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Article

Numerical Investigation of Pressure Influence on the Confined Turbulent Boundary Layer Flashback Process

Lehrstuhl für Thermodynamik, Technische Universität München, 85747 Garching, Germany
*
Author to whom correspondence should be addressed.
Fluids 2019, 4(3), 146; https://doi.org/10.3390/fluids4030146
Submission received: 14 June 2019 / Revised: 26 July 2019 / Accepted: 28 July 2019 / Published: 1 August 2019
(This article belongs to the Special Issue Numerical Simulations of Turbulent Combustion)

Abstract

:
Boundary layer flashback from the combustion chamber into the premixing section is a threat associated with the premixed combustion of hydrogen-containing fuels in gas turbines. In this study, the effect of pressure on the confined flashback behaviour of hydrogen-air flames was investigated numerically. This was done by means of large eddy simulations with finite rate chemistry as well as detailed chemical kinetics and diffusion models at pressures between 0.5 bar and 3 bar. It was found that the flashback propensity increases with increasing pressure. The separation zone size and the turbulent flame speed at flashback conditions decrease with increasing pressure, which decreases flashback propensity. At the same time the quenching distance decreases with increasing pressure, which increases flashback propensity. It is not possible to predict the occurrence of boundary layer flashback based on the turbulent flame speed or the ratio of separation zone size to quenching distance alone. Instead the interaction of all effects has to be accounted for when modelling boundary layer flashback. It was further found that the pressure rise ahead of the flame cannot be approximated by one-dimensional analyses and that the assumptions of the boundary layer theory are not satisfied during confined boundary layer flashback.

1. Introduction

The combustion of hydrogen-rich fuels instead of pure hydrocarbon fuels in gas turbines is one possible measure to reduce anthropogenic CO 2 emissions in power production. Hydrogen-rich synthetic fuels can be produced by reforming or gasification of hydrocarbon fuels. The low carbon content of these synthetic fuels results in low CO 2 production during the combustion process. The CO 2 emissions that accrue during the synthesis process on the other hand can be captured and stored prior to the combustion process [1,2]. Another measure to decrease CO2 emission in power production is the exploitation of renewable energy resources. Power production from renewable resources and power demand generally show strong fluctuations. Hydrogen can be produced from the electrolysis of water in times of excess power output. By using the produced hydrogen as a fuel in gas turbines, the imbalance of power production and demand can be compensated without additional CO 2 emission [1,2].
In order to meet the strict regulations of NOx emissions, lean premixed combustion is usually applied in gas turbines [3]. By mixing fuel and oxidizer upstream of the combustion chamber, combustible fuel-air mixtures exist upstream of the combustion chamber. This allows for flame flashback into the premixing channel of the burner, which potentially causes critical damage to the premixing channel and requires engine shutdown. Boundary layer flashback (BLF) is upstream flame propagation which takes place in the low velocity region of the boundary layer. Hydrogen flames show high burning velocities and a high reactivity near walls. This makes hydrogen combustion in gas turbines prone to BLF [4].
Due to the risk associated with BLF, it is essential to be aware of the flashback limits and their influencing parameters. The influence of preheat temperature [5,6], flame confinement [7] and acoustic oscillations [8] on the flashback behaviour, for example, have been investigated experimentally. Furthermore, Daniele et al. [5] and Kalantari et al. [6] investigated the influence of pressure on the flashback limits of unconfined turbulent lean premixed flames with high hydrogen content. They observed that the flashback equivalence ratio Φ F B decreases with pressure p and follows the power law Φ F B p n . Depending on the operating conditions in the experiments, the pressure exponent n lay between 0.27 and 0.51. They concluded that this strong increase in flashback tendency with increasing pressure is mainly caused by the decrease in quenching distance. The change in turbulent flame speed with pressure on the contrary only had a minor effect on the flashback limits.
Hoferichter and Sattelmayer [8] showed that the flashback limits of unconfined flames, which are acoustically excited, approach the flashback limits of confined flames, which are not acoustically excited. The confined case of BLF is thus the limiting of both cases regarding the flashback safety of burners. Although it is of high technical relevance, the pressure influence on the flashback process of confined turbulent flames has not been investigated yet. Furthermore, only the global influence of pressure on unconfined flashback limits has been investigated so far. The influence of pressure on parameters, such as the quenching distance, had to be estimated from analytical considerations [5,6].
Hoferichter et al. [9] developed an analytical model to predict atmospheric confined boundary layer flashback limits. In their model, flashback is assumed to occur when the average flame front causes a pressure rise which is large enough to cause boundary layer separation. The adapted Stratford separation criterion [10],
Δ p m a x ρ u U F B 2 = 0.0975 2 3 ,
is applied for the prediction of boundary layer separation and the confined flashback limits. U F B is the channel centerline velocity at which boundary layer separation and flashback are expected. The pressure rise Δ p m a x ahead of the flame front is estimated from one-dimensional considerations. The conservation of mass and momentum and assuming equal pressures far upstream and downstream of the flame results in the pressure rise
Δ p m a x = ρ u S t , m a x 2 T a d T u 1 ,
which is dependent on the fresh gas density ρ u , the maximum turbulent flame speed S t , m a x and the ratio of unburnt gas temperature T u to adiabatic flame temperature T a d . The turbulent flame speed is estimated from the laminar flame speed, flame stretch and the maximum turbulent fluctuation velocity [9]. The pressure rise from Equation (2) and the Stratford separation criterion (1) lead to the flashback criterion
S t , m a x 2 U F B 2 T a d T u 1 = 0.0975 2 3 ,
or
U F B = 0.0975 1 3 S t , m a x T a d T u 1 .
This criterion implies that the flashback centerline velocity is only dependent on the maximum turbulent flame speed and the gas expansion ratio given by the temperatures T a d and T u . This contradicts the observation of Daniele et al. [5] and Kalantari et al. [6], who found that the quenching distance has a strong influence on unconfined BLF limits. Furthermore, the one-dimensional approximation of the pressure rise ahead of the flame front contradicts the findings of Eichler [11] from two-dimensional simulations of confined laminar BLF. He observed that the velocity field and the pressure rise ahead of the flame are of two-dimensional nature, which prohibits the prediction of the pressure rise based on one-dimensional considerations.
Several numerical simulations of turbulent flashback of hydrogen-rich fuels have been presented in recent years [4,12,13,14]. These simulations significantly improved the understanding of the BLF process. Endres and Sattelmayer [15] recently presented first simulations that accurately reproduced confined flashback limits of turbulent hydrogen-air flames at atmospheric pressure. They applied large eddy simulations (LES) with finite rate chemistry and a detailed species diffusion model. The study also showed that under atmospheric conditions, upstream flame propagation occurs when the flow separation zone size ahead of the propagating flame front is significantly larger than the quenching distance of the flame.
A similar LES model as previously presented for atmospheric calculations [15] is applied in the present work. This approach allows for a detailed analysis of the flashback process at different pressure levels. The comparison of the numerically obtained flashback limits at atmospheric pressure with experimental flashback limits [16] ensures that the chosen simulation approach is capable of accurately reproducing the flashback process. Flashback can then be investigated at pressures between 0.5 bar and 3 bar, where no experimental data is available. Although changing the pressure leads to altered molecular viscosities and Reynolds numbers, the atmospheric channel flow approaching the flame is left unchanged in this work. Comparing the results at different pressure levels allows for the investigation of the influence of average quantities, such as the maximum turbulent flame speed and the average flow deflection, on the flashback limits. This is followed by an analysis of the influence of local quantities, such as the local quenching distance and the local separation zone size, on the flashback process. Finally, the results are used to investigate the applicability of the one-dimensional pressure estimation (2) and the Stratford separation criterion (1) for BLF prediction.

