1. Introduction
Sinuous geometry widely exists in natural watercourses, and rivers with such shape are called meandering rivers. The flow pattern in meandering rivers is complex due to the existence of secondary flow, which arises from the combined actions of centrifugal forces, lateral pressure gradients caused by the tilting water surface, and wall shear stresses [
1]. This curvature-induced secondary flow can affect the primary flow and momentum transport, making the velocity redistribute and form a highly three-dimensional helical motion [
2]. The changes in flow structure complicate the process of mass transport and energy transfer [
3] and thus make it difficult to predict the pollutant transport in meandering rivers. The industrial wastewater and sanitary sewage are mostly discharged into rivers from the outlet of pipelines, which can be regarded as a point source effluent entering the river. Considering the severe pollution in watercourses worldwide, there is a growing need to better understand the fate of pollutants once they enter natural rivers or man-fabricated channels with sinuous geometry [
4]. Since the release positions of a point source can significantly affect the pollutant distribution in the near field and the mixing process in the far field [
5,
6], it is of great interest to quantify the transport characteristics of the point source pollutant in a sinuous open channel.
The experimental research on pollutant transport in sinuous open channel flows mainly focus on the measurement of scalar distribution and the determination of transverse dispersion coefficient in generalized water flumes. Fischer [
3] was among the first to assess the effect of a secondary current on pollutant transport inside a channel bend. By analyzing the measured velocity distribution, he proposed some theoretical equations describing the relationship between the transverse dispersion coefficient and some other hydraulic parameters. Later, Chang [
5] conducted a series of tracer tests in an idealized meandering channel to study the process of lateral mixing. He found that different release positions of a point source can greatly affect the distribution of tracer concentration downstream, which arises from the existence of secondary circulation that accelerates the lateral mixing. Fukuoka [
6] performed similar experiments in a sinuous flume and he stated that secondary flow causes a considerable lateral spreading of the tracer so that the mixing was much stronger than in a straight channel. Aside from flume experiments with rectangular cross-sections, Boxall [
7] made a meandering flume with natural bed profiles and the longitudinal and transverse mixing of the tracer was evaluated. He concluded that lateral mixing in meandering channels is dominated by vertical shear in spanwise velocities resulting from secondary circulations, while the longitudinal spreading is attenuated by the same effects. Despite some minor differences, most researchers agree that it is the secondary circulation that exerts a major impact on the mixing of pollutants in meandering rivers.
Numerical study has made substantial effort in the accurate reproduction of the experiment, and based on some high-precision numerical models, case studies have been carried out to address some issues in depth. In earlier years, due to the unaffordable computational cost, research has focused on two-dimensional numerical models to simulate meandering flow and scalar transport [
8]. These models were capable of making sound predictions to a certain extent, but more or less relied on the semi-empirical formulations in the aspect of a transverse dispersion coefficient [
9]. A three-dimensional numerical model based on
k-ε turbulence model combined with an advection-diffusion equation for pollutant transport was developed by Demuren [
10] and the results agree well with the laboratory measurements of Chang [
5] and Fukuoka [
6]. By using the
k-ε turbulence model, Huang [
11] discussed the impact of river sinuosity on the distribution patterns of a heavier or lighter pollutant released into a wide river. He also investigated the distribution characteristics of heavier or lighter pollutants released at different cross-sectional positions of a wide river [
12]. With the advancement of computing technologies, application of unsteady turbulence models for scientific study has become a trend. Large-eddy simulation (LES) can model the details of the bend flows more accurately compared with Reynolds-Averaged Navier–Stokes (RANS) models and more economically compared with Direct Numerical Simulation (DNS). As Booij [
13] found in a comparison study in bend flow, the RANS model fails to reproduce the outer bank cell correctly, while the LES performs well in providing detailed information of cells. Moreover, other research [
14,
15] has also demonstrated the superiority of LES. Balen [
15] compared various LES models in simulating the velocity field in channel bends but obtained a nearly identical result, indicating that different subgrid-scale models in LES have little influence on the large-scale motion in the open channel bend. Ignacio et al. [
16] investigated the pollutant mixing in a meandering open channel flow with different point source positions in spanwise directions using LES, but the impact of release locations in longitudinal direction is unexplored. Balen [
17] studied the influence of the water depth on the flow behavior and plume statistics of the line source within a channel bend with LES, and he found that the gradient-hypothesis of diffusion is limitedly valid.
