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New Insights in Catalytic Oxidation Processes for Water Treatment
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New Insights in Catalytic Oxidation Processes for Water Treatment

A special issue of Water (ISSN 2073-4441). This special issue belongs to the section "Wastewater Treatment and Reuse".

Deadline for manuscript submissions: closed (10 August 2024) | Viewed by 7037

Special Issue Editors

Prof. Dr. Fei Qi

E-Mail Website
Guest Editor
College of Environmental Science and Engineering, Beijing Forestry University, Beijing 100083, China
Interests: advanced oxidation; water treatment; water reuse; nanotechnology; catalytic ozonation; membrane catalysis; photocatalysis; persulfate-based process
Dr. Yang Guo

E-Mail Website
Guest Editor
School of Environment and Resource, Shanxi University, Taiyuan 030006, China
Interests: advanced oxidation processes; catalytic ozonation; membrane catalysis; chemical kinetic modelling; emerging contaminants
Dr. Yinqiao Zhang

E-Mail Website
Guest Editor
School of Engineering, China Pharmaceutical University, Nanjing, China
Interests: water treatment; advanced oxidation process; electrochemistry; emerging contaminant; reactive species; non-radical process
Dr. Shangyi Li

E-Mail Website
Guest Editor
Department of Environmental Science and Engineering, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing 100029, China
Interests: water treatment; catalysts synthesis, advanced oxidation process; emerging contaminant; interface reaction
Special Issues, Collections and Topics in MDPI journals
Dr. Chen Li

E-Mail Website
Guest Editor
College of Environmental Science and Engineering, Beijing Forestry University, Beijing 100107, China
Interests: water treatment; catalytic ceramic membrane; nanofiltration; membrane fouling; photocatalysis; dissolved organic matters; pharmaceutically active compounds
Special Issues, Collections and Topics in MDPI journals

Special Issue Information

Dear Colleagues,

Catalytic oxidation processes have been considered as promising for water and wastewater treatment. During the catalytic oxidation processes, highly reactive radicals such as hydroxyl, sulfate, chlorine, and nitrogen radicals are generated to oxidize a broad range of refractory organics (emerging contaminants and certain inorganic pollutants, etc) or to increase biodegradability as a pre-treatment prior to an ensuing biological treatment. However, how to produce and utilize reactive radicals effectively and stably are very crucial to catalytic oxidation processes. The practical application of catalytic oxidation processes is challenged by the reaction rates, harmful byproducts, scaling-up, etc. This Special Issue will focus on the kinetic studying, mechanistic understanding, and large-scale applications of catalytic oxidation processes for water and wastewater treatment, including ozone-, UV-, H2O2-, Cl2-, persulfate-, membrane-based catalytic oxidation; electrocatalytic catalytic oxidation; and photocatalytic catalytic oxidation processes. Research articles, reviews, and short communications on relevant topics are welcomed.

Prof. Dr. Fei Qi
Dr. Yang Guo
Dr. Yinqiao Zhang
Dr. Shangyi Li
Dr. Chen Li
Guest Editors

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Water is an international peer-reviewed open access semimonthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2600 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • catalytic oxidation processes
  • ozone
  • ultraviolet
  • hydrogen peroxide
  • chlorine
  • persulfate
  • catalytic membrane
  • photocatalysis
  • water treatment

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Published Papers (4 papers)