2. Numerical Model

Despite introducing in-situ adaptive tabulation and a low-Mach number approximation in the reactive solver, the numerical model is similar to the numerical model of Endres and Sattelmayer [15]. For the sake of completeness, a shortened presentation of the numerical model will be given here. For more details on the model, the reader is referred to the article of Endres and Sattelmayer [15].
The numerical model for inert and reactive simulations is implemented in the framework of the open source computational fluid dynamics package OpenFOAM [17]. The governing equations are solved with a finite volume discretization. Derivatives in time are discretised by a second order accurate quadratic backward differencing scheme. Spatial discretization is handled by the second order accurate central differencing scheme and by a stabilised central differencing scheme [18].

2.1. Inert Simulations

An accurate inert base flow is a basic requirement for the atmospheric flashback simulations in order to precisely predict the experimental BLF limits. In the experiments, the velocity profile at the beginning of the flame stabilization section well reproduced the characteristics of a fully developed channel flow [16]. Therefore, the inert simulations also aim at accurately predicting the mean velocity profile and the velocity fluctuations of a fully developed channel flow.
The incompressible OpenFOAM solver pimpleFoam is used for the inert simulations. In this solver, the incompressible Navier-Stokes equations are solved with a segregated approach. The time step size is automatically adapted in order to keep the local non-acoustic Courant number below 0.8. The OpenFOAM version of the Smagorinsky model [15,17,19,20] is used for modelling the subgrid scale (SGS) kinematic viscosity ν S G S . The chosen model constants are equivalent to a Smagorinsky constant of c S = 0.168 and are close to the original value of c S = 0.17 proposed by Lilly [21]. The filter width Δ is approximated by the cube root of the local cell volume. Van Driest damping is applied to the filter width in order to account for low Reynolds effects near walls and to ensure a vanishing SGS viscosity at walls [22,23].
The numerical flashback results at atmospheric pressure are compared with experimental flashback results in a rectangular channel [7]. Bulk velocities U b of 10 m   s 1 , 20 m   s 1 and 30 m   s 1 are investigated. For the representation of the experimental rectangular channel geometry, the computational domain for the inert simulations is a channel with a half height of δ = 8.75   m m , a length of 6 δ and a width of 3 δ . Cyclic boundary conditions are prescribed at the front and back patches in order to obtain a quasi two-dimensional configuration. Cyclic boundary conditions are also set at the inlet and outlet patches. This allows for full development of the channel flow. In order to obtain the desired bulk velocities, an average streamwise pressure gradient is automatically prescribed along the channel. The walls are modelled as no-slip walls without applying a wall model. Therefore, small wall-normal cell sizes y 1 + < 0.8 of the cells adjacent to walls are chosen. The wall-normal cell size is gradually increased towards the channel centerline where the cell size is ten times the cell size at the wall. The resulting maximum cell sizes and cell counts in streamwise (x), wall-normal and spanwise (z) direction are given in Table 1. All cell sizes are made non-dimensional by the kinematic viscosity ν and the theoretical friction velocity calculated with the empirical correlation developed by Pope [24],
u τ , P o p e = 0.09 y δ Re 0.88 .
The kinematic viscosity was fixed to ν = 1.8 × 10 5   m 2   s 1 .
This numerical setup resulted in accurate average velocity profiles and turbulent kinetic energy profiles compared to literature DNS results [15]. It was furthermore shown by Endres and Sattelmayer [15] that the flashback limits obtained from the atmospheric reactive simulations were insensitive to changes in the domain size of the inert simulations and to changes in the resolution of the inert base flow. The time-dependent velocity profiles from the inert simulations were therefore again sampled and projected onto the inlet of the domain of the reactive simulations.
The chosen viscosity well represents the viscosity of the investigated hydrogen-air mixtures at atmospheric pressure. By changing the domain pressure to subatmospheric or elevated pressure, the kinematic viscosity of the hydrogen-air mixtures is changed. This modifies the flow Reynolds number and the channel flow characteristics. In the present work, the inert viscosity and the inert base flow are however left unchanged compared to the atmospheric calculations. The effect of pressure on the inert velocity profile is thereby eliminated and the sole effect of pressure on the combustion and flow separation properties is investigated.