This study aims to investigate the influence of release positions of a point source on the pollutant distribution and mixing process in a sinuous open channel. Apart from personal research interest, this study is also about practical applications in the hydraulic and environmental aspect. For instance, the reasonable design and operation of outlet structures must comply with water pollution criteria. Furthermore, the potential emergency of oil spills on water requires quick prediction of oil transport for providing feasible solutions. Furthermore, the findings can guide the management of river environments and help design measures for ecology improvement.
Although many studies have focused on the basic phenomenon of mass transport in secondary circulation, in-depth investigations into the pollutant mixing mechanism and the correlation between pollutant mixing efficiency and release positions of the point source in meandering rivers has not yet been adequately studied and well-understood. There is a gap in literatures about the assessment of mixing efficiency in quantification for such cases. The objective of this study is to quantitatively evaluate the effect of point source release positions on pollutant distribution and mixing process in a sinuous open channel. In addition, another motivation is to explore the role of secondary flow and turbulent diffusion in pollutant mixing. For this purpose, a three-dimensional numerical sinuous flume using LES for turbulence modelling was established, with the same configurations as the reported experiment by Chang [
5] for validation and calibration. Afterwards, two sets of cases in which the point sources were arranged at identical intervals in spanwise and streamwise directions were configured to evaluate the mixing efficiency. The role of secondary circulation together with turbulent diffusion in pollutant mixing is discussed. Moreover, the instantaneous and fluctuational characteristics of concentration are touched on. The mixing efficiency among different scenarios is also compared with appropriate indices.
3. Results and Discussion
In this section, the time-averaged values are denoted by the capital letters, whereas the instantaneous values are represented by the lower-case letters. For the convenience of data analysis, the velocity and scalar field were normalized by bulk velocity (Uav) and cross-sectional concentration (Cav), respectively. The variable names in the results are consistent with the following formula: Uh* = Uh/Uav (Uh is the depth-averaged streamwise velocity), U* = U/Uav, C* = C/Cav, u* = u/Uav, c* = c/Cav, CRMS* = CRMS/Cav. Moreover, the coordinate was scaled by the water depth (H) for brevity. Namely, X* = X/H, Y* = Y/H, Z* = Z/H.
3.1. Verification of Numerical Model
The depth-averaged streamwise velocity and concentration of the scalar from the simulation and experiment are compared for model validation. The measured and simulated dimensionless depth-averaged streamwise velocity
Uh* is displayed in
Figure 5. The comparison shows a similar trend between the two, which means a good agreement is obtained. It is noticeable that the streamwise velocity distributions of the upstream half of the bend (left column of
Figure 5) are symmetrical to their counterparts from the downstream half of the bend (right column of
Figure 5).
The measured and simulated depth-averaged scalar concentration
Ch normalized by local mean concentration
Cs is shown in
Figure 6. The definition of local mean concentration
Cs proposed by Chang [
5] is:
where
H is the water depth;
Q is the discharge;
Δx is the transverse length of sampling intervals;
n is the number of sampling intervals.
The verification result of the scalar field is also satisfied with the similar trend between measurements and calculations. The peaks of transverse concentration distribution are almost at the same locations within the cross-sections, and the tiny deviations in some regions are acceptable. It is obvious that the transverse distribution of the concentration is different among C1, C2, and C3, especially in 9B and 9C sections, which results from the distinct release positions.
