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Atmosphere, Volume 16, Issue 9 (September 2025) – 88 articles

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20 pages, 926 KB  
Article
Unveiling Microbial Diversity in Greek Urban Air and Recreational Seawater Using DNA Barcoding
by Angelina Metaxatos, Dafni Georgiadou, Dimitris G. Hatzinikolaou and Gediminas Mainelis
Atmosphere 2025, 16(9), 1082; https://doi.org/10.3390/atmos16091082 (registering DOI) - 14 Sep 2025
Abstract
Air and seawater samples were collected in 2022–2023 and analyzed through a common DNA extraction, purification, and Next-Generation Sequencing protocol. The study targeted bacteria, archaea, fungi, and plant-associated taxa to compare community structure across both milieus. Given the scarcity of data on environmental [...] Read more.
Air and seawater samples were collected in 2022–2023 and analyzed through a common DNA extraction, purification, and Next-Generation Sequencing protocol. The study targeted bacteria, archaea, fungi, and plant-associated taxa to compare community structure across both milieus. Given the scarcity of data on environmental microbiomes in Greece, we aimed to investigate further the diversity and variability of these microbiomes for the first time, using barcoding to provide data on microbial signatures in the air and seawater. Sequencing data revealed significant spatial and seasonal variability and a high diversity and richness of microbiome communities in both habitats. After quality filtering, we detected 21 phyla and 345 genera of bacteria and archaea, 3 phyla and 149 genera of fungi, and 17 Viridiplantae orders in the urban air. At the same time, in the recreational waters, we isolated 20 phyla and 420 genera of bacteria and archaea, 2 phyla, and 53 genera of fungi and 19 orders of Viridiplantae. Many of the fungal and bacterial taxa detected in this study can be potentially pathogenic. These findings highlight the potential of DNA barcoding as a reliable tool for integrative environmental monitoring, offering insights into the composition of environmental microbiomes. Microbiome monitoring is valuable for the environment and health, and it will be more efficient by integrating DNA analysis with the development of open databases and artificial intelligence. Full article
(This article belongs to the Section Air Quality)
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15 pages, 18587 KB  
Article
Ocean State Estimation in CESM via a Localized Particle Filter: Joint Assimilation of Satellite SST and In Situ TS Profiles
by Zheqi Shen, Yulong Yao and Yuting Zhang
Atmosphere 2025, 16(9), 1081; https://doi.org/10.3390/atmos16091081 (registering DOI) - 13 Sep 2025
Abstract
The recently developed localized particle filter (LPF) is extended to a fully coupled general circulation model (CGCM), specifically the Community Earth System Model (CESM), to assess its efficacy in assimilating multisource ocean observations, including satellite sea surface temperature (SST) and in situ temperature [...] Read more.
The recently developed localized particle filter (LPF) is extended to a fully coupled general circulation model (CGCM), specifically the Community Earth System Model (CESM), to assess its efficacy in assimilating multisource ocean observations, including satellite sea surface temperature (SST) and in situ temperature and salinity (TS) profiles. The LPF introduces localization in the weighting and resampling steps to avoid the filter degeneracy problem, thereby enhancing its performance in assimilating nonlinear systems. Data assimilation experiments using real ocean observations reveal that the LPF has notable advantages in improving the quality of subsurface and deep ocean temperature and salinity, particularly below 200 m. The results are evaluated against objective analysis data, confirming the potential applicability of the LPF in operational settings. Furthermore, a comparative analysis with the ensemble adjustment Kalman filter (EAKF) elucidates the merits and limitations of the LPF, and further underscores the pronounced advantage of LPF in the deep ocean. However, when TS profiles are already assimilated, supplementing the LPF with additional SST data produces adverse effects, a behavior markedly different from that of the EAKF. This discrepancy signals the need for refined data pre-processing strategies within the LPF in real operational applications. Full article
15 pages, 5053 KB  
Article
Beyond Global Trends: Two Decades of Climate Data in the World’s Highest Equatorial City
by Rasa Zalakeviciute, Fidel Vallejo, Bolívar Erazo, Oscar Chimborazo, Santiago Bonilla-Bedoya, Danilo Mejia, Tobias Isaac Tapia-Flores, Genesis Chuquimarca and Yves Rybarczyk
Atmosphere 2025, 16(9), 1080; https://doi.org/10.3390/atmos16091080 (registering DOI) - 12 Sep 2025
Abstract
While humanity stands at a critical point—one future leading toward sustainability, equity, and resilience, the other toward escalating conflicts, ecological collapse, and irreversible loss—climate change emerges as one of the most urgent challenges of the 21st century. The Global South, specifically the northwestern [...] Read more.
While humanity stands at a critical point—one future leading toward sustainability, equity, and resilience, the other toward escalating conflicts, ecological collapse, and irreversible loss—climate change emerges as one of the most urgent challenges of the 21st century. The Global South, specifically the northwestern South American region, lacks model confidence and reports on current climatic conditions due to gaps in historical data. This study, therefore, presents temperature and precipitation trends in the highest city on the equator, Quito, Ecuador, from 2004–2024. Six different districts were analyzed for maximum, average, and minimum temperatures, as well as cumulative precipitation, in terms of monthly and annual statistics, using Seasonal-Trend Decomposition. Over the past two decades, this Andean city has warmed by an average of +0.95 °C, with minimum temperatures rising at rates twice the global urban average of extreme urban heat islands (+2.47 °C), while precipitation has nearly doubled in rapidly developing parts of the city. These profound changes, shaped by urban expansion, El Niño–Southern Oscillation variability, and climate change, demand urgent adaptation in water management, urban planning, and climate resilience strategies, as well as comparative studies with rural Ecuador to differentiate local vs. regional climate signatures. Full article
(This article belongs to the Section Climatology)
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19 pages, 5134 KB  
Article
Spatial–Temporal Variations of Air Pollutants and Its Relationship with Meteorological Factors During 2014 to 2022 in Jiangsu Province, China
by Zihao Wu, Honglei Wang, Yue Ke, Yan Yin, Xuedong Zhou, Jinghua Chen, Kui Chen, Jun Guo, Jia Wang, Keqing Wang and Yixiao Wu
Atmosphere 2025, 16(9), 1079; https://doi.org/10.3390/atmos16091079 - 12 Sep 2025
Abstract
This study analyzes the spatial and temporal distribution characteristics of pollutants and the influence of meteorological factors using data from 13 cities in Jiangsu Province from 2014 to 2022. The results showed that, from 2014 to 2022, the average concentrations of PM2.5 [...] Read more.