2.2. Reactive Simulations

The numerical model for the reactive simulations applied by Endres and Sattelmayer [15] was proven to accurately predict the flashback behaviour of atmospheric turbulent hydrogen-air flames. However, it was later noted that despite applying a wave-transmissive boundary condition, acoustic pressure oscillations occured in the domain, which possibly influenced the results. A low Mach number approximation
ρ = p 0 R s T
is thus applied to the compressible governing equations [25]. By calculating the gas density ρ from a constant thermodynamic pressure p 0 , the specific gas constant R s and temperature T, density changes are decoupled from pressure changes and acoustic oscillations are prevented. The constant thermodynamic pressure is also used to calculate the molecular gas properties as well as the chemical reaction rates. The Navier-Stokes equations on the other hand are solved for the dynamic pressure p d . In addition, the transport equation for sensible enthalpy and the Favre-filtered transport equations
ρ ¯ Y k ˜ t + ρ ¯ u i ˜ Y k ˜ x i + j k , i ¯ x i x i ρ ¯ ν S G S Sc S G S Y k ˜ x i = ω ˙ k ¯
for the mass fractions Y k of each species k are solved in order to include chemical reactions. The SGS Schmidt number S c S G S is assumed to be unity. The Smagorinsky model is used for modelling the SGS viscosity ν S G S . The chemical reaction rate ω k is obtained from a system of chemical reactions of Arrhenius type solved by the Seulex ordinary differential equations (ODE) solver [26]. The detailed chemical kinetics mechanism of Burke et al. [27] is used for modelling the chemistry of hydrogen combustion. This mechanism consists of 9 species and 23 reactions. In order to increase the speed of the calculations compared to the calculations in Reference [15], in-situ adaptive tabulation [28,29] is applied in the present work. By storing the results of the direct solution of the chemical reaction mechanism, a look-up table is created for mapping the gas composition, pressure and temperature from the previous solver iteration to the current iteration. The number of computationally costly ODE integrations is thereby kept at a minimum. The reaction mapping is approximated linearly by a mapping gradient matrix. The maximum error of this linear approximation is set to 10 4 .
The filtered chemical reaction rate ω ˙ k ¯ of species k is assumed to be equivalent to the reaction rate directly obtained from the filtered temperature, pressure and species mass fraction distribution. This approach is usually referred to as implicit LES (ILES) [25,30] or quasi-laminar combustion model [31]. The subgrid turbulence-chemistry interaction is neglected in ILES. Therefore, it has to be ensured that the flame either has a laminar character at the subgrid scales [15,32] or that the LES cells are perfectly stirred by turbulent fluctuations [25].
Endres and Sattelmayer [15] showed that a detailed diffusion model is essential for the prediction of correct flame shapes and flashback limits. The diffusion mass flux j k , i is therefore calculated as the sum of the diffusion mass flux due to species mass fraction gradients j k , i Y and the Soret diffusion mass flux j k , i T due to temperature gradients.
j k , i = j k , i Y + j k , i T = ρ D k Y k x i D k T 1 T T x i
The mixture diffusion coefficient D k of species k is obtained from the binary diffusion coefficients D j , k of species j through species k and a gas composition dependent mixture equation [33,34]. The binary diffusion coefficients are in turn obtained from an empricial equation based on the kinetic gas theory [35,36]. The Soret diffusion coefficients D k T are calculated according to an empirical correlation [37]. The mixture thermal diffusivity α for the transport equation of sensible enthalpy is calculated from the thermal diffusivities of each species by applying a gas composition dependent mixture equation [34,38]. The species thermal diffusivities are approximated by a third degree logarithmic polynomial [15]. The polynomial coefficients are calculated beforehand by applying a least squares fit to the species thermal diffusivities obtained with Cantera [38]. The kinematic viscosity ν is obtained from the Sutherland law [39] with the Sutherland parameter A S = 1.67121   k g   m 1   s 2   K 0.5 and the Sutherland temperature T S = 170.672   K .
Hoferichter and Sattelmayer [8] showed the flashback limits of confined BLF are of high technical relevance for unconfined flames with acoustic excitation. The present simulations therefore aim at reproducing the confined flashback limits presented by Eichler et al. [16]. As in the atmospheric calculations of Endres and Sattelmayer [15], the computational domain depicted in Figure 1 represents a rectangular channel with a length of 6 δ and a width of 3 δ for U b = 10   m   s 1 and a width of 2.23 δ for U b = 20   m   s 1 and U b = 30   m   s 1 . The time dependent velocity profile is prescribed at the inlet and a constant dynamic pressure is prescribed at the outlet. In order to obtain the flow characteristics of an infinitely wide channel, cyclic boundary conditions are prescribed at the front and back patch. The lower wall is modelled as an isothermal wall at 293.15 K up to x 3 δ and as an adiabatic wall for x > 3 δ , in order to represent the cooled steel walls followed by a ceramic tile for flame stabilization in the experiments [16]. The base mesh from the inert calculations is left unchanged. In order to well resolve the stable and propagating flame front, the mesh is automatically refined by adaptive mesh refinement. The hexahedral cells are split in each spatial direction resulting in eight smaller hexahedral cells. This cell split is applied to a cell if the change Δ H 2 = Y H 2 V c 1 / 3 of hydrogen mass fraction in one cell of volume V c is larger than 10% of the unburnt hydrogen mass fraction. The maximum number of splits per cell is limited to one or two splits in the investigated cases.
The approach for obtaining flashback limits is similar to the atmospheric calculations in Reference [15]. A constant velocity is assumed in the channel at the beginning of the calculations. The species mass fractions of hydrogen, oxygen and nitrogen are set to an equivalence ratio at which no flashback is expected. The flame front is initialized by setting the temperature and species mass fractions in a rectangular box with a height of 1 m m to the burnt gas values. As soon as the velocity fluctuations prescribed at the inlet reach the flame front, the flame front is wrinkled and stabilizes at the leading edge of the adiabatic wall. When the flame wrinkling is fully developed, the equivalence ratio Φ at the inlet is increased by a small step of 0.02 to 0.05. This is repeated until the flame front propagates upstream along the isothermal wall without being completely washed out. This equivalence ratio is defined as the flashback equivalence ratio Φ F B .

