Advances in Smart and Tough Hydrogels (2nd Edition)

A special issue of Gels (ISSN 2310-2861). This special issue belongs to the section "Gel Applications".

Deadline for manuscript submissions: 30 December 2024 | Viewed by 1850

Special Issue Editors

The Wallace H. Coulter Department of Biomedical Engineering, Georgia Institute of Technology and Emory University, Atlanta, GA 30332, USA
Interests: nanomaterials; polymers; hydrogels; biomaterials; zwitterionic materials
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Guest Editor
College of Materials Science & Engineering, Zhejiang University of Technology, Hangzhou 310014, China
Interests: zwitterionic polymers; stimuli-responsive hydrogels; nanocomposite design and fabrication
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Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China
Interests: smart gels; soft actuators; shape memory materials
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Guest Editor
School of Medicine, Shanghai Jiaotong University, Shanghai 200240, China
Interests: bone tissue engineering; hydrogel; 3D printing; bio-mimetic hydrogel
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Special Issue Information

Dear Colleagues,

We are delighted to announce the launch of the newest Special Issue of Gels, “Advances in Smart and Tough Hydrogels (2nd Edition)”, which is dedicated to recent developments in the theoretical and fundamental aspects as well as the synthesis, characterization, and applications of smart and tough gels. Within this context, a broad range of subjects will be covered, including structure and dynamics, molecular modeling and simulation, and applications. 

Since the discovery of polymeric gels, scientists have conducted in-depth explorations of chemical structures, network distributions, and functional and component regulations for hydrogels to adapt to the application of hydrogels in different fields. Typically, if you search “smart and tough hydrogels” in Google Scholar, you may discover thousands of exciting findings and great peer-reviewed publications. As the hottest topics in the field of hydrogels, both stimuli-responsive (smart) hydrogels and tough hydrogels have attracted widespread attention as biomimetic systems due to their ability to respond to subtle changes in external and internal stimuli, ranging from physical triggers to chemical triggers, or to exhibit highly mechanical strength comparable to artificial bones. Progress in this field requires an interdisciplinary effort to accomplish a more detailed understanding of the structure and interactions that define the behavior of smart and tough hydrogels, making it possible to tailor the properties of these materials. Many theoretical, experimental, and practical application challenges remain.

Since this topic is of interest to a wide audience of researchers in different fields, including (but not limited to) physical science, chemistry, materials science, mechanical engineering, biomedical and tissue engineering, etc., we believe that the launch of this topic will stimulate new research and discoveries in the field of smart and tough hydrogels. We look forward to receiving your contributions.

Dr. Dong Zhang
Prof. Dr. Jintao Yang
Dr. Xiaoxia Le
Prof. Dr. Dianwen Song
Guest Editors

Manuscript Submission Information

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Keywords

  • stimuli-responsive hydrogels
  • tough hydrogels
  • synthesis and characterization
  • molecular understanding for tough hydrogels
  • sequence–structure–property relationships
  • biomimetic, biological, and biomedical applications
  • functional modifications

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Published Papers (1 paper)

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Research

16 pages, 4637 KiB  
Article
Fabrication of Tough Double-Network Hydrogels from Highly Cross-Linked Brittle Neutral Networks Using Alkaline Hydrolysis
by S. Shams Es-haghi and R. A. Weiss
Gels 2024, 10(1), 29; https://doi.org/10.3390/gels10010029 - 28 Dec 2023
Viewed by 1513
Abstract
This paper describes a simple method to synthesize tough hydrogels from a highly cross-linked neutral network. It was found that applying alkaline hydrolysis to a highly cross-linked hydrogel synthesized from acrylamide (AAm) can increase its swelling ratio dramatically. Double-network (DN) hydrogels synthesized from [...] Read more.
This paper describes a simple method to synthesize tough hydrogels from a highly cross-linked neutral network. It was found that applying alkaline hydrolysis to a highly cross-linked hydrogel synthesized from acrylamide (AAm) can increase its swelling ratio dramatically. Double-network (DN) hydrogels synthesized from polymerization of loosely cross-linked AAm networks inside a highly cross-linked AAm gel were not tough. However, repeating the same recipes with a second polymerization step to synthesize a DN hydrogel from a hydrolyzed highly cross-linked AAm gel resulted in tough hydrogels. Those gels exhibited finite tensile behavior similar to that of conventional DN hydrogels. Moreover, craze-like patterns were observed during tensile loading of a DN hydrogel synthesized from a hydrolyzed highly cross-linked first network and a loosely cross-linked second network. The patterns remained in the gel even after strain hardening at high stretch ratios. The craze-like pattern formation was suppressed by increasing the concentration of cross-linking monomer in the second polymerization step. Crack propagation in DN hydrogels synthesized using hydrolysis was also studied by applying a tensile load on notched specimens. Full article
(This article belongs to the Special Issue Advances in Smart and Tough Hydrogels (2nd Edition))
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