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Article

Diatomite and Glucose Bioresources Jointly Synthesizing Anode/Cathode Materials for Lithium-Ion Batteries

1
Graduate School of Life Science and Systems Engineering, Kyushu Institute of Technology, 2-4 Hibikino, Wakamatsu, Kitakyushu 808-0196, Japan
2
Medical Engineering and Technology Research Center, School of Radiology, Shandong First Medical University & Shandong Academy of Medical Sciences, Taian 271000, China
3
College of Materials and Chemistry, China Jiliang University, Hangzhou 310018, China
4
School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China
*
Authors to whom correspondence should be addressed.
Coatings 2023, 13(1), 146; https://doi.org/10.3390/coatings13010146
Submission received: 30 November 2022 / Revised: 3 January 2023 / Accepted: 7 January 2023 / Published: 11 January 2023

Abstract

Large-scale popularization and application make the role of lithium-ion batteries increasingly prominent and the requirements for energy density have increased significantly. The silicon-based material has ultra-high specific capacity, which is expected in the construction of next-generation high specific-energy batteries. In order to improve conductivity and maintain structural stability of the silicon anode in application, and further improve the energy density of the lithium-ion battery, we designed and synthesized carbon-coated porous silicon structures using diatomite and polysaccharides as raw materials. The electrode materials constructed of diatomite exhibit porous structures, which can provide fast transport channels for lithium ions, and effectively release the stress caused by volume expansion during cycling. At the same time, the electrical conductivity of the materials has been significantly improved by compounding with biomass carbon, so the batteries exhibit stable electrochemical performance. We systematically studied the effect of different contents of biomass carbon on the Li2MnSiO4/C cathode, and the results showed that the carbon content of 20% exhibited the best electrochemical performance. At a current density of 0.05C, the capacity close to 150 mAh g−1 can be obtained after 50 cycles, which is more than three times that of without biomass carbon. The silicon-based anode composited with biomass carbon also showed excellent cycle stability; it could still have a specific capacity of 1063 mAh g−1 after 100 cycles at the current density of 0.1 A g−1. This study sheds light on a way of synthesizing high specific-capacity electrode materials of the lithium-ion battery from natural raw materials.
Keywords: diatomite; lithium-ion batteries; Li2MnSiO4/C cathode; natural raw materials diatomite; lithium-ion batteries; Li2MnSiO4/C cathode; natural raw materials

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MDPI and ACS Style

Chen, Y.; Jiang, B.; Zhao, Y.; Liu, H.; Ma, T. Diatomite and Glucose Bioresources Jointly Synthesizing Anode/Cathode Materials for Lithium-Ion Batteries. Coatings 2023, 13, 146. https://doi.org/10.3390/coatings13010146

AMA Style

Chen Y, Jiang B, Zhao Y, Liu H, Ma T. Diatomite and Glucose Bioresources Jointly Synthesizing Anode/Cathode Materials for Lithium-Ion Batteries. Coatings. 2023; 13(1):146. https://doi.org/10.3390/coatings13010146

Chicago/Turabian Style

Chen, Yun, Bo Jiang, Yue Zhao, Hongbin Liu, and Tingli Ma. 2023. "Diatomite and Glucose Bioresources Jointly Synthesizing Anode/Cathode Materials for Lithium-Ion Batteries" Coatings 13, no. 1: 146. https://doi.org/10.3390/coatings13010146

APA Style

Chen, Y., Jiang, B., Zhao, Y., Liu, H., & Ma, T. (2023). Diatomite and Glucose Bioresources Jointly Synthesizing Anode/Cathode Materials for Lithium-Ion Batteries. Coatings, 13(1), 146. https://doi.org/10.3390/coatings13010146

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