2.3. Les Regimes for Hydrogen Combustion

The requirement for the applicability of the ILES approach is that the SGS flame either has a laminar structure, or that the reaction and mixing processes are not influenced by SGS fluctuations. The LES combustion regimes developed by Pitsch and Duchamp de Lageneste [32] can be used to point out the laminar character of the SGS flame structure in the presented simulations. In the derivation of the original LES combustion regime diagram, Pitsch and Duchamp de Lageneste assume that the diffusivity D of the gas mixture equals the kinematic viscosity ν . This assumption is however invalid for hydrogen combustion. In the following, the LES combustion regimes are therefore analyzed for the general case, where D ν .
The combustion regimes are defined by the Karlovitz number K a and the ratio of the LES filter width Δ to the laminar flame length scale l f = D / s l , 0 [40], where s l , 0 is the laminar flame speed. The Karlovitz number is defined as the ratio of the flame time scale t f = l f 2 / D to the time scale t η = η 2 / ν of the Kolmogorov eddies. The Kolmogorov length scale η = ν 3 / ϵ 0.25 can be approximated by the kinematic viscosity ν and the dissipation rate ϵ = c ϵ k S G S 1.5 Δ 1 . Here, k S G S is the SGS turbulent kinetic energy and c ϵ is a model constant. This results in the diffusivity and viscosity dependent Karlovitz number calculated from LES quantities,
K a = c ϵ k S G S 1 . 5 D 2 Δ s l , 0 4 ν .
The wrinkled flamelet regime and the corrugated flamelet regime are separated by the Gibson length scale. The Gibson length scale is defined by the equality of the laminar flame speed and the SGS velocity fluctuation k S G S . In the wrinkled flamelet regime, the SGS velocity fluctuation is smaller or equal to the laminar flame speed. According to Peters [40], fluctuations with a velocity smaller than the laminar flame speed do not wrinkle the flame front. The SGS flame therefore has a laminar character in the wrinkled flamelet regime while it has a non-laminar character in the corrugated flamelet regime. With the assumption that D = ν , the condition s l , 0 = k S G S for the Gibson length scale leads to a mixture independent relation between the Karlovitz number and Δ / l f . For hydrogen however, D ν and the condition for the Gibson length scale lead to
Δ l f = K a 2 D ν ,
when assuming c ϵ 1 . This takes the viscosity and diffusivity of the gas mixture into account when evaluating the SGS combustion regime. This results in the different lines between the wrinkled flamelet and corrugated flamelet regime in Figure 2 and Figure 3.
Figure 2 and Figure 3 show the SGS combustion regimes at different pressure levels for the highest corresponding equivalence ratios investigated in the current work. Each data point represents one cell along the y-axis of the unrefined mesh. The velocity fluctuations are obtained from the inert calculations and the laminar flame speed is calculated from the correlation developed by Böck [41] for atmospheric flames. The influence of pressure on the laminar flame speed is taken into account by the proportionality s l , 0 p m . The pressure exponent m is obtained from the results of Bradley et al. [42]. Following Bechtold and Matalon [43], the Lewis number L e of gas mixtures can be obtained from the species diffusivities and a mixture and flame temperature dependent weight function.
L e = α D = 1 + α O 2 D O 2 1 + α H 2 D H 2 1 1 + Z e 1 Φ 1 2 + Z e 1 Φ 1
For this calculation, the species diffusivities D H 2 = 7.29 × 10 5   m 2   s 1 and D O 2 = 1.88 × 10 5   m 2   s 1 and species thermal diffusivities α H 2 = α O 2 = 2.25 × 10 5   m 2   s 1 are assumed to be mixture independent. The Zeldovich number
Z e = E T a d T u R T a d 2
is calculated from the adiabatic flame temperature T a d , the unburnt gas temperature T u = 293.15 K the constant activation energy E = 20 kcal mol 1 = 8.368 × 10 4   k J   kmol 1 and the universal gas constant R. With the resulting Lewis numbers and the actual mixture thermal diffusivities α obtained from Cantera, the mixture diffusivities D can be computed using the Lewis number definition L e = α / D . The input and resulting parameters for the diffusivity calculation for all cases are listed in Table A1 in Appendix A.
It is evident from Figure 2 that all cases at U b = 10   m   s 1 lie within the laminar flamelet and the DNS regimes. In the laminar flamelet regime the filter width Δ is smaller than the Kolmogorov length scale η . The SGS flow is therefore approximately laminar and no SGS turbulence fluctuations will have an influence on the combustion process [32]. At U b = 20   m   s 1 and p = 1 bar, all cells also lie within the laminar flamelet and DNS regimes. At U b = 20   m   s 1 and p = 2 bar as well as at U b = 30   m   s 1 and p = 1 bar, some cells lie within the thin reaction zones regime. In this regime, the SGS turbulent eddies are small enough to penetrate the flame preheat zone and affect the mixing processes in the preheat zone [32]. The cells in the thin reaction zone regime should therefore not be modeled with the ILES combustion model. This has to be taken into account when analyzing the results of the two cases. Especially for U b = 30   m   s 1 and p = 1   bar , the majority of the cells however lie within the laminar flamelet and DNS regimes and show a laminar SGS flame structure. In order to also investigate the pressure influence for different bulk velocities, the U b = 20   m   s 1 case at p = 2   bar and the U b = 30   m   s 1 case at p = 1   bar are included here nevertheless. For all other cases the ILES approach is valid and the results are expected to deliver accurate results.

3. Results

The presented approach leads to flashback limits at different pressure levels with the unaltered inert base flow. In the following, the pressure influence on the flashback limits is investigated. This is followed by an analysis of the macroscopic flame structure and the flame resolution resulting from the macroscopic flame structure. Finally, the influence of pressure on the combustion and flow separation characteristics is investigated on the basis of average pressure and velocity fields and on the basis of local flame quenching and boundary layer separation.