This study analyzes the spatial and temporal distribution characteristics of pollutants and the influence of meteorological factors using data from 13 cities in Jiangsu Province from 2014 to 2022. The results showed that, from 2014 to 2022, the average concentrations of PM2.5, PM10, SO2, and CO in Jiangsu were high in the north and low in the south, while the NO2 concentration was low in the north and high in the south, all of which decreased over time. O3 concentration was higher on the eastern coast and increased with the year. PM2.5 pollution days in northern Jiangsu were higher in autumn and winter. O3 pollution days in southern Jiangsu were higher in spring, summer, and autumn. There was a significant positive correlation between O3 and temperature in spring and autumn, and it was weaker in summer. Relative humidity (RH) in winter was positively correlated with PM2.5 and RH showed a significant negative correlation with PM10 in spring, summer, and autumn. The scavenging effect of precipitation on PM10 concentration was the most pronounced, followed by PM2.5. Precipitation has the weakest scavenging effect on CO, only reducing its concentration by an average of 13%. Precipitation also exhibits a significant scavenging effect on O3. The decrease in O3 was the smallest on heavy rain days (14.7%) and the largest on severe, torrential rain days (25.9%). Full article
(This article belongs to the Section Air Quality)
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28 pages, 8552 KB  
Article
Identifying Optimal Reanalysis and Remote Sensing Data Combinations for Multi-Scale SPEI-Based Drought Assessment in Zhejiang Province, China
by Suli Pan, Di Ma, Haiting Gu, Chao Xu, Xiaojie Zhou and Qiang Zhu
Atmosphere 2025, 16(9), 1078; https://doi.org/10.3390/atmos16091078 - 12 Sep 2025
Viewed by 15
Abstract
Accurate drought assessment is crucial for effective regional water resource management. While reanalysis and remote sensing products enable high-resolution drought assessment, their regional application requires rigorous local validation. This study evaluates nine data combinations, pairing three precipitation products with three evapotranspiration products, to [...] Read more.
Accurate drought assessment is crucial for effective regional water resource management. While reanalysis and remote sensing products enable high-resolution drought assessment, their regional application requires rigorous local validation. This study evaluates nine data combinations, pairing three precipitation products with three evapotranspiration products, to identify the optimal combination for robust SPEI estimation and subsequently to investigate the spatiotemporal variations in drought conditions during 1980–2020 in Zhejiang Province, China. The results indicate that the choice of precipitation product is the dominant factor influencing SPEI accuracy, with the combination of CMFD V2.0 precipitation and GLEAM v4.2a evapotranspiration identified as the most reliable for SPEI estimation across multiple timescales (SPEI1/3/6/12). The long-term trend analysis of the SPEI derived from this optimal data combination reveals significant spatiotemporal heterogeneity: temporally, a pronounced “wetter winters, drier springs” seasonal pattern emerges, posing a substantial threat to agricultural water security; spatially, a distinct divergence shows central/northeastern areas wetting while southern/southeastern regions experience a significant drying trend, particularly for long-term hydrological drought (SPEI12). Additionally, the prevalence of light droughts across the province suggests a sustained baseline of water stress. Attribution analysis further demonstrates that precipitation is the dominant driver of droughts across all timescales. This study contributes both a validated, high-resolution data foundation for regional drought assessment and a scientific basis for targeted drought adaptation strategies. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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16 pages, 2959 KB  
Article
High-Time-Resolution Measurements of Equivalent Black Carbon in an Urban Background Site of Lecce, Italy
by Daniela Cesari, Ermelinda Bloise, Marianna Conte, Adelaide Dinoi, Giuseppe Deluca, Antonio Pennetta, Paola Semeraro, Eva Merico and Daniele Contini
Atmosphere 2025, 16(9), 1077; https://doi.org/10.3390/atmos16091077 - 11 Sep 2025
Viewed by 77
Abstract
Carbonaceous aerosols represent a significant component of atmospheric aerosol, with implications for climate and human health. The recent EU Directive 2024/2881 highlights the need to monitor emerging pollutants like black carbon more effectively. This study presents an brief field campaign at an urban [...] Read more.
