Research Progress of Organic Corrosion Inhibitors in Metal Corrosion Protection
Abstract
:1. Introduction
2. Classification of OCIs
2.1. Alkyl Chain CIs
No. | Name | Molecular Structure | Metal/Corrosive Medium | Inhibitor Type/Adsorption Isotherm | Ref. |
---|---|---|---|---|---|
1 | Cetrimonium 4 hydroxy cinnamate (CTA-4OHcinn) | Aluminum/0.01 M NaCl solution with 6.5% ethanol | Mixed type/- | [14] | |
2 | Cetrimonium 4 ethoxy cinnamate (CTA-4EtOcin) | ||||
3 | Bis[2-hydroxy-3-(dodecyldimethylammonio) propyl]-isopropylamine dichloride | 2024 Al-Cu-Mg alloy/1 M HCl | Mixed type/Langmuir | [18] | |
4 | Bis[2-amido-3-(dodecyldimethylammonium) propyl]-propylamine dichloride | 2024 Al-Cu-Mg alloy/1 M HCl | Mixed type/Langmuir | [19] | |
5 | Hexanediyl-1,6-bis-(diethyl alkyl ammonium bromide) (CmC6Cm(Et)·2Br (m = 10, 12, 14, 16)) | Aluminum/1 M HCl | -/Langmuir | [20] | |
6 | 1,3-butan-bis-(dimethyl dodecyl ammonium bromide) | Mild Steel/1 M HCl | -/- | [21] | |
7 | Decyltriphenylphosphonium bromide | Mild Steel/0.5 M H2SO4 | Mixed type/Langmuir | [22] | |
8 | Methylamine-N,N-bis(methylenephosphonate) | C1010 carbon steel/3.5% NaCl solution (pH = 3) | Mixed type/Langmuir | [23] | |
9 | Ehtylamine-N,N-bis(methylenephosphonate) | ||||
10 | Butylamine-N,N-bis(methylenephosphonate) | ||||
11 | Hexylamine-N,N-bis(methylenephosphonate) | ||||
12 | Octylamine-N,N-bis(methylenephosphonate) | ||||
13 | Dodecylamine-N,N-bis(methylenephosphonate) | ||||
14 | 1,4-bis(dodecy dipropyl ammonium bromide)-butane | Copper/3.5% NaCl | mixed type/Langmuir | [24] |
2.2. Imidazole and Its Derivatives
No. | Name | Molecular Structure | Metal/Corrosive Medium | Inhibitor Type/Adsorption Isotherm | Ref. |
---|---|---|---|---|---|
1 | Dissymmetric bis-quaternary ammonium salt (DBAS) | Q235 steel/2% NaCl solution saturated with CO2 | Mixed type/- | [30] | |
2 | sodium 2-(1Himidazol-1-yl)-4-methylpentanoate (IZS-L) | Mild steel/Artificial seawater | Mixed type/Langmuir | [31] | |
3 | sodium 2-(1H-imidazol-1-yl)-3-phenyl propanoate (IZS-P) | ||||
4 | sodium 2-(1H-imidazol-1-yl)-4-(methylthio)butanoate (IZS-M) | ||||
5 | Lauric acid/Myristic acid/Palmitic acid/Stearic acid based cationic Gemini imidazoline surfactants | X70 carbon steel/3.5% M NaCl solution | Mixed type/- | [32] | |
6 | 1-hexyl-5-methyl-1H-benzo[d][1,2,3]triazlol-1-ium bromide (HBT) | Copper electrodes/seawater | Mixed type/Langmuir | [33] | |
7 | 1-dodecyl-5-methyl-1H-benzo[d][1,2,3]triazlol-1-ium bromide (DBT) | ||||
8 | 1-octadecyl-5-methyl-1H-benzo[d][1,2,3]triazlol-1-ium bromide (OBT) | ||||
9 | 1-(2-aminobutyl)-2-ethyl]-1,3-diazacyclopenta-2,4-diene ionic liquid | API 5L-X52 steel/3% of NaCl saturated with CO2 | Mixed type/Langmuir | [34] | |
10 | (E)-2-styryl-1H-benzo[d]imidazole (STBim) | carbon steel/15% HCl | Mixed type/Langmuir | [35] |
2.3. Pyridine and Its Derivatives CIs
No. | Name | Molecular Structure | Metal/Corrosive Medium | Inhibitor Type/Adsorption Isotherm | Ref. |
---|---|---|---|---|---|
1 | Tetradecylpyridinium bromide | Aluminum/1.0 M HCl | Cathodic/Langmuir | [38] | |
2 | Hexadecylpyridinium Bromide (HPyBr) | Mild steel/0.5 M H2SO4 | Mixed type/Langmuir | [39] | |
3 | Hexadecylpyridinium Chloride (HPyCl) | ||||
4 | 2-amino-6-(3,4-dimethoxyphenyl)-4-phenylnicotinonitrile | Carbon steel/6 M H2SO4 | Mixed type/Langmuir | [40] | |
5 | 2-amino-4-(3,4-dimethoxyphenyl)-6-phenylnicotinonitrile | ||||
6 | N-alkyl-4-(4-hydroxybut-2-ynyl) pyridinium bromides | X70 steel/5 M HCl | Mixed type/Langmuir | [41] | |
7 | 4-(4-Methoyphenyl) 3,5-dimethyl-1,4,7,8-tetrahydrodipyrazolopyridine) | Mild steel/1 M HCl | Mixed type/Langmuir | ||
8 | 3,5dimethyl-4-phenyl-1,4,7,8-tetrahydrodipyrazolopyridine | [42] | |||
9 | 3,5-dimethyl-4-(3-nitrophenyl)-1,4,7,8-tetrahyddrodipyrazolopyridine) | ||||