3.1. Pressure Influence on Confined Flashback Limits

At atmospheric pressure, confined boundary layer flashback is modeled at bulk velocitites of 10   m   s 1 , 20   m   s 1 and 30   m   s 1 . It was shown by Endres and Sattelmayer [15] that one cell split is sufficient to resolve the flame front at U b = 10   m   s 1 and U b = 20   m   s 1 . Applying two cell splits by the adaptive mesh refinement algorithm at U b = 20   m   s 1 and U b = 30   m   s 1 is furthermore prohibitive due to the associated computational costs. The adaptive mesh refinement is therefore set to a maximum of one cell split for the atmospheric simulations. With this refinement strategy, the flame is stable up to equivalence ratios of 0.38 , 0.55 and 0.7 for bulk velocities of 10   m   s 1 , 20   m   s 1 and 30   m   s 1 , respectively. Although flame tongues already form and propagate at these equivalence ratios, they are generally flushed out by high speed flow structures after a few millimeters of propagation. When further increasing the equivalence ratios to 0.4 , 0.6 and 0.75 for bulk velocities of 10   m   s 1 , 20   m   s 1 and 30   m   s 1 , flame propagation can no longer be prevented by the approaching flow and the flame is not fully flushed out of the isothermal channel section. It is noted that the flashback limit for U b = 20   m   s 1 and atmospheric pressure has increased from Φ = 0.55 to Φ = 0.6 compared to the results presented in Reference [15]. This is due to the changed definition of the flashback limit. Flame propagation was previously declared flashback if the flame was capable of propagating for more than 5 m m [15]. For U b = 20   m   s 1 and Φ = 0.55 it is however observed that the flame may still be flushed out after a propagation of more than 5 m m . Flame propagation is therefore now only declared flashback if the flame is not fully flushed out of the isothermal channel section.
In Figure 4, the numerically obtained stable equivalence ratios and the equivalence ratios at flashback are compared with experimental flashback limits obtained by Eichler et al. [16] with a similar channel configuration. In the experiments, flashback was first observed approximately at Φ = 0.35 , Φ = 0.54 and Φ = 0.71 . It is evident that despite a slight underestimation of the flashback tendency for bulk velocities of 10   m   s 1 and 20   m   s 1 , the numerical simulations are capable of reproducing the experimental flashback limits with reasonable accuracy. The simulations are therefore capable of representing the flashback process not only qualitatively but also quantitatively. This is in accordance with the findings in Reference [15], where no low Mach number approximation was applied.
In addition to the atmospheric simulations, flashback simulations are performed at a subatmospheric pressure of 0.5   bar and at slightly elevated pressures of 2   bar and 3   bar . At p = 0.5   bar , bulk velocities of 10   m   s 1 and 20   m   s 1 are numerically investigated. As the flame thickness is expected to be larger at lower pressure levels, no additional mesh refinement is necessary compared to the atmospheric simulations. Only one cell split is thus applied to the base mesh by the adaptive mesh refinement algorithm. The flame thickness is however reduced at higher pressure levels. Two cell splits are therefore applied at p = 2   bar and a bulk velocity of 10   m   s 1 . As already mentioned for the atmospheric simulations, two cell splits can not be applied to simulations with U b = 20   m   s 1 due to limited computational resources. A maximum of only one cell split is therefore applied at U b = 20   m   s 1 and p = 2   bar . As one cell split is not expected to be sufficient for p = 3   bar and U b = 20   m   s 1 , the investigation of the highest pressure level is limited to U b = 10   m   s 1 . Here, the initial inert mesh is refined in x-direction by increasing the cell count in x-direction by a factor of 1.5 . The adaptive mesh refinement additionally refines the mesh by applying a maximum of two cell splits.
The flashback limits at different pressure levels resulting from this refinement strategy are depicted in Figure 5. Here, the flashback limit is defined as the first equivalence ratio, where the flame is not flushed out of the isothermal section of the channel. The error bars illustrate the fact that flashback might already occur at any equivalence ratio between the last stable simulation and the first simulation in which flashback occurs. For p = 0.5   bar and U b = 20   m   s 1 , no flashback was observed up Φ = 1.7 . The laminar flame speed obtained from Cantera simulations reaches its maximum below this equivalence ratio. Increasing the equivalence ratio beyond Φ = 1.7 does therefore not increase flashback propensity and flashback is not expected to occur for p = 0.5   bar and U b = 20   m   s 1 . From Figure 5 it is evident that increasing the pressure leads to lower flashback limits. Only the case at p = 3   bar and U b = 10   m   s 1 shows an identical flashback limit compared to the lower pressure case at p = 2   bar . At U b = 10   m   s 1 , the pressure exponent of the dependency Φ F B p n is n = 0.46 , n = 0.37 , n = 0.29 at pressures of 1   bar , 2   bar and 3   bar compared to the flashback limit at p = 0.5   bar . At U b = 20   m   s 1 , the pressure exponent is n = 0.26 at p = 2   bar compared to the flashback limit at p = 1   bar . In literature, pressure exponents of unconfined flashback have been found to lie between n = 0.27 and n = 0.51 for H 2 -CO-air flames and between n = 0.43 and n = 0.49 for H 2 -air flames [5,6]. The numerically obtained pressure exponents for confined flames are thus similar to experimentally obtained pressure exponents for unconfined flames. In the confined simulations, there is however no unique pressure exponent for one bulk velocity. Instead, the pressure exponent for U b = 10   m   s 1 decreases with increasing pressure.

3.2. Macroscopic Flame Structure and Turbulent Flame Speed

The propagating flame fronts at all four pressure levels can be compared in Figure 6. It is evident that flame front wrinkling increases with pressure. Furthermore, the radius of the propagating flame tongue decreases with increasing pressure. This is caused by the decrease of flame thickness with higher pressure. The smaller flame thickness makes the flame more susceptible to flame wrinkling and allows for smaller flame structures. The flame thickness δ f is defined by
δ f = T a d T u max T x i ,
where T / x i is the temperature gradient. The turbulent flame thickness is obtained by sampling the magnitude of the temperature gradient of one time step on isosurfaces of the progress variable c. The progress variable for lean mixtures is defined by the unburnt hydrogen mass fraction Y H 2 , u and the local hydrogen mass fraction Y H 2 :
c = Y H 2 , u Y H 2 Y H 2 , u .
19 isosurfaces of c between 0.05 and 0.95 from at least 27 time steps during flame flashback are considered for sampling the temperature gradient. Wall normal turbulent flame thickness profiles are obtained for each of the 19 isosurfaces by calculating the flame thickness from the streamwise, spanwise and time average of the sampled temperature gradient. A minimum average flame thickness of all flame thickness profiles is computed for each wall normal distance. This approach results in the minimum flame thickness profiles in Figure 7. It is evident that although the equivalence ratio is reduced with increasing pressure, the flame thickness significantly reduces with increasing pressure.
The flame thickness profiles in Figure 7 can be used to obtain a minimum resolution of the simulations. The flame thickness is therefore divided by the cube root of the cell volume. This results in minimum resolutions of 3.0 cells per flame thickness for U b = 10   m   s 1 and Φ = 0.33 at p = 3   bar up to 5.5 cells per flame thickness for U b = 10   m   s 1 and Φ = 0.55 at p = 0.5   bar . The minimum resolution requirement of 3 cells per flame thickness [25] is thus fulfilled for all cases.
Increasing the pressure from 2 bar to 3 bar at U b = 10   m   s 1 and Φ = 0.33 does not decrease the average flame thickness as strongly as at lower pressures. This is confirmed by the laminar flame thicknesses in Figure 8 obtained from freely propagating flame simulations with Cantera [38]. It is evident that at low pressures, flame thickness decreases with increasing pressure. At higher pressures, the flame thickness however increases with increasing pressure. At very high pressure levels, the flame thickness of all equivalence ratios decreases again with increasing pressure. It is therefore expected that the flame thickness is increased and the susceptibility to flame front wrinkling is decreased at low equivalence ratios and higher pressures. In addition, the laminar flame speed decreases with increasing pressure [38]. The turbulent flame speed at flashback conditions does therefore not necessarily increase with pressure.
The turbulent flame speed in the simulations can be estimated from Figure 9, where the average stable flame shapes are shown for all operating conditions. The flame shapes are represented by isolines of the averaged progress variable, which are obtained by spatially averaging the temporal average of the hydrogen mass fraction field. The decreasing laminar flame speed at higher pressures can not be compensated by the increased flame front wrinkling due to smaller flame thicknesses. This leads to smaller average flame angles at higher pressure. The average flame shape is however only an inaccurate measure for the turbulent flame thickness. Figure 10 therefore shows the turbulent flame speed profiles of all stable cases at U b = 10   m   s 1 and U b = 20   m   s 1 . Here, the turbulent flame speed is defined as the average gas velocity component normal to the flame front [40]. This gas velocity is measured at the c ¯ = 0.05 isoline of the average flame front. The measured gas velocity is corrected by the factor T u / T in order to account for the temperature rise to the flame temperature T at c ¯ = 0.05 . The actual turbulent flame speeds depend on the chosen value of c ¯ for the flame speed evaluation. The turbulent flame speed profiles in Figure 10 are therefore normalized by the maximum turbulent flame speed at the corresponding bulk velocity. The turbulent flame speed profiles demonstrate that the maximum turbulent flame speed at conditions close to flashback varies strongly with pressure. The maximum turbulent flame speed at U b = 10   m   s 1 and p = 3   bar is only 73% of the maximum turbulent flame speed at U b = 10   m   s 1 and p = 0.5   bar . From Equation (4), this difference in turbulent flame speed would result in a deviation of 40% in flashback channel centerline velocity. This shows that the average flame shape, the turbulent flame speed and Equation (4) are poor indicators for the susceptibility of boundary layer flashback.