Carbonaceous aerosols represent a significant component of atmospheric aerosol, with implications for climate and human health. The recent EU Directive 2024/2881 highlights the need to monitor emerging pollutants like black carbon more effectively. This study presents an brief field campaign at an urban background site aimed at characterizing carbonaceous aerosols. Daily samples of PM10 and PM2.5 were analyzed using a Sunset thermal-optical analyzer to determine organic and elemental carbon (OC, EC), while real-time equivalent black carbon (eBC) was measured with three independent instruments: MAAP, AE33, and Giano BC1. Total carbon (TC) was monitored using an online TCA08 thermo-catalytic analyzer. The average concentration of PM10 was 17.1 µg/m3 and 10.4 µg/m3 for PM2.5. On average, OC and EC represented 16.5% and 3.6% of PM10 mass, and 22.6% and 5.5% of PM2.5. SOC accounted for 36% of OC. The in situ Mass Absorption Cross-section (MAC), recalculated for the ECO site, was between 8.0 and 12.2 m2/g. eBC concentrations were modulated by the daily evolution of the planetary boundary-layer height and combustion sources. The apportionment of eBC was 65% from fossil fuel and 35% from biomass burning. Biomass-burning emissions were further confirmed by optical measurements, with BrC contributing 35% of absorption at 370 nm. Full article
(This article belongs to the Section Air Quality)
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27 pages, 3192 KB  
Article
Amplified Eastward SAPS Flows Observed in the Topside Ionosphere near Magnetic Midnight
by Ildiko Horvath and Brian C. Lovell
Atmosphere 2025, 16(9), 1076; https://doi.org/10.3390/atmos16091076 - 11 Sep 2025
Viewed by 161
Abstract
We report the exceptional observations of amplified eastward subauroral polarization streams (SAPS) made by the F15 spacecraft at ~840 km altitude near magnetic midnight during 2015–2016 in 17 events. The results show the dawn-cell-associated amplified eastward SAPS flows streaming alongside the duskward-extending dawn [...] Read more.
We report the exceptional observations of amplified eastward subauroral polarization streams (SAPS) made by the F15 spacecraft at ~840 km altitude near magnetic midnight during 2015–2016 in 17 events. The results show the dawn-cell-associated amplified eastward SAPS flows streaming alongside the duskward-extending dawn cell. The amplified eastward SAPS flows maximized at ~3200 m/s within their respective deep plasma density troughs, mimicking the SAPS flows and thus implying positive feedback mechanisms in action, where the electron temperature reached ~7000 K. One set of correlated magnetosphere–ionosphere conjugate observations is also presented. This illustrates the magnetotail-reconnection-related inward-directed cross-tail convection electric field (EC) reaching the near-earth plasmasheet’s tailward end, while the inward-directed SAPS E field was absent on the inner-magnetosphere plasmapause, and the emerging eastward SAPS flow in the conjugate ionosphere. These results provide observational evidence that the earthward-propagating inward-directed dawn–dusk cross-tail E field (1) mapped down to auroral latitudes with an equatorward direction, (2) propagated to subauroral latitudes, and (3) played a key role in the development of the emerging eastward SAPS flow and in the amplification of the fully-developed eastward SAPS flows near magnetic midnight, while positive feedback mechanisms supported further SAPS growth. Full article
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28 pages, 54121 KB  
Article
Effect of Friction Material on Vehicle Brake Particle Emissions
by Marie Hoff, Yan-Ming Chen, Laurent Meunier, Christophe Bressot and Martin Morgeneyer
Atmosphere 2025, 16(9), 1075; https://doi.org/10.3390/atmos16091075 - 11 Sep 2025
Viewed by 68
Abstract
This study focuses on the influence of different brake pad formulations on the emission of particulate matter coming from car braking systems. The brake particles were characterised using a pin-on-disc bench and some particle measuring devices such as CPC, APS, SMPS and a [...] Read more.
This study focuses on the influence of different brake pad formulations on the emission of particulate matter coming from car braking systems. The brake particles were characterised using a pin-on-disc bench and some particle measuring devices such as CPC, APS, SMPS and a PM10 sampling unit. Seven samples of brake pad materials of different compositions (1 NAO and 6 Low Steel) were tested against grey cast iron discs. The results presented in this work show differences in particle number concentration and PM10 emission factor between the different friction materials tested. Three friction materials, LS04, LS06 and NAO01, reduce particle number emissions by up to 71% and PM10 emissions by up to 57%. On the other hand, this reduction in particulate emissions goes along with a reduction of 20% to 27% in the coefficient of friction. The microscopic analyses carried out on the test parts (pins and discs) show differences between the most emissive and the least emissive friction pairs, which may explain the differences observed in particle emissions. Correlations between the emission of particles and the concentration of iron of the PM10, as well as the steel fibre content in the formulas, were found. Full article
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14 pages, 2284 KB  
Article
Multi-Aspect Analysis of Wildfire Aerosols from the 2023 Hongseong Case: Physical, Optical, Chemical, and Source Characteristics
by Jun-Oh Bu, Hee-Jung Ko, Hee-Jung Yoo and Sang-Min Oh
Atmosphere 2025, 16(9), 1074; https://doi.org/10.3390/atmos16091074 - 11 Sep 2025
Viewed by 103
Abstract
This study characterized the aerosol changes during the April 2023 Hongseong wildfire in Chungcheongnam-do, Korea, using physical, optical, and chemical data from the Anmyeon-do Global Atmosphere Watch station. The observation period was divided into three distinct phases: immediately after the wildfire (Period I), [...] Read more.