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Research

11 pages, 1584 KiB  
Article
The Treatment of Antibiotic Excess Sludge via Catalytic Wet Oxidation with Cu-Ce/γ-Al2O3 and the Production of a Carbon Source
by Shangye Chu, Hai Lin and Xu Zeng
Water 2024, 16(9), 1249; https://doi.org/10.3390/w16091249 - 27 Apr 2024
Viewed by 912
Abstract
In the present study, the effectiveness of catalytic wet oxidation triggered by using Cu-Ce/γ-Al2O3 to degrade antibiotic excess sludge was investigated, during which some small molecule carboxylic acids were produced, which are valuable in biological wastewater treatment as an organic [...] Read more.
In the present study, the effectiveness of catalytic wet oxidation triggered by using Cu-Ce/γ-Al2O3 to degrade antibiotic excess sludge was investigated, during which some small molecule carboxylic acids were produced, which are valuable in biological wastewater treatment as an organic carbon source. The influence of reaction parameters on the degradation efficiency was explored through single-factor and orthogonal experiments, including catalyst amount, reaction temperature and time, and oxygen supply amount. The results illustrated that the treatment system can achieve 81.2% COD and 93.8% VSS removal rates under optimized reaction conditions. Carboxylic acids produced after the sludge degradation mainly included acetic acid, propanoic acid, etc. The results of wastewater biological treatment experiments exhibited that the degraded solution after catalytic wet oxidation has potential to be used as a carbon source to meet the demand of biological treatment, which helps the removal of COD and TN. This work confirms the effectiveness of catalyst for enhancing antibiotic excess sludge treatment, which provided a new idea for the rational disposal of antibiotic excess sludge. Full article
(This article belongs to the Special Issue New Insights in Catalytic Oxidation Processes for Water Treatment)
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24 pages, 7363 KiB  
Article
Multi-Heteroatom Doped Fe@CN Activation Peroxomonosulfate for the Removal of Trace Organic Contaminants from Water: Optimizing Fabrication and Performance
by Jiamin Chen, Ruijun Ren, Yatao Liu, Chen Li, Zhenbei Wang and Fei Qi
Water 2023, 15(24), 4241; https://doi.org/10.3390/w15244241 - 11 Dec 2023
Cited by 2 | Viewed by 1404
Abstract
Modification of catalysts by multi-heteroatom doping (S, P, B) is an effective way to improve the peroxomonosulfate activation performance of catalysts. In recent years, highly toxic and persistent trace organic contaminants have been frequently detected in water. Consequently, we proposed the advanced oxidation [...] Read more.
Modification of catalysts by multi-heteroatom doping (S, P, B) is an effective way to improve the peroxomonosulfate activation performance of catalysts. In recent years, highly toxic and persistent trace organic contaminants have been frequently detected in water. Consequently, we proposed the advanced oxidation processes of peroxomonosulfate activated by multi-heteroatom doped Fe@CN (X-Fe@CN) to eliminate trace organic contaminants. The physical phases of X-Fe@CN and its precursors were characterized by X-ray diffraction and scanning electron microscopy. In evaluating the catalytic properties and iron ion leaching of X-Fe@CN-activated PMS for the removal of dicamba and atenolol, B-Fe@CN and PB-Fe@CN were selected and optimized. The active sites of the catalysts were characterized by X-ray photoelectron spectroscopy and Raman. The pathways of PMS activation by B-Fe@CN and PB-Fe@CN were identified in combination with electron paramagnetic resonance and electrochemical experiments. Defects, O-B-O and pyrrolic nitrogen on the surface of B-Fe@CN could adsorb and activate PMS to produce SO4•−, ·OH and 1O2. Further doping with P enhanced the electron transfer on the catalyst surface, thus accelerating the activation of peroxomonosulfate. This study compared the effects of multi-heteroatom modifications and further demonstrated the synergistic effect between P and B, which can provide a theoretical basis for the selection of multi-heteroatom doped catalysts in water treatment. Full article
(This article belongs to the Special Issue New Insights in Catalytic Oxidation Processes for Water Treatment)
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19 pages, 1627 KiB  
Article
River Ecosystem Health Assessment in Rapid Urbanization Regions (Shenzhen, China) under the Guidance of Bioremediation Objectives
by Lan Fu, Xiaoyu Dong, Henglun Shen, Tianshun Zhu and Fangfang Sun
Water 2023, 15(21), 3859; https://doi.org/10.3390/w15213859 - 6 Nov 2023
Cited by 1 | Viewed by 2137
Abstract
As a coastal city with rapid urbanization and high-intensity human activities, Shenzhen, China has carried out a series of comprehensive treatments for water pollution control and ecological restoration in recent years. However, the restoration effect is mainly reflected in the improvement of water [...] Read more.