3.3. Average Pressure and Velocity Fields

Eichler et al. [16] showed that confined flames induce a pressure rise ahead of the flame which leads to flow deflection away from the wall. This can also be observed in Figure 11a, where the streamlines of the time and spanwise averaged velocity field are depicted together with the average flame shape and pressure field for the stable case at U b = 10   m   s 1 and p = 0.5   bar . Ahead of the flame the streamlines are deflected away from the wall. The turbulent flame brush redirects the streamlines back towards the wall. The flow redirection is caused by the fact that the tangential gas velocity is not changed by the flame front, while the velocity component normal to the flame front increases due to the density decrease across the flame. Ahead of the flame the flow is deflected away from the wall and the axial gas velocity decreases. The two-dimensional flow pattern is linked to a two-dimensional pressure field with a pressure maximum just ahead of the leading flame tip. This confirms the two-dimensional nature of the velocity field and of the pressure rise ahead of the flame observed by Eichler [11].
The flashback equivalence ratio decreases with increasing pressure. The expansion ratio ρ u / ρ b of unburnt gas density ρ u to burnt gas density ρ b therefore also decreases with increasing pressure. This leads to weaker flow deflection at higher pressures, which can be seen when comparing the streamlines in Figure 11b for the stable case at p = 3   bar with the streamlines in Figure 11a at p = 0.5   bar . The different streamline patterns in Figure 11 show that average boundary layer separation is not an indicator for flame flashback. The boundary layer at p = 0.5   bar shows stronger flow deflection and is much closer to average boundary layer separation than the boundary layer at p = 3   bar . At elevated pressures, flashback thus occurs at reduced turbulent flame speeds, reduced expansion ratios and at reduced average flow deflection ahead of the flame. These average quantities alone can therefore not describe the flashback propensity of a flame. Instead, local processes at the flame tip, such as flame quenching and local flow separation have to be taken into account.

3.4. Quenching Distance and Local Flow Separation

In addition to the average quantities previously presented, the local quantities at the propagating flame front also show significant differences depending on the operating conditions. By tracking the flame front during flashback, the separation zone size and quenching distance during flashback are obtained. Figure 12 exemplarily shows the hydrogen reaction rate and flow separation zone on a cutting plane through the foremost flame tip during flashback at U b = 20   m   s 1 and p = 1   bar . From this cutting plane, a wall-normal profile of the maximum hydrogen reaction rate can be obtained. The quenching distance δ q is then defined as the wall distance of the first local maximum of this maximum hydrogen reaction rate profile. The separation zone size y s is the wall-normal size of the region, where the streamwise velocity u 0 .
Endres and Sattelmayer [15] showed that upstream flame propagation takes place when the separation zone size is significantly larger than the average quenching distance. This is also evident for U b = 20   m   s 1 and p = 1   bar in Figure 13, where the x position of the foremost flame tip is compared to the separation zone size and the quenching distance during flashback. This is however not necessarily always the case. During flashback at U b = 10   m   s 1 and p = 0.5   bar , upstream flame propagation also occurs in time periods where the separation zone size is considerably smaller than the quenching distance. This implies that the flame speed for this operating condition is high enough for the flame to propagate upstream at wall distances above the separation zone and not only in the backflow region of the separation zone.
The average quenching distances and separation zone sizes during upstream propagation of all cases under investigation are listed in Table 2. The quenching distance decreases with increasing pressure. This is in accordance with the trend of the flame thickness, which also decreases with pressure. Dividing the quenching distance by the average flame thickness at the quenching wall distance from the profiles in Figure 7 results in the quenching Peclet numbers P e q in Table 2. For head-on quenching of laminar hydrogen-oxygen and hydrogen-air flames, Dabireau et al. [44] and Gruber et al. [45] found quenching Peclet numbers of P e q = 1.7 and P e q = 1.4 . Except for U b = 20   m   s 1 and p = 2   bar , where a few cells lie in the thin reaction zones regime, the current quenching Peclet numbers are of the same order of magnitude as the Peclet numbers from literature. The difference in quenching Peclet numbers are likely to arise due to the difference in quenching configuration. The Peclet numbers given here are for turbulent sidewall quenching while the cited literature values are for laminar head-on quenching.
The average separation zone size also decreases with increasing pressure. With increasing pressure, the flame thickness and the flame tip radius decrease while the fresh gas density increases with increasing pressure. This leads to weaker flow deflection ahead of the flame, as already seen from the average streamlines in Figure 11. From Table 2 it is however evident that the ratio of separation zone size to quenching distance is not constant. For U b = 10   m   s 1 for example, it increases from 0.84 at p = 0.5   bar to 2.23 at p = 2   bar . The decrease of quenching thickness with pressure is thus stronger than the decrease of separation zone size. There is hence no unique ratio between separation zone size and quenching distance which could be used as a criterion for the onset of flame flashback.
From p = 2   bar to p = 3   bar , the ratio of separation zone size to quenching distance is reduced from 2.23 to 2.16. This indicates that here, the separation zone size decreases more strongly than the quenching distance. In addition to the turbulent flame speed, this is another reason why the simulation at U b = 10   m   s 1 and p = 3   bar does not show a higher flashback equivalence ratio than at p = 2   bar . It was shown in Section 3.2 that the laminar flame thickness increases with pressure at very lean gas mixtures and higher pressures than investigated in the present study. It is possible that the quenching distance and the separation zone size show a similar trend and increase with increasing pressure. Depending on the ratio of separation zone size to quenching distance, this may increase or decrease the flashback propensity of the confined flames at higher pressures.