This study characterized the aerosol changes during the April 2023 Hongseong wildfire in Chungcheongnam-do, Korea, using physical, optical, and chemical data from the Anmyeon-do Global Atmosphere Watch station. The observation period was divided into three distinct phases: immediately after the wildfire (Period I), during precipitation (Period II), and the re-entry of wildfire smoke after precipitation (Period III). During Periods I and III, the PM10 mass concentrations were 75.7 ± 31.2 and 98.2 ± 55.6 µg/m3, respectively, which were approximately 2.4 and 3.1 times higher than the 2023 annual average (31.8 µg/m3) at the Anmyeon-do site. Aerosol scattering coefficients increased by factors of 4.0 and 6.9, and absorption coefficients by 5.5 and 4.2, respectively. Source apportionment using real-time data from a Monitor for Aerosols and Gases in ambient Air (MARGA) instrument combined with PCA demonstrated that aerosol emissions during Periods I and III were predominantly influenced by biomass burning sources. Analysis of PM10 and PM2.5 filter samples showed biomass burning markers, such as K+ and C2O42−, increased by 5.5–31.4 times compared with those in Period II. Elevated levels of combustion-related elements, including S, K, V, and Pb, further confirmed the influence of wildfire smoke on air quality during the affected periods. Full article
(This article belongs to the Section Aerosols)
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25 pages, 522 KB  
Article
Artificial Intelligence-Based Methods and Algorithms in Fog and Atmospheric Low-Visibility Forecasting
by Sancho Salcedo-Sanz, David Guijo-Rubio, Jorge Pérez-Aracil, César Peláez-Rodríguez, Antonio Manuel Gomez-Orellana and Pedro Antonio Gutiérrez-Peña
Atmosphere 2025, 16(9), 1073; https://doi.org/10.3390/atmos16091073 - 11 Sep 2025
Viewed by 174
Abstract
The accurate prediction of atmospheric low-visibility events due to fog, haze or atmospheric pollution is an extremely important problem, with major consequences for transportation systems, and with alternative applications in agriculture, forest ecology and ecosystems management. In this paper, we provide a comprehensive [...] Read more.
The accurate prediction of atmospheric low-visibility events due to fog, haze or atmospheric pollution is an extremely important problem, with major consequences for transportation systems, and with alternative applications in agriculture, forest ecology and ecosystems management. In this paper, we provide a comprehensive literature review and analysis of AI-based methods applied to fog and low-visibility events forecasting. We also discuss the main general issues which arise when dealing with AI-based techniques in this kind of problem, open research questions, novel AI approaches and data sources which can be exploited. Finally, the most important new AI-based methodologies which can improve atmospheric visibility forecasting are also revised, including computational experiments on the application of ordinal classification approaches to a problem of low-visibility events prediction in two Spanish airports from METAR data. Full article
(This article belongs to the Special Issue Numerical Simulation and Forecast of Fog)
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23 pages, 8778 KB  
Article
Performance Evaluation of Real-Time Sub-to-Seasonal (S2S) Rainfall Forecasts over West Africa of 2020 and 2021 Monsoon Seasons for Operational Use
by Eniola A. Olaniyan, Steven J. Woolnough, Felipe M. De Andrade, Linda C. Hirons, Elisabeth Thompson and Kamoru A. Lawal
Atmosphere 2025, 16(9), 1072; https://doi.org/10.3390/atmos16091072 - 11 Sep 2025
Viewed by 149
Abstract
Accurate sub-seasonal-to-seasonal (S2S) forecasts are critical for mitigating extreme weather impacts and supporting development in West Africa. This study evaluates real-time ECMWF S2S rainfall forecasts during the 2020–2021 West African monsoon (March–October) and uses corresponding hindcasts for comparison. We verify forecasts at 1–4 [...] Read more.
Accurate sub-seasonal-to-seasonal (S2S) forecasts are critical for mitigating extreme weather impacts and supporting development in West Africa. This study evaluates real-time ECMWF S2S rainfall forecasts during the 2020–2021 West African monsoon (March–October) and uses corresponding hindcasts for comparison. We verify forecasts at 1–4 dekads lead against two satellite-based rainfall datasets (TAMSAT and GPM-IMERG) to cover observational uncertainty. The analysis focuses on spatio-temporal monsoon patterns over the Gulf of Guinea (GoG) and Sahel (SAH). The results show that ECMWF-S2S captures key monsoon features. The forecast skill is generally higher over the Sahel than the GoG, and peaks during the main monsoon period (July–August). Notably, forecasts achieve approximately 80% synchronization with observed rainfall-anomaly timing, indicating that roughly 4 out of 5 dekads have correctly predicted wet/dry phases. Probabilistic evaluation shows strong reliability. The debiased ranked probability skill score (RPSS) is high across thresholds, whereas the average ROC AUC (~0.68) indicates moderate discrimination. However, forecasts tend to under-predict very low rains in the GoG and very high rains in the Sahel. Using multiple datasets and robust metrics helps mitigate observational uncertainty. These results, for the first real-time S2S pilot over West Africa, demonstrate that ECMWF rainfall forecasts are skillful and actionable (especially up to 2–3 dekads ahead), providing confidence for early-warning and planning systems in the region. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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27 pages, 1025 KB  
Review
The Asymmetry of the El Niño–Southern Oscillation: Characteristics, Mechanisms, and Implications for a Changing Climate
by Jin Liang, De-Zheng Sun, Biao Jin, Yifei Yang, Cuijiao Chu and Minjia Tan
Atmosphere 2025, 16(9), 1071; https://doi.org/10.3390/atmos16091071 - 11 Sep 2025
Viewed by 214
Abstract
The El Niño–Southern Oscillation (ENSO) is inherently asymmetric, a primary characteristic where its warm phase (El Niño) and cold phase (La Niña) differ in amplitude, spatial pattern, and temporal evolution. This review synthesizes over two decades of research to provide a comprehensive overview [...] Read more.