As a coastal city with rapid urbanization and high-intensity human activities, Shenzhen, China has carried out a series of comprehensive treatments for water pollution control and ecological restoration in recent years. However, the restoration effect is mainly reflected in the improvement of water quality and riparian landscape, and there is still a big gap in reaching the river’s ecological restoration goals. Therefore, it is necessary to make a full investigation and evaluation of river aquatic systems that focuses on the restoration of aquatic communities and ecosystem health. We surveyed forty-seven sampling sites in nine basins to investigate water quality and aquatic organisms (algae and macroinvertebrates) during the low-water period in 2019. Under the guidance of the EU Water Framework Directive (WFD), the urban river ecosystem health assessment system, with a total of twenty indicators from six criteria layers, was established. We addressed the bioremediation objectives in this system and aquatic organism indicators as high-weight characteristic indicators. The results showed that the degradation of the river ecosystem in Shenzhen is serious, which is mainly reflected in the simple structure of the aquatic biological community and the low biodiversity. Only one “healthy” sample site, accounting for 2% of the total sampling sites; six sites of “sub-health” level, accounting for 13%; twenty-four “poor” sample points, accounting for 51%; sixteen “extremely poor” sample points, accounting for 34%. From the perspective of spatial distribution, the river ecological status of Daya Bay Basin and Dapeng Bay Basin is good, which is at the level of “health” to “sub-health”; the Guanlan River Basin, Maozhou River Basin, Shenzhen River Basin, Shenzhen Bay Basin, Pingshan River Basin, and most of the Longgang River Basin are of “poor to extremely poor” grade; the Pearl Estuary basin is of “extremely poor” grade. This assessment system can be used as an effective tool to monitor the ecological health status, especially the enhancement of biodiversity and ecosystem function of rivers. Moreover, it could provide important decision-making guidance for river management affected by high-intensity human activities. Full article
(This article belongs to the Special Issue New Insights in Catalytic Oxidation Processes for Water Treatment)
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15 pages, 4342 KiB  
Article
Modeling BTEX Multiphase Partitioning with Soil Vapor Extraction under Groundwater Table Fluctuation Using the TMVOC Model
by Yang Yang, Jingwei Zheng, Juan Li, Huan Huan, Xiaobing Zhao, Ningqing Lv, Yan Ma and Hao Zhang
Water 2023, 15(13), 2477; https://doi.org/10.3390/w15132477 - 6 Jul 2023
Cited by 1 | Viewed by 1890
Abstract
The effects of groundwater table fluctuation (GTF) on the remediation of a petrochemically polluted riverside using soil vapor extraction (SVE) were investigated. The migration and transformation of benzene, toluene, ethylbenzene, and o-xylene (BTEX) in cases of natural attenuation, SVE without GTF, and SVE [...] Read more.
The effects of groundwater table fluctuation (GTF) on the remediation of a petrochemically polluted riverside using soil vapor extraction (SVE) were investigated. The migration and transformation of benzene, toluene, ethylbenzene, and o-xylene (BTEX) in cases of natural attenuation, SVE without GTF, and SVE with GTF were simulated using the TMVOC model. The results showed that the optimized extraction well pressure and influencing radius of the target site were 0.90 atm and 8 m, respectively. The removal rates of BTEX in cases of natural attenuation, SVE without GTF, and SVE with GTF were 11.49%, 85.16%, and 97.33%, respectively. The removal rate of BTEX was maximized in the case of SVE with a GTF amplitude of 0.5 m to 1 m. The removal rates of benzene (99.99%), toluene (99.74%), ethylbenzene (96.37%), and o-xylene (94.72%) were maximized in the case of SVE with GTF. For the cases of SVE without GTF and SVE with GTF, mass losses of BTEX in gaseous (0.05 kg, 0.05 kg, respectively) and aqueous phases (5.46 kg, 5.87 kg, respectively) were consistent. However, the mass loss of BTEX in the non-aqueous phase liquid (NAPL) phase in the case of SVE with GTF (155.13 kg) exceeded that in the case of SVE without GTF (135.41 kg). This is because GTF positively affected both the solubility and volatility of BTEX in the NAPL phase. With the groundwater table decreasing, flows of gas and gaseous pollutants increased by 25% along the vertical section. At this stage, the removal rates of volatile organic compounds can be further improved by increasing the flow of the extraction well. Full article
(This article belongs to the Special Issue New Insights in Catalytic Oxidation Processes for Water Treatment)
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