1. Introduction
Plastic, a synthetic material made from various organic compounds with a high molecular mass, was first introduced in 1907 by Leo Baekeland [
1]. Since then, it has changed numerous industries. During World War II, there was rapid growth in the plastic industry, as manufacturers could use plastic to replace products previously manufactured using natural resources. The best example was nylon, which replaced silk and was used for parachutes, helmets, and body armour; another was plexiglass, used as a substitute for glass in aircraft [
2].
Over time, plastics replaced the use of traditional materials. It has become one of the essential materials in day-to-day life. Properties such as high strength, corrosion resistance, easily mouldability, waterproofness, and its ductile nature make it fit a wide range of applications. It is used in almost every sector, such as in electrical and electronic applications, packaging, logistics, and industrial machinery. More than 50% of plastic was produced after the year 2000. Most plastic is used for packaging [
3].
Its production involves the polymerisation or polycondensation of natural materials, such as cellulose, coal, natural gas, salt, crude oil, minerals, and plants. It can be moulded into various shapes, sizes, and forms. It also possesses remarkable properties, such as lightness, durability, flexibility, and affordability, and is thus a popular choice over traditional materials, such as wood, natural fibres, rubber, and paper [
4].
Despite having advantages, such as cheaper cost and ease of production, it affects the environment if not utilised properly. According to EEA, plastics have many other effects, including contributions to climatic change, and the report says that there is no control over the production and consumption of plastics [
5]. There is a great need to develop a circular trend by inventing various recycling techniques. However, according to the Ellen MacArthur Foundation, only 14% of the plastic produced is recycled [
6]. Every year, countries worldwide discard millions of tons of plastic waste. Less than 20% of waste plastic is recycled to make new plastics, while the remaining plastics are either disposed of in landfills or burnt or dumped [
7]. The only way to minimise its impact is to stop using it; however, in the modern world, this is impossible due to excessive reliance on plastic items. Thus, one of the valuable solutions is to convert the available waste plastic into raw material for various new plastic goods, speeding up the recycling process.
Technically, all polymers are recyclable and can be used once or more to create an identical product [
8]. However, it must be carried out in controlled conditions and requires high-end machinery and technology. This is not a feasible solution, because it harms the environment and makes industries unprofitable. Therefore, it is best to sort waste plastic according to its categorisation and qualities to extract recyclable plastic and use it to produce plastic products in the future. Because of the process-induced breakdown of the polymer chain, the properties of such recycled materials may differ from those of the original. These properties can be regained by adding the appropriate additives and strength-enhancing materials [
9].
Researchers conducted experiments to investigate the optimal combination of raw materials, plastic, and sand to achieve maximum brick strength. These experiments involved varying proportions of the raw materials. One specific experiment conducted by Wahid et al. [
10] utilised a mixture of sand, sand dust, and cement in a ratio of [9:9:4]. The mixture was then mixed with plastic waste in weights of 0%, 5%, 10%, and 15%. The highest compression strength observed was 12.4 N/mm
2 when 0% plastic was used, and the strength decreased as the percentage of plastic increased. The reduction in strength was attributed to poor adhesion between the plastic waste and cement. Additionally, a longer curing time was required due to the significant volume of cement and sand. These findings suggest that plastic waste in brick production may not necessarily improve the strength of bricks, and further research is needed to optimise the proportions of the raw materials and curing process.
In an extension of the research of Wahid et al. [
10], another researcher, Agyeman et al. [
11], mixed plastic: quarry dust: sand ratios of 1:1:2 and 2:1:2 by weight. The resulting samples were then cured for seven days by being sprinkled with water. The bricks produced from these mixtures were tested for their compressive strengths and water absorption rates. It was found that the bricks produced from the 1:1:2 mixture had a compressive strength of 6.07 N/mm
2 and a water absorption rate of 4.9%, while the bricks produced from the 2:1:2 mixture had a higher compressive strength of 8.53 N/mm
2 and a lower water absorption rate of 0.5%.
As per Circular Action Hub (CAH) [
12], mixing recyclable plastics with sawdust, concrete, mud, or sand can replace conventional building materials. High-density polyethylene is one of those recyclable plastics. Typically, HDPE produces storage containers for milk, shampoo, oil, and chemicals. It is comparatively more stable and emits fewer hazardous gases, and is thus acceptable for recycling under certain controlled circumstances. Globally, about 40 million tonnes of HDPE waste are generated [
13].