The El Niño–Southern Oscillation (ENSO) is inherently asymmetric, a primary characteristic where its warm phase (El Niño) and cold phase (La Niña) differ in amplitude, spatial pattern, and temporal evolution. This review synthesizes over two decades of research to provide a comprehensive overview of ENSO asymmetry. It systematically examines the observed manifestations, evaluates the competing physical mechanisms, and analyzes the ongoing challenges in climate modeling. The key findings in the literature indicate that this asymmetry is driven by complex interactions of nonlinear processes, where atmospheric mechanisms such as state-dependent westerly wind bursts and threshold responses of deep convection are now considered dominant driving factors, which are subsequently amplified and modulated by oceanic feedback. The main challenge in this field is that most of the current state-of-the-art climate models underestimate ENSO asymmetry, which is related to mean-state bias and brings uncertainty to future predictions. Furthermore, a key finding from recent projection studies is that while the asymmetry in ENSO’s sea surface temperature is expected to weaken in a warmer climate, the asymmetry of its global rainfall impacts may paradoxically be amplified. Future research should focus on balanced improvements in ocean and atmospheric model components, development of new diagnostic tools to clarify the roles of different feedbacks, or establishment of a framework that clearly links asymmetry to the full spectrum of ENSO diversity. By consolidating the current state of knowledge and highlighting key unresolved questions, this work provides an essential roadmap to improve the prediction and projection of Earth’s most far-reaching mode of climate variability. Full article
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29 pages, 2031 KB  
Review
Perfluorinated and Polyfluoroalkyl Compounds in the Atmosphere: A Review
by Haoran Yang, Ying Liang, Shili Tian, Xingru Li and Yanju Liu
Atmosphere 2025, 16(9), 1070; https://doi.org/10.3390/atmos16091070 - 10 Sep 2025
Viewed by 251
Abstract
Perfluoroalkyl and polyfluoroalkyl substances (PFASs) are a class of synthetic organic compounds with extremely high chemical stability and environmental persistence that are widely used in the industrial sector and in consumer goods. Their strong C-F bonds make them difficult to degrade, meaning they [...] Read more.
Perfluoroalkyl and polyfluoroalkyl substances (PFASs) are a class of synthetic organic compounds with extremely high chemical stability and environmental persistence that are widely used in the industrial sector and in consumer goods. Their strong C-F bonds make them difficult to degrade, meaning they can migrate through the atmosphere and settle over long distances, posing long-term risks to the global ecological environment and human health. This article systematically reviews the classification, physicochemical properties, concentration levels, spatial distribution, migration and transformation behaviors, and health and ecological impacts of PFASs in the atmosphere, along with related analytical detection techniques and pollution control methods. Studies show that short-chain PFASs are more likely to migrate through the atmosphere due to their high water solubility and volatility, while long-chain PFASs tend to be adsorbed onto particulate matter and display stronger bioaccumulation. Although atmospheric research on PFASs lags behind that focused on their dynamics in water and soil, the existing data still reveal a difference in their distribution and regional pollution characteristics in the gas and particle phases. Toxicological studies have confirmed that PFAS exposure is associated with liver injury, immunosuppression, developmental toxicity, and cancer risk and can threaten ecological security through the food chain. Currently, governance technologies are confronted with the challenges of low efficiency and high cost. In the future, it will be necessary to combine multi-media models, new analytical techniques, and international collaboration to promote the development of source control and innovative governance strategies. Full article
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17 pages, 1611 KB  
Article
Analysis of Airborne Fungal Spores in Lima, Perú (2021–2024): Seven Clinically Important Spore Types
by Alexa Paredes Idiaquez, Oscar Calderón-Llosa, Manuel Feliciano and Estefanía Sánchez-Reyes
Atmosphere 2025, 16(9), 1069; https://doi.org/10.3390/atmos16091069 - 10 Sep 2025
Viewed by 70
Abstract
Fungal spore calendars help illustrate the abundance and distribution of spores throughout the year, enabling clinicians and patients to predict and treat allergic symptoms based on spore presence and concentration. This three-year study (2021–2024) established the first fungal spore calendar for the most [...] Read more.
Fungal spore calendars help illustrate the abundance and distribution of spores throughout the year, enabling clinicians and patients to predict and treat allergic symptoms based on spore presence and concentration. This three-year study (2021–2024) established the first fungal spore calendar for the most clinically important spore types in Lima, Perú: Alternaria, Cladosporium, Nigrospora, Curvularia, Drechslera, Fusarium, and Stemphylium. Air sampling was performed using a Burkard volumetric spore trap placed on the rooftop of SANNA Clínica el Golf in San Isidro, Lima. Cladosporium was the most abundant (37,945 spores/m3), followed by Nigrospora (11,558), Curvularia (3946), Fusarium (2454), Alternaria (2138), Drechslera (1850), and Stemphylium (201). The highest concentrations of Alternaria, Nigrospora, Curvularia, and Drechslera were recorded in 2023–2024, with seasonal peaks mainly during spring/summer. Meteorological correlations showed that Alternaria, Cladosporium, Nigrospora, and Curvularia were positively correlated with temperature while Drechslera had a negative correlation. Cladosporium, Curvularia, Fusarium, and Stemphylium were negatively correlated with relative humidity, while other types showed a mix of both positive and negative responses or inverse responses. These two meteorological parameters are likely the main influences on spore concentrations; however, other factors may include other meteorological parameters. Cladosporium correlated positively with southwesterly winds, and negatively with northwesterly, winds, and Curvularia was positively correlated with northeasterly winds. Full article
(This article belongs to the Special Issue Airborne Fungal and Pteridophyte Spores)
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35 pages, 3181 KB  
Article
An Integrated Goodness-of-Fit and Vine Copula Framework for Windspeed Distribution Selection and Turbine Power-Curve Assessment in New South Wales and Southern East Queensland
by Khaled Haddad
Atmosphere 2025, 16(9), 1068; https://doi.org/10.3390/atmos16091068 - 10 Sep 2025
Viewed by 154
Abstract
Accurate modelling of near surface wind speeds is essential for robust resource assessment, turbine design, and grid integration. This study presents a unified framework comparing four candidate marginal distributions—Weibull, Gamma, Lognormal, and Generalised Extreme Value (GEV)—across 21 years of daily observations from 11 [...] Read more.