3.5. Implications for Analytical Flashback Prediction

The comparison of the pressure rise estimated by the analytical model of Hoferichter et al. [9] with the pressure rise obtained from LES shows that the analytical model does not accurately predict the quantitative values of the pressure rise. According to the analytical model the pressure rise for the stable atmospheric case at U b = 10   m   s 1 and Φ = 0.38 is 32.2 Pa , while in the simulations only 5.5 Pa are observed. This pressure rise is similar to the pressure rise observed with the compressible solver from Reference [15]. The low Mach number assumption thus does not have a strong effect on the average pressure rise ahead of the flame front. At U b = 20   m   s 1 and Φ = 0.55 and at U b = 30   m   s 1 and Φ = 0.7 the pressure rise ahead of the flame is 22.9 Pa and 63.7 Pa in the simulations. The analytical model however predicts a pressure rise of 106.4 Pa and 214.3 Pa for the same operating conditions. The pressure rise ahead of the flames of all cases is thus overestimated by the one-dimensional pressure calculation of the analytical model. At the same time, the Stratford separation criterion underestimates the separation propensity at BLF. The Stratford criterion is based on the boundary layer theory. The application of the boundary layer theory requires a uniform wall-normal pressure. Figure 14 shows the average wall-normal pressure profile just upstream of the stable atmospheric flame at U b = 20   m   s 1 . It is evident that the pressure is not constant over the channel height. Such a non-uniform pressure profile does not only cause flow deceleration but also flow deflection. This increases the tendency for boundary layer separation. The boundary layer theory and the Stratford criterion cannot be applied in this case.

4. Conclusions

The influence of pressure on the combustion and flow characteristics was investigated by comparing LES results of confined BLF at different pressure levels and bulk velocities. At elevated pressure the flame thickness decreases and the flame is corrugated more strongly by turbulence and thermal-diffusive instabilities. The turbulent flame speed and the flame angle at conditions close to flashback however decreased with increasing pressure. The average flow deflection ahead of the flame also decreased with increasing pressure. Lower turbulent flame speeds and weaker flow deflection ahead of the flame at higher pressure levels would imply a reduced flashback propensity at higher pressure levels. It was however shown that the flashback propensity increased with increasing pressure. The turbulent flame speed, the average flame shape and flow deflection alone are thus poor indicators for the onset of BLF.
Instead, additional quantities such as the quenching distance and the local separation zone size have to be accounted for. The quenching thickness decreases with increasing pressure. At the same time, the local separation zone size ahead of the propagating flame tip decreases with increasing pressure. The reduced flame thickness and quenching distance lead to a smaller flame tip diameter, which reduces the deflection of the approaching flow by the flame. Although these two local effects are counteracting, they do not cancel out and their influence on the flashback limits cannot be neglected. Confined BLF is instead a complex process, which is influenced by the local flame speed, the flame thickness, the quenching distance and the separation tendency of the approaching flow. The low separation zone sizes and high quenching distances at low pressure increase the flashback resistance of the flame, thus allowing for higher stable equivalence ratios. As the flame speed increases with increasing equivalence ratio at low pressures, the susceptibility of the flame to flashback increases. Usually flame propagation occurs inside the recirculating flow of the separation zone. The high flame speeds at low pressures however also allows for flame propagation in regions without recirculating flow.
Finally it was noted that the underlying assumptions of the boundary layer theory and of one-dimensional pressure approximations are not satisfied in confined BLF. The application of one-dimensional pressure approximations leads to an overestimation of the pressure rise ahead of the flame. The application of the boundary layer theory leads to an underestimation of the separation probability. These two errors are counteracting and might possibly compensate each other. Due to this inconsistency, the analytical flashback prediction model [9] should however rather be regarded as a correlation on the experimental flashback data, which is capable of accurately accounting for flashback influences such as preheat temperature or fuel composition.

Author Contributions

Conceptualization: A.E. and T.S.; methodology, software, validation, formal analysis, investigation, writing—original draft preparation, visualization: A.E.; writing—review and editing, supervision: T.S.

Funding

This research was funded by the German research foundation DFG, project No. SA 781/19-1.

Acknowledgments

The authors gratefully acknowledge the compute and data resources provided by the Leibniz Supercomputing Centre (www.lrz.de).

Conflicts of Interest

The authors declare no conflict of interest. The funders had no role in the design of the study; in the collection, analyses, or interpretation of data; in the writing of the manuscript, or in the decision to publish the results.

Abbreviations

The following abbreviations are used in this manuscript:
BLFBoundary Layer Flashback
LESLarge Eddy Simulation
ILESImplicit LEL
ODEOrdinary Differential Equations
SGSSubgrid Scale

Appendix A

Table A1. Parameters for the mixture diffusivity calculation.
Table A1. Parameters for the mixture diffusivity calculation.
p Φ T ad s l , 0 p = 1 bar m α ν Le D
in bar in Kin m s 1 in m 2 s 1 in m 2 s 1 in m 2 s 1
0.50.551741.40.76−0.267.275 × 10 5 3.722 × 10 5 0.4581.587 × 10 4
10.41422.30.35−0.353.248 × 10 5 1.754 × 10 5 0.3948.246 × 10 5
10.61838.60.92−0.243.698 × 10 5 1.864 × 10 5 0.4847.640 × 10 5
10.752096.81.40−0.184.003 × 10 5 1.944 × 10 5 0.5727.000 × 10 5
20.331257.20.20−0.401.559 × 10 5 8.689 × 10 6 0.3704.212 × 10 5
20.51640.70.61−0.291.763 × 10 5 9.166 × 10 6 0.4354.053 × 10 5
30.331257.20.20−0.401.039 × 10 5 5.793 × 10 6 0.3702.808 × 10 5

