific heat (All deposits)1000 J·K/kg
Threshold pressure P t 1 × 105 Pa [27]
pore structure index ϑ 0.45
Index for liquid phase n l 3.50
Index for gas phase n g 3.50
Irreducible aqueous saturation S i r l 0.30
Irreducible gas saturation S i r g 0.03
Table 2. Simulation scheme.
Table 2. Simulation scheme.
Scenario
Number
Development
Mode
Ws (m)Fc (D·cm)Scenario
Number
Development
Mode
Ws (m)Fc (D·cm)
01#TS100_13#HF + FS8010
02#HF + TS100514#HF + FS10010
03#HF + TS1001015#HF + FS12010
04#HF + TS1002016#HF + FS14010
05#HF + TS1004017#HF + FS8020
06#HF + TS802018#HF + FS10020
07#HF + TS1202019#HF + FS12020
08#HF + TS1402020#HF + FS14020
09#HF + FS80521#HF + FS8040
10#HF + FS100522#HF + FS10040
11#HF + FS120523#HF + FS12040
12#HF + FS140524#HF + FS14040
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Nie, S.; Chen, C.; Chen, M.; Song, J.; Wang, Y.; Ma, Y. Numerical Evaluation of a Novel Development Mode for Challenging Oceanic Gas Hydrates Considering Methane Leakage. Sustainability 2022, 14, 14460. https://doi.org/10.3390/su142114460

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Nie S, Chen C, Chen M, Song J, Wang Y, Ma Y. Numerical Evaluation of a Novel Development Mode for Challenging Oceanic Gas Hydrates Considering Methane Leakage. Sustainability. 2022; 14(21):14460. https://doi.org/10.3390/su142114460

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Nie, Shuaishuai, Chen Chen, Min Chen, Jian Song, Yafei Wang, and Yingrui Ma. 2022. "Numerical Evaluation of a Novel Development Mode for Challenging Oceanic Gas Hydrates Considering Methane Leakage" Sustainability 14, no. 21: 14460. https://doi.org/10.3390/su142114460

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