High mechanical strength, transparency, non-toxicity, no effect on taste, and permeability that may be disregarded for carbon dioxide are all characteristics of HDPE plastic. In addition to being transparent, processable, colourable, and thermally stable, HDPE plastic is chemically resistant, tensile, and impact-resistant [
14].
The polyethylene grade with the most stiffness and least flexibility is HDPE. It works well for various uses, such as garbage cans and everyday home items, including miniature bottles and clothespins. This non-toxic, lightweight material can replace less eco-friendly materials because it is readily recyclable [
15].
An analysis conducted by Sahani et al. [
16] found that recycling plastic waste in manufacturing bricks and tiles is an effective way to reduce waste. The study suggested that when plastic and sand are combined in the proper ratio, the resulting bricks have a higher compression strength than traditional clay bricks. The highest compression strength was achieved with a plastic-to-sand ratio of 1:4, valued at 12.28 N/mm
2. However, as the amount of plastic in the mixture decreased, the compression strength also decreased.
The research of Kulkarni et al. [
17] shows that HDPE plastics have a higher compression strength of 14.6% than conventional bricks, with a brick wall’s ultimate load-carrying capacity being 197.5 KN. This means they can be used to build structures supporting higher loads. According to Maneeth et al. [
18], bitumen acts as a binder and enhances the strength of the bricks because of its stability and density. However, as the bitumen percentage increases, the compression strength declines from 10 N/mm
2 to 2.04 N/mm
2, with the ideal bitumen percentage being 2%. According to Benny T.K. et al. [
19], bitumen-added bricks have a hydrophobic property that prevents water from infiltrating them. They also have a higher compression strength than standard bricks, with a compression loading of 120 KN. In this way, large amounts of waste can be used without affecting the environment and reducing the cost of construction.
This publication aims to manufacture plastic sand bricks using bitumen and find the optimum percentages of plastic and sand for producing bricks with higher compression strength and a lower water absorption rate than conventional bricks.
4. Discussion
The idea of using HDPE bricks instead of standard bricks was to turn waste plastic into a usable product. Using a novel manufacturing process, the primary goal of the study was to determine the ideal plastic-to-sand ratio. Brick samples can be prepared by varying the proportion of plastic in the mixture. The proportions considered were 75%, 60%, 50%, 40%, and 25% by weight. In samples where 75% plastic was used, bitumen was added in proportions of 1%, 2%, and 3% by weight. It was observed that the compression stress of the bricks increased gradually as the amount of bitumen was increased until it reached a maximum stress of 33.46 MPa. However, if the amount of bitumen added exceeded 2%, the bricks became softer. This can be observed in
Figure 2a, where the stress value is decreased to 31.8 MPa. Due to its good adhesive property, bitumen was used to increase the strength of the bricks, even though the plastic in the mixture was sufficient to bind the sand. However, excessive amounts of bitumen had a negative impact on the quality of the bricks.
It was observed that the strength of bricks could be improved by varying the proportion of plastic used in the mixture. Specifically, when the amount of plastic was reduced by 15%, the stress values increased from 21.2 MPa to 22.6 MPa. The stress values decreased to 16.25 MPa when the amount of plastic was further reduced to 25%. Moreover, when 9 g of bitumen was added to a sample containing 60% plastic, the stress values reached a maximum of 37.5 MPa.
The increase in stress values with a reduction in the amount of plastic or the addition of bitumen was likely due to the changes in the physical properties of the brick. With a reduction in the amount of plastic or adding bitumen, the interlocking of the sand particles can be improved, leading to increased strength and stress values. However, adding too much bitumen may have adverse effects, as it can make the bricks softer and weaker. The mixture of 60% plastic and 9 g bitumen in sand produced the strongest results. The average stress of all the samples was found to be 25 MPa, and it was noted that the majority of stress readings deviated by an average of 2.54 MPa from the average stress. In order to find the average compression stress, a set of five observations of compression stress values were taken and mean stress was calculated. Additionally, the standard deviation was calculated to find the spread or variation in the compression values. This helped in the assessment of risk and of how much the stress values differed from the mean stress.
Bricks should absorb the least amount of water possible. As seen in
Figure 9, the water absorption test demonstrated that no bricks absorbed more water than 1% after being soaked for 24 h. This is especially helpful in the construction sector, because when bricks absorb more water, damage to the building arose. This test is also valuable in areas where water leakage is a primary concern. The bricks with the highest water absorption percentage were 0.9%. The decrease in plastic content in bricks increased their water absorption rate, with most bricks having a water absorption rate of around 0.2%. However, as plastic content decreased, the water absorption rate increased, potentially reaching a rate of 0.9%. The permissible range was 1% to 2%, while zero was the best value for a brick. The 0.9% water content was caused by the tiny gaps between the granules and the quick cooling of the bricks in the hot press.