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Figure 1. Computational domain and stable flame shape for reactive LES.
Figure 1. Computational domain and stable flame shape for reactive LES.
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Figure 2. LES combustion regimes for U b = 10   m   s 1 .
Figure 2. LES combustion regimes for U b = 10   m   s 1 .
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Figure 3. LES combustion regimes for U b = 20   m   s 1 and U b = 30   m   s 1 .
Figure 3. LES combustion regimes for U b = 20   m   s 1 and U b = 30   m   s 1 .
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Figure 4. Atmospheric flashback limits obtained from the reactive LES compared to experimental flashback limits of Eichler et al. [16].
Figure 4. Atmospheric flashback limits obtained from the reactive LES compared to experimental flashback limits of Eichler et al. [16].
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Figure 5. Pressure influence on numerical flashback limits.
Figure 5. Pressure influence on numerical flashback limits.
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Figure 6. Instantaneous flame fronts and separation zones during flashback at the pressure levels (a) 0.5 bar, (b) 1 bar, (c) 2 bar and (d) 3 bar for U b = 10   m   s 1 . The flame front is represented by the red c = 0.5 isosurface. The separation zone is represented by the blue u = 0 isosurface.
Figure 6. Instantaneous flame fronts and separation zones during flashback at the pressure levels (a) 0.5 bar, (b) 1 bar, (c) 2 bar and (d) 3 bar for U b = 10   m   s 1 . The flame front is represented by the red c = 0.5 isosurface. The separation zone is represented by the blue u = 0 isosurface.
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Figure 7. Flame thickness profiles at flashback conditions for (a) U b = 10   m   s 1 and for (b) U b = 20   m   s 1 and U b = 30   m   s 1 .
Figure 7. Flame thickness profiles at flashback conditions for (a) U b = 10   m   s 1 and for (b) U b = 20   m   s 1 and U b = 30   m   s 1 .
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Figure 8. Pressure dependence of the laminar flame thickness obtained from one-dimensional freely propagating flame simulations.
Figure 8. Pressure dependence of the laminar flame thickness obtained from one-dimensional freely propagating flame simulations.
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Figure 9. Comparison of average stable flame shapes at different pressure levels evaluated at c ¯ = 0.5 . (a) for U b = 10   m   s 1 and (b) for U b = 20   m   s 1 .
Figure 9. Comparison of average stable flame shapes at different pressure levels evaluated at c ¯ = 0.5 . (a) for U b = 10   m   s 1 and (b) for U b = 20   m   s 1 .
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Figure 10. Comparison of turbulent flame speeds at different pressure levels for (a) U b = 10   m   s 1 and for (b) U b = 20   m   s 1 .
Figure 10. Comparison of turbulent flame speeds at different pressure levels for (a) U b = 10   m   s 1 and for (b) U b = 20   m   s 1 .
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Figure 11. Average streamlines, average flame shape and average pressure field of the stable cases at U b = 10   m   s 1 at (a) p = 0.5 bar and at (b) p = 3 bar. The average flame shape is represented by the blue c ¯ = 0.5 isoline.
Figure 11. Average streamlines, average flame shape and average pressure field of the stable cases at U b = 10   m   s 1 at (a) p = 0.5 bar and at (b) p = 3 bar. The average flame shape is represented by the blue c ¯ = 0.5 isoline.
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Figure 12. Hydrogen reaction rate and flame separation during flashback. Blue line represents the u = 0 isosurface.
Figure 12. Hydrogen reaction rate and flame separation during flashback. Blue line represents the u = 0 isosurface.
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Figure 13. Flame front position, separation zone size and quenching distance during flame flashback. Flame front position x f is given by the foremost cell with c > 0.5 .
Figure 13. Flame front position, separation zone size and quenching distance during flame flashback. Flame front position x f is given by the foremost cell with c > 0.5 .
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Figure 14. Wall-normal average dynamic pressure profile ahead of the stable flame front at atmospheric pressure and U b = 20   m   s 1 .
Figure 14. Wall-normal average dynamic pressure profile ahead of the stable flame front at atmospheric pressure and U b = 20   m   s 1 .
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Table 1. Simulation parameters for inert large eddy simulations (LES).
Table 1. Simulation parameters for inert large eddy simulations (LES).
U b Re u τ , Pope Re τ , Pope y 1 + Δ x + Δ y + Δ z + N x × N y × N z
10   m   s 1 97220.598290.70.6313.4212.528.90 130 × 118 × 98
20   m   s 1 19,4441.101535.20.6613.7213.119.02 234 × 208 × 178
30   m   s 1 29,1671.573764.40.7918.3516.2412.07 250 × 240 × 190
Table 2. Quenching and separation parameters at flashback conditions.
Table 2. Quenching and separation parameters at flashback conditions.
p U b Φ δ q δ f y = δ q Pe q y sep ¯ y sep ¯ / δ q
in barin m s 1 in mmin mm in mm
0.5100.550.780.810.960.660.84
1100.40.420.391.060.651.56
1200.60.360.390.920.551.53
1300.750.370.390.940.531.45
2100.330.240.181.310.542.23
2200.50.180.260.680.281.58
3100.330.180.181.000.392.16

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Endres, A.; Sattelmayer, T. Numerical Investigation of Pressure Influence on the Confined Turbulent Boundary Layer Flashback Process. Fluids 2019, 4, 146. https://doi.org/10.3390/fluids4030146

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Endres A, Sattelmayer T. Numerical Investigation of Pressure Influence on the Confined Turbulent Boundary Layer Flashback Process. Fluids. 2019; 4(3):146. https://doi.org/10.3390/fluids4030146

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Endres, Aaron, and Thomas Sattelmayer. 2019. "Numerical Investigation of Pressure Influence on the Confined Turbulent Boundary Layer Flashback Process" Fluids 4, no. 3: 146. https://doi.org/10.3390/fluids4030146

APA Style

Endres, A., & Sattelmayer, T. (2019). Numerical Investigation of Pressure Influence on the Confined Turbulent Boundary Layer Flashback Process. Fluids, 4(3), 146. https://doi.org/10.3390/fluids4030146

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