10 | 2-phenyl-5-(pyridin-3-yl)-1,3,4-oxadiazole (POX) | Mild steel/1 M HCl | Mixed type/Langmuir | [43] | |
11 | 2-(4-methoxyphenyl)-5-(pyridin-3-yl)-1,3,4-oxadiazole (4-PMOX) | ||||
12 | 2-Amino-4-(4-methoxyphenyl)-6-phenylnicotinonitrile (AMP) | N80 steel/15% HCl | Mixed type/Langmuir | [44] | |
13 | 2-Amino-6-(2,4-dihydroxyphenyl)-4-(4-methoxyphenyl)nicotinonitrile (ADP) |
2.4. Quinoline and Its Derivatives
No. | Name | Molecular Structure | Metal/Corrosive Medium | Inhibitor Type/Adsorption Isotherm | Ref. |
---|---|---|---|---|---|
1 | 8-hydroxyquinoline | X60 steel/15% HCl | Mixed type/- | [45] | |
2 | 2-1-methyl-quinoline-nonyl | X80 pipeline steel/NACE solution (CO2 environment) | Cathodic/- | [46] | |
3 | 2-chloro-3-formyl quinoline | Mild steel/1 M HCl | Mixed type/Freundlich | [47] | |
4 | 8-hydroxyquinoline grafted triazole derivatives | Carbon steel/0.5 M H2SO4 | Mixed type/Langmuir | [48] | |
5 | 4-chloro,8-(trifluoromethyl)quinoline (CTQ) | Mild steel/1 M HCl | Mixed type/Langmuir | [49] | |
6 | 2-(quinolin-2-yl)quinazolin-4(3H)-one | Q235 steel/1 M HCl | Mixed type/Langmuir | [50] | |
7 | 3-((8-hydroxyquinolin-5-yl)-methyl)-2-phenylquinazolin-4(3H)-one (HQ-ZH) | Mild steel/1 M HCl | Mixed type/Langmuir | [51] | |
8 | 2-(2-hydroxyphenyl)-3-((8-hydroxyquinolin-5-yl)-methyl)-quinazolin-4(3H)-one (HQZOH) | ||||
9 | 3-((8-hydroxyquinliene-5-yl)-2-(4-nitrophenyl)-quinazolin-4(3H)-one (HQ-ZNO2) |
2.5. Natural Products
Name | Molecular Structure | Metal/Corrosive Medium | Inhibitor Type/Adsorption Isotherm | Ref. |
---|---|---|---|---|
Rhamnolipid-1 | X70 carbon steel/Simulated seawater | Mixed type/- | [3] | |
Rhamnolipid-2 | ||||
Caffeic acid (Caf) | Mg alloy AZ91D/3.5 wt% NaCl | Mixed type/- | [52] | |
Chichoric acid (Chi) | ||||
2-(3,4-Dihydroxy-phenyl)-3,5,7-trihydroxy-chromen-4-one (DPT) | Q235 steel/1M HCl | Mixed type/Langmuir | [53] | |
6,7-Dimethoxy-2-(4-methoxy-phenyl)-chromen-4-one (DMP) | ||||
3-(3-Hydroxy-4-methoxy-phenyl)-6,8-dimethoxy-1,2,3,4-tetrahydro-naphthalen-2-ol (HMP) | ||||
5,7-Dihydroxy-2-(4-hydroxy-phenyl)-3-methyl-chroman-4-one (DHP) | ||||
Phenyl alanine | Mg-Al-Zn alloy/chloride-free neutral aqueous buffer solution | Anodic/Langmuir | [55] | |
A representation of Elaeis guineensis oil | AA6063 Al-Mg-Si alloy/3.5% NaCl | Mixed type/Langmuir | [56] | |
Chlorogenic acid | A36 mild steel/1M HCl | Mixed type/Langmuir | [58] | |
Vanillic acid | ||||
Scopoletin | ||||
Trans-1,4-polyisoprene (TPI) | Q235 steel/3.5 wt% NaCl | -/- | [59] | |
Poly(citric acid-curcumin) (Cur-PCA) | 3105 aluminum alloy/1 mol/L HCl prepared using 3.5% NaCl solution | Mixed type/El-Awady | [60] | |
Bisabolol | Aluminum/3.5 wt% NaCl | Mixed type/Freundlich | [61] | |
Camphene | ||||
Cineole |
3. Mechanism of OCIs
4. Conclusions
Author Contributions
Funding
Data Availability Statement
Conflicts of Interest
References
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Zhao, W.; Li, F.; Lv, X.; Chang, J.; Shen, S.; Dai, P.; Xia, Y.; Cao, Z. Research Progress of Organic Corrosion Inhibitors in Metal Corrosion Protection. Crystals 2023, 13, 1329. https://doi.org/10.3390/cryst13091329
Zhao W, Li F, Lv X, Chang J, Shen S, Dai P, Xia Y, Cao Z. Research Progress of Organic Corrosion Inhibitors in Metal Corrosion Protection. Crystals. 2023; 13(9):1329. https://doi.org/10.3390/cryst13091329
Chicago/Turabian StyleZhao, Wenwen, Feixiang Li, Xianghong Lv, Jianxiu Chang, Sicong Shen, Pan Dai, Yuan Xia, and Zhongyue Cao. 2023. "Research Progress of Organic Corrosion Inhibitors in Metal Corrosion Protection" Crystals 13, no. 9: 1329. https://doi.org/10.3390/cryst13091329
APA StyleZhao, W., Li, F., Lv, X., Chang, J., Shen, S., Dai, P., Xia, Y., & Cao, Z. (2023). Research Progress of Organic Corrosion Inhibitors in Metal Corrosion Protection. Crystals, 13(9), 1329. https://doi.org/10.3390/cryst13091329