The efflorescence test (
Table 6) demonstrated that there were no soluble salts or alkalis present on the bricks with higher plastic–sand ratio (i.e., 3:1, 3:2, and 1:1), but the bricks with less plastic (i.e., 2:3) showed a slight alkali presence. When bitumen percentage increased, the alkalis were reduced, and for the ratio of 1:3, all bricks showed alkalis, which demonstrated that with more plastics, the presence of alkalis decreased. The relative temperature rise shown in
Table 7 demonstrated that the temperature difference was greatest for bricks that contained the most plastic and bitumen. As a result, the temperature transfer from one side of the brick to the other took longer, which could be advantageous in a fire accident. The results showed that the initial temperatures of the bricks were all around 19.2 °C. When the samples were placed on a heat source maintained at 400 °C, the temperatures at the left and right faces of the bricks after 3 min ranged from 325 °C to 338 °C and 42 °C to 62 °C, respectively. It was observed that the temperature difference increased as the amount of plastic in the bricks increased, indicating that heat conduction was decreasing.
As in Kulkarni’s [
17] study, bitumen was added after the HDPE and quartz sand were ground into granules. This caused the bitumen to be distributed equally, which strengthened bonds. It was discovered through several tests, including the efflorescence, water absorption, and compression tests, that HDPE bricks performed better than conventional bricks. The combination of high-density polyethylene, sand, and bitumen in this study increased the strength of the brick. The bricks’ compression strength gradually improved for the plastic sand ratio, rising from 22.08 MPa with 0% bitumen to a peak of 33.46 Mpa with 2% bitumen and falling just short of 32 MPa for 3% bitumen. These results suggested that bitumen aided in fusing sand and plastic, increasing the strength of the brick. During the initial point of the compression test, no stress was observed, indicating that the specimen may have been able to undergo further compression and that a more compact specimen could be made with less thickness.
5. Conclusions
This research work inferred that recycling plastic waste for building projects was the way of the future, as it would help reduce plastic waste and the price of bricks in the construction industry. HDPE, quartz sand, and bitumen were used in this research work to make bricks, and it was found that this combination led to an improvement in the strength of the bricks while reducing their weight. Additionally, the cost of these bricks was almost 50% less than conventional bricks. The cost of one conventional brick is around 0.20 to 0.50 euros. However, the cost of one plastic sand brick is around 0.092 euros, including the raw materials cost (i.e., for 1 kg of plastics, it costs 0.33 euros; for 1 kg of quartz sand, it costs 0.248 euros; and for 2% bitumen by weight (9 g), it costs 0.057 euros). HDPE and bitumen made the bricks more water-resistant by reducing their permeability, and quartz sand improved the binding between the plastics due to its strong binding properties.
This research indicates that adding bitumen to bricks can significantly enhance their tensile strength, with a maximum value of 37.5 MPa observed. However, it is important to note that an increase in the proportion of bitumen led to a decrease in the strength of the bricks. Therefore, it is recommended to use bitumen in moderation (i.e., around 9 g to 13.5 g) to achieve optimal results. Additionally, the combination of HDPE and quartz sand ensured that the bricks were void-free and free of alkalis, making them a suitable choice for the construction industry.
Overall, bricks with a bitumen content of 2% (i.e., 9 g of bitumen) and a plastic–sand ratio of 3:2 showed better properties than other bricks. Every brick had a compression strength that was better than typical clay bricks. For use in building, homes, and pallets, bricks with a higher percentage of plastics were preferable to those with a lower percentage of plastic (i.e., 2:3 and 1:3) since the bricks with fewer plastics possessed a significantly lower compression strength and a higher presence of alkalis. Plastic bricks are the best option for construction, parking chairs, and pathway pallets since they are very light, have a good load bearing capacity, have less water absorption, are inexpensive, and can gradually reduce plastic waste.
Although this is a useful method for recycling used plastic, plastic has the potential to emit greenhouse gases when used in excessively high temperatures. Conducting this experiment in a vacuum is always advised so that the carbon atoms released during heating cannot produce carbon dioxide and carbon monoxide, which affects the environment.
Further, this formula can be developed into high-strength tiles and hallow interlocking bricks that could replace the current materials without compromising strength. It was also found that the surfaces of the bricks were smoother. Hence, this process can be used to manufacture parts that need surface lubrication to reduce friction.