Accurate modelling of near surface wind speeds is essential for robust resource assessment, turbine design, and grid integration. This study presents a unified framework comparing four candidate marginal distributions—Weibull, Gamma, Lognormal, and Generalised Extreme Value (GEV)—across 21 years of daily observations from 11 sites in New South Wales and southern Queensland, Australia. Parameters are estimated by maximum likelihood, with L-moments used when numerical fitting fails. Univariate goodness-of-fit is evaluated via information criteria (Akaike Information Criterion, AIC; Bayesian Information Criterion, BIC) and distributional tests (Anderson–Darling, Cramér–von Mises, Kolmogorov–Smirnov). To capture spatial dependence, we fit an 11-dimensional regular vine (“R-vine”) copula to the probability-integral-transformed data, selecting pair-copula families by AIC and estimating parameters by sequential likelihood. A composite score (70% univariate, 30% copula) ranks distributions per location. Results demonstrate that Lognormal best matches central behaviour at most sites, Weibull remains competitive for bulk modelling, Gamma often excels in moderate tails, and GEV best represents extremes. All turbine yield results presented are illustrative, showing how statistical choices impact energy estimates; they should not be interpreted as operational forecasts. In a case study, 5000 joint simulations from the top-two models drive IEC V90 and E82 power curves, revealing up to 10% variability in annual energy yield due solely to marginal choice. This workflow provides a replicable template for comprehensive wind resource and load hazard analysis in complex terrains. Full article
(This article belongs to the Section Meteorology)
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16 pages, 2339 KB  
Article
Characterization of Secondary Aerosol Formation via HONO and HNO3 Reactions and Source Apportionment in Daejeon and Iksan, Republic of Korea
by Kyoung-Chan Kim, Yong-Jae Lim and Jin-Seok Han
Atmosphere 2025, 16(9), 1067; https://doi.org/10.3390/atmos16091067 - 10 Sep 2025
Viewed by 157
Abstract
This study investigates the atmospheric formation and sinks of HONO and HNO3 and their contribution to secondary PM2.5 formation in Daejeon (urban) and Iksan (suburban), South Korea. Continuous observations revealed distinct concentration patterns: Iksan exhibited elevated ammonia and nitrate levels associated [...] Read more.
This study investigates the atmospheric formation and sinks of HONO and HNO3 and their contribution to secondary PM2.5 formation in Daejeon (urban) and Iksan (suburban), South Korea. Continuous observations revealed distinct concentration patterns: Iksan exhibited elevated ammonia and nitrate levels associated with agricultural activities and biomass burning, while Daejeon showed higher NOx concentrations driven by traffic and industrial sources. Positive Matrix Factorization (PMF) analysis indicated that secondary formation was the dominant contributor to PM2.5 at both sites, with biomass burning exerting an additional influence in Iksan. Among observed precursors, HNO3 showed the highest conversion to aerosol nitrate, highlighting aerosol-phase reactions as its primary sink, followed by dry deposition. Seasonal analysis demonstrated that HONO loss was largely controlled by photolysis in summer. Externally transported aerosols contributed more than locally formed particles at both sites, emphasizing the role of regional background pollution. These findings provide a scientific basis for region-specific air quality strategies that combine local precursor control with the management of long-range transport. Full article
(This article belongs to the Section Aerosols)
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19 pages, 994 KB  
Article
Collaborative Analysis and Path Exploration of Atmospheric VOCs and Carbon Emissions in Textile Industry Enterprises: A Case Study of Suzhou
by Yuyan Chen, Jiahui Zhang, Yue He, Zhaoxiang Liu and Yun Pan
Atmosphere 2025, 16(9), 1066; https://doi.org/10.3390/atmos16091066 - 10 Sep 2025
Viewed by 166
Abstract
Achieving synergistic effects in pollution reduction and carbon mitigation is of great significance for promoting the comprehensive green transformation of economic and social development. This study focuses on the textile industry in a specific city, aiming to (1) analyze the energy consumption and [...] Read more.
Achieving synergistic effects in pollution reduction and carbon mitigation is of great significance for promoting the comprehensive green transformation of economic and social development. This study focuses on the textile industry in a specific city, aiming to (1) analyze the energy consumption and pollutant emission characteristics of the textile industry in a district of Suzhou from 2017 to 2021; (2) conduct carbon accounting for 18 typical textile enterprises using the emission factor method with extended accounting boundaries; and (3) explore targeted low-carbon collaborative control pathways for pollution and carbon reduction. The results show that from 2017 to 2021, the proportion of raw coal in the comprehensive energy consumption of the textile industry in the city decreased annually to 35.68%, while the proportion of natural gas increased to 13.96%. The adoption of natural gas significantly reduced carbon emissions. The industry’s total output value rose markedly, while energy consumption intensity declined noticeably. The production and emission of volatile organic compounds (VOCs) generally decreased, with the proportion of final combustion emissions of VOCs in carbon accounting being relatively low (0–19.79%). Based on the findings, this study provides strategic foundations for collaborative governance, including optimizing energy structures, substituting VOC-containing raw materials, and improving production processes. Full article
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23 pages, 7046 KB  
Article
Atmospheric Scattering Prior Embedded Diffusion Model for Remote Sensing Image Dehazing
by Shanqin Wang and Miao Zhang
Atmosphere 2025, 16(9), 1065; https://doi.org/10.3390/atmos16091065 - 10 Sep 2025
Viewed by 186
Abstract
Remote sensing image dehazing presents substantial challenges in balancing physical fidelity with generative flexibility, particularly under complex atmospheric conditions and sensor-specific degradation patterns. Traditional physics-based methods often struggle with nonlinear haze distributions, while purely data-driven approaches tend to lack interpretability and physical consistency. [...] Read more.