3.2. Time-Averaged Hydrodynamic Characteristics
3.2.1. Distribution of Streamwise Velocity
The normalized streamwise velocity
U* in the form of contours and isolines are displayed in
Figure 7. Considering the symmetric characteristic of velocity field in sinuous channels, only the upstream half of the meander is shown, namely Section #01–#06, whereas the velocities in the downstream half of the meander can be deduced. It demonstrates that the high velocity region gradually approaches the inner bank before entering the bend (
Figure 7a,b), and this region is close to the inner bank wall within the bend (
Figure 7c,d). From Section #04 the maximum velocity region starts to shift towards the centerline of the channel and repeat the above procedures in the next bend. This phenomenon coincides with the findings in some literatures [
16,
27]. It can be found that a shear layer is formed between the high velocity region and inner bank walls, where a high longitudinal velocity gradient occurs. This region normally generates streamwise oriented vortices (SOV) due to the effect of shearing and leads to high intensities of turbulence [
28].
The plane view of the
U* distribution and dynamic axis of flow is shown in
Figure 8. It can be observed that the maximum velocity stays close to the inner bank within bends and goes back to the centerline in straight reaches. Moreover, the dynamic axis is found to take the shortest path marching forward along the channel.
3.2.2. Secondary Flow Structures
As stated before, secondary flow plays a significant role in the lateral mixing of the pollutant within meanders. To evaluate the effect of secondary current on pollutant transport, the vectors of secondary flow and contours of vorticities in typical cross-sections are presented in
Figure 9. The vectors are non-dimensional with bulk velocity
Uav, and the vorticities
Ωθ are normalized through bulk velocity
Uav and hydraulic radius
R. As can be observed, there exists more than one large flow circulation in each section which are often called center-region cells [
29]. Moreover, a flat circulation cell near the bottom that spans more than half of the section can be noticed, with an opposite rotational direction to that of cells located in the middle and upper part of the section. Moreover, at the four corners of a cross-section, small cells with different intensities are formed. Compared with the longitudinal velocity in
Figure 7, it can be found that the value of vorticity in the region of high velocity is small, while the high vorticity occurs in the area with lower velocity near the sidewalls. It is clearly visible that near the bottom of the inner bank of Section #03–#06 (
Figure 9c–f), a high intensity of vorticity is formed which was accompanied by a large velocity gradient and strong turbulence effect.
3.2.3. Turbulent Viscosity
Turbulent viscosity dominates the diffusion rate in the process of pollutant mixing in turbulent flows.
Figure 10 displays the distribution of normalized turbulent viscosity
νt, and it reveals that the large turbulent viscosity mainly occurs in the region where the gradient of streamwise velocity is high (
Figure 7). This phenomenon can also be deduced from Equations (6) and (8) that turbulent viscosity (subgrid viscosity) is proportional to the velocity gradient. In other words, the high gradient of streamwise velocity arising from flow shearing results in larger turbulent viscosity and vigorous diffusion. However, the secondary current is not the case (
Figure 8), probably because its order of magnitude is smaller than that of streamwise velocity. The Van Driest damping function is employed so that the turbulent viscosity is relevantly low near walls despite a strong shear effect.
3.3. Time-Averaged Scalar Distribution
3.3.1. Time-Averaged Concentration Field
The simulation results reveal that the different release positions of pollutants from point sources significantly affect the downstream concentration distribution along the sinuous channel.
Figure 11 displays the contours of the time-averaged concentration
C* of S1, S3, and S5. It can be discovered that there are obvious differences in the variation in the pollutant concentration along the channel among the three scenarios. In S1 for example, the pollutants quickly reach the bottom and continue to transport to the right bank after release. However, there exists an evident difference in the speed of lateral spreading between the pollutants in the top and bottom part of the cross-section. At Section #05, the bottom pollutants reach the opposite bank and move upwards along the right bank until Section #07, where the high concentration region of the bottom contacts with that of the top, forming a concentric ring structure surrounding the water with low concentration. In S3, the pollutants are continuously transported to both the sides and bottom after release, presenting a radial shape. At Section #04, the center of the contaminant cloud moves to the bottom, and gradually deviates to the bottom of the left bank in the subsequent transport process, and a low concentration area appears at the top of the right bank. The contaminant cloud in S5 also quickly reaches the bottom, while the pollutants at the top continue to move to the left bank while the bottom is gradually penetrated by the water with low concentration from the left bank, and the center of the contaminant cloud gradually moves to the center of the section to form a concentric ring structure surrounding the high concentration pollutants. In comparison, the contaminant cloud in S1 and S3 eventually forms a belt concentrated at the bottom of the left bank, while S5 forms a contaminant cloud located in the center of the section. In addition, the maximum concentration of S3 is low, which indicates rapid mixing.