Remote sensing image dehazing presents substantial challenges in balancing physical fidelity with generative flexibility, particularly under complex atmospheric conditions and sensor-specific degradation patterns. Traditional physics-based methods often struggle with nonlinear haze distributions, while purely data-driven approaches tend to lack interpretability and physical consistency. To bridge this gap, we propose the Atmospheric Scattering Prior embedded Diffusion Model (ASPDiff), a novel framework that seamlessly integrates atmospheric physics into the diffusion-based generative restoration process. ASPDiff establishes a closed-loop feedback mechanism by embedding the atmospheric scattering model as a physics-driven regularization throughout both the forward degradation simulation and the reverse denoising trajectory. The framework operates through the following three synergistic components: (1) an Atmospheric Prior Estimation Module that uses the Dark Channel Prior to generate initial estimates of the transmission map and global atmospheric light, which are then refined through learnable adjustment networks; (2) a Diffusion Process with Atmospheric Prior Embedding, where the refined priors serve as conditional guidance during the reverse diffusion sampling, ensuring physical plausibility; and (3) a Haze-Aware Refinement Module that adaptively enhances structural details and compensates for residual haze via frequency-aware decomposition and spatial attention. Extensive experiments on both synthetic and real-world remote sensing datasets demonstrate that ASPDiff significantly outperforms existing methods, achieving state-of-the-art performance while maintaining strong physical interpretability. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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15 pages, 1849 KB  
Article
Determining Wind Shear Threshold by Using Historical Sounding Data in Experimental Area
by Tingting Shu, Qinglin Zhu, Xiang Dong, Houcai Chen, Leke Lin and Xuan Liu
Atmosphere 2025, 16(9), 1064; https://doi.org/10.3390/atmos16091064 - 10 Sep 2025
Viewed by 144
Abstract
This paper conducts a technical study on a method for determining the occurrence threshold of wind shear based on historical sounding data. After analyzing the impact of low-altitude wind shear on aircraft flight safety, a method for determining the occurrence threshold of wind [...] Read more.
This paper conducts a technical study on a method for determining the occurrence threshold of wind shear based on historical sounding data. After analyzing the impact of low-altitude wind shear on aircraft flight safety, a method for determining the occurrence threshold of wind shear based on historical sounding data is proposed. A statistical analysis of the sounding data from the test area over a period of 15 years from 2010 to 2024 has been conducted, which includes the occurrence events and probability statistics of 1000 m wind shear for all 12 months of the year. The simulation results validate the feasibility and effectiveness of the method for determining the occurrence threshold of wind shear based on historical sounding data in the test area, forming a method that can be extended to all altitude ranges of aircraft flight and all flight regions globally. This statistical method provides a technical foundation for the efficient detection of wind shear at local airports and enhances flight safety at these airports. Full article
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12 pages, 3945 KB  
Article
Land-Use Impacts on Soil Nutrients, Particle Composition, and Ecological Functions in the Green Heart of the Chang-Zhu-Tan Urban Agglomeration, China
by Qi Zhong, Zhao Shi, Cong Lin, Hao Zou, Pan Zhang, Ming Cheng, Tianyong Wan, Wei and Cong Zhang
Atmosphere 2025, 16(9), 1063; https://doi.org/10.3390/atmos16091063 - 10 Sep 2025
Viewed by 296
Abstract
Urban green hearts provide essential ecosystem services, including carbon sequestration, water purification, and hydrological regulation. The Green Heart Area of the Chang-Zhu-Tan Urban Agglomeration in Hunan Province, China, is the largest globally, and plays a critical role in regional water management. These functions [...] Read more.
Urban green hearts provide essential ecosystem services, including carbon sequestration, water purification, and hydrological regulation. The Green Heart Area of the Chang-Zhu-Tan Urban Agglomeration in Hunan Province, China, is the largest globally, and plays a critical role in regional water management. These functions are increasingly threatened by intensive land-use, while soil, as the foundational ecosystem component, mediates water retention, nutrient cycling, and erosion resistance. This study examined the effects of four land-use types—cropland, plantation, arbor woodland, and other woodland—on soil particle composition and key nutrients (organic carbon, total nitrogen, and total phosphorus). Statistical comparisons among land-use types were performed. Results indicated that silt was the dominant soil fraction across all land-uses (64–72%). Arbor woodland exhibited significantly higher sand content (29%) compared to cropland (19%; p < 0.05), suggesting improved water permeability and erosion resistance. Cropland showed elevated nutrient levels, with TN (1450.32 mg·kg−1) and TP (718.86 mg·kg−1) exceeding both national averages and those in arbor woodland. Coupled with acidic soil conditions (pH 5.23) and lower stoichiometric ratios (C/N: 10.82; C/P: 35.67; N/P: 3.29), these traits indicate an increased risk of nutrient leaching in croplands. In contrast, arbor woodland displayed more balanced C:N:P ratios (C/N: 12.21; C/P: 48.05; N/P: 3.84), supporting greater nutrient retention and aggregate stability. These findings underscore the significant influence of land-use type on soil ecological functions, including water infiltration, runoff reduction, and climate adaptability. The study highlights the importance of adopting conservation-oriented practices such as reduced tillage and targeted phosphorus management in croplands, alongside reforestation with native species, to improve soil structure and promote long-term ecological sustainability. Full article
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18 pages, 3309 KB  
Article
An Analysis of the Spatial-Temporal Characteristics and Regulatory Strategies Pertaining to CH4 Emissions in China from 2000 to 2023
by Lin Yang, Min Wang, Rupu Yang, Liping Li and Xiangzhao Feng
Atmosphere 2025, 16(9), 1062; https://doi.org/10.3390/atmos16091062 - 9 Sep 2025
Viewed by 151
Abstract
Methane (CH4), the second-largest global greenhouse gas and a key driver of tropospheric ozone formation, critically influences climate change and air quality. As the world’s largest CH4 emitter, China must develop targeted mitigation strategies to support its carbon peak and [...] Read more.