Compared with the flow structures in
Figure 9, it can be found that the transverse transport process of pollutants in distinct scenarios is closely related to the secondary circulation. There exists a large range of flow motions from the left bank to the right bank in the middle and upper part of Section #02, which keep decreasing in the subsequent sections until it vanishes in Section #06. Meanwhile, a small range of flow motion can be observed from the right bank to the left bank near the bottom of Section #02, which continues to expand in the subsequent section until it almost occupies the whole section at Section #06. In addition, in Section #03 and the following sections, a flow motion from the left bank to the right bank at the bottom is generated. The above phenomenon of lateral flow motion leads to the differences in the pollutant transport process at the surface and bottom of the cross-section. It is worth noting that there is a small annular flow structure at the top corner of the section, which is an important incentive of faster vertical transport in S1 and S5. In addition, there is a strong turbulence structure at the bottom of the right bank within Section #04 to #06, but the mixing here is not significant.
3.3.2. Time-Averaged Concentration Flux
An effective method of analyzing the transport process of pollutants is the calculation of time-averaged concentration flux which represents the overall scalar transport rate.
Figure 12 and
Figure 13 show the cross-sectional averaged flux of concentration along the channel in the streamwise (
Fs) and transverse direction (
Ft), respectively.
Fs and are
Ft are calculated by the following equations:
where
U and
V denotes the time-averaged streamwise and transverse velocity, respectively;
n is the number of sampling points within the profiles. The sampling points are uniformly distributed on the whole profiles whose data are obtained by performing interpolations from the data in the cell centers.
In
Figure 12, the value of
Fs shows obvious deviations in the vicinity of release points, which arises from the gathered contaminant cloud with high concentration. The curves gradually converge and maintain the trend until the end of the domain for S1–S5, which indicates that complete mixing is achieved. However, for S6–S10 the
Fs rebound near the end of the domain, which may result from a significant difference in longitudinal velocity because the pollutants in S6–S10 are released in different positions in a streamwise direction. In
Figure 13, the
Ft in S1–S5 fluctuate along channel, presenting a nearly identical shape. These curve fluctuations result from the distinct strength of secondary circulation in different cross-sections. Stronger secondary motion leads to higher
Ft. Meanwhile, the
Ft in S6-S10 also fluctuates but with a shift between cases which also stems from the differences in streamwise release positions.
3.4. Instantaneous Field
The instantaneous flow characteristics and turbulence statistics of the concentration is analyzed in this section. The non-dimensional instantaneous quantities of streamwise velocity u* isolines (
Figure 14), secondary current vectors as well as vorticity
ωθ contours (
Figure 15) and concentration distribution contours of S1, S3, and S5 (
Figure 16) are displayed. For simplicity, only the slices of Section #04 and #07 were extracted, which are at the apex of the bend and the halfway point of the straight reach, respectively. Generally, the flow structure and concentration distribution are more disorganized and unstructured compared with time-averaged quantities. However, the high velocity region near the inner bank and a relevantly uniform velocity distribution in the straight channel, despite of the turbulence, can be observed. Moreover, the vectors of large-scale secondary motions are of similar directions and orders with time-averaged results. For the concentration field, the shapes of pollutant clouds of instantaneous values differ with that of time-averaged values, with a high spatial variability. Among three scenarios, S3 shows a higher mixing rate than the other two.
The root mean square fluctuations of concentration of S3 is shown in
Figure 17. As can be seen in the contours, the intensities of the concentration fluctuations are of the same order of magnitude with the time-averaged quantities. The concentration fluctuations are mainly found in the vicinity of the release position of the point source, which is in accordance with other research [
30,
31,
32]. The fluctuation plume significantly declines once it enters the straight reach (
Figure 17e), while the concentration itself is relevantly high.
3.5. Mixing Efficiency
In order to evaluate the mixing efficiency of pollutant, two indices were imposed for the assessment of mixing rate along the channel. The normalized root mean square of concentration
Cm within the profile is an effective parameter to quantify the uniformity of the pollutant’s spatial distribution, which have been widely used in similar studies [
33,
34]. The definition of
Cm can be expressed by:
where
Cav is the cross-sectional average concentration;
Ci is the concentration of sampling points whose data are obtained by performing interpolations from the data in the cell centers. A smaller vale of
Cm represents better mixing.
Figure 18 demonstrates the variations in
Cm of different scenarios along the channel. The curves of S1–S5 reveal a similar trend that the quantities all decrease sharply in the upstream half of the meander (region in Section #02–#06 marked on the
Figure 18a), and then come to a slow decline in the straight reach. In the downstream half of the meander (region in Section #08–#12 marked on the
Figure 18a) the curves gradually approach the horizontal axis and converge, which indicates that a good mixing was achieved among all the cases in this area; this is the case for S6–S10 in
Figure 18b. However, some deviations can be observed in the upstream half of the meander where the values of
Cm in S5 (
Figure 18a) and S10 (
Figure 18b) which are higher than the other cases, while the value of
Cm in S3 and S4 as well as S8 and S9 is smaller in the rest of the region. This implies that both cases obtain a higher mixing rate under the effect of secondary flow in the upstream half of the meander. It can be concluded from variations in
Cm that it is more likely to obtain a higher mixing rate when the point source is placed near the centerline in transverse and near the apex of the bend in streamwise. Furthermore, the mixing is mostly achieved in the first half of the meander period, while the mixing rate scarcely changes in the second half for all cases.
Another parameter proposed by Fischer [
35] is the percentage of complete mixing
P. It is generally considered that complete mixing is achieved if the concentration variations within a cross-section are ±5% of the downstream uniform concentration.
P is then calculated through the ratio of complete mixing area to the whole cross-sectional area. Normally, a larger
P represents a higher level of mixing.
Figure 19 demonstrates the varying
P of different scenarios along the channel. The curve demonstrates a clear distinction among cases along the channel. The S4 in
Figure 19a and S8 along with S9 in
Figure 19b present a higher level of mixing, which is in accordance with the conclusion drawn from
Cm.
The
Cm and
P curves present a similar trend and have minor differences in each case group. To further quantitatively distinguish the overall mixing efficiency in the computational domain among different cases, the mean value
Cm* and
P* were calculated by averaging the
Cm and
P of all cross-sections in each case.
Figure 20 displays the value of
Cm* and
P*, whereas the abscissa
W stands for the point source’s distance from the left bank in S1–S5, and the abscissa
Lb refers to the point source’s distance from the entrance of the bend in S6–S10. Generally, the point sources arranged near the centerline of the channel in transverse or near the apex of the bend in streamwise have relevantly lower
Cm* and higher
P*, which indicates a higher mixing rate. Specifically, the minimum value of
Cm* is found in S3 (
Figure 20a) and S8 (
Figure 20b) of each set of cases, with a value of 0.334 and 0.218, respectively. However, the maximum value of
P* is identified in S4 (
Figure 20a) and S10 (
Figure 20b), with a value of 0.228 and 0.295, respectively. This inconsistency indicates the contradiction between the two indices in picking the best-mixed scenario. As a result, an effective assessment of the pollutant’s mixing efficiency requires comprehensive consideration [
36] with more than one index.