Methane (CH4), the second-largest global greenhouse gas and a key driver of tropospheric ozone formation, critically influences climate change and air quality. As the world’s largest CH4 emitter, China must develop targeted mitigation strategies to support its carbon peak and neutrality goals while reducing ozone pollution. Here, we analyzed the spatiotemporal evolution of provincial CH4 emissions in China from 2000 to 2023 using spatial autocorrelation, hotspot detection, trend analysis, and K-means clustering. Our results revealed a triphasic emission trajectory—rapid growth followed by stabilization and a recent resurgence—with all provinces except Tibet showing increasing trends. The energy sector emerged as the primary contributor, particularly in Inner Mongolia, Shanxi, and Shaanxi, whereas agricultural emissions dominated in pastoral regions, such as Inner Mongolia and Sichuan, and rice-growing areas, such as Hunan and Hubei. Coastal provinces, including Shandong, Jiangsu, and Guangdong, exhibited waste disposal as their predominant CH4 source. Based on these patterns, we classified the emission zones into four distinct typologies: coal-dominant, waste-dominant, oil-agriculture composite, and multifactorial systems, proposing tailored mitigation frameworks that integrate CH4 and ozone co-reduction. This study provides a spatially resolved foundation for synergistic climate and air quality governance in China. Full article
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8 pages, 679 KB  
Brief Report
Exploring the Relative Effects of Natural Gas and Biogas Cooking on Indoor Air Quality in Residential Kitchens
by Wande Benka-Coker, Kailey Sipe, Dinela Dedic, Alexander Jones, Bramley Hawkins, Emily Lyons, Matt Steiman and Megan Benka-Coker
Atmosphere 2025, 16(9), 1061; https://doi.org/10.3390/atmos16091061 - 9 Sep 2025
Viewed by 178
Abstract
Indoor air pollution from gas stove combustion remains a public health concern, given links to adverse cardiorespiratory health effects, yet few studies have characterized or compared the air quality impacts of different gas-based cooking fuels. We investigated kitchen-level concentrations of nitrogen dioxide (NO [...] Read more.
Indoor air pollution from gas stove combustion remains a public health concern, given links to adverse cardiorespiratory health effects, yet few studies have characterized or compared the air quality impacts of different gas-based cooking fuels. We investigated kitchen-level concentrations of nitrogen dioxide (NO2) and fine particulate matter (PM2.5) concentrations in four homes in Central Pennsylvania that used natural gas and/or biogas fueled stoves. We conducted time-resolved kitchen monitoring and assessed pollutant concentrations during cooking and non-cooking periods. We applied linear mixed-effect regression models with kitchen-level random effects and time-varying covariates to estimate the influence of fuel type on indoor air quality. During cooking, mean kitchen NO2 concentrations during cooking were more than 160% higher in homes using natural gas compared with biogas (95% confidence interval [CI]: 109.4%, 211.1%), although both levels remained below the WHO guideline. PM2.5 concentrations showed limited sensitivity to fuel type, with modest differences observed. Adjusted mixed-effect regression models revealed attenuated but consistent associations, with natural gas use increasing NO2 exposure by 2.8 ppb, or 60.3% (95% CI: 1.7, 4.6 ppb). These findings suggest further research into understanding the exposure and health benefits of alternative fuels in residential kitchen settings is merited. Full article
(This article belongs to the Special Issue Enhancing Indoor Air Quality: Monitoring, Analysis and Assessment)
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19 pages, 2861 KB  
Article
Airborne Hirst Volumetric Sampling Gives an Insight into Atmospheric Dispersion of Pollen and Fungal Spores
by Branko Sikoparija, Slobodan Birgermajer, Bojana Ivosevic, Vasko Sazdovski, Pia Viuf Ørby, Mathilde Kloster and Ulrich Gosewinkel
Atmosphere 2025, 16(9), 1060; https://doi.org/10.3390/atmos16091060 - 9 Sep 2025
Viewed by 205
Abstract
The volumetric Hirst method is considered a golden standard in aerobiology for determining particle number concentrations of bioaerosols. Using Hirst-type pollen and spore traps on mobile platforms (i.e., aircraft, cars, motorbikes, bicycles or carried by pedestrians) is anticipated to significantly enhance the spatial [...] Read more.
The volumetric Hirst method is considered a golden standard in aerobiology for determining particle number concentrations of bioaerosols. Using Hirst-type pollen and spore traps on mobile platforms (i.e., aircraft, cars, motorbikes, bicycles or carried by pedestrians) is anticipated to significantly enhance the spatial and temporal granularity of data for bioaerosol monitoring. Mobile sampling promises to enhance our understanding of bioaerosol dynamics, ecological interactions and the impact of human activities on airborne biological particles. In this article, we present the design and test of an airborne Hirst-type volumetric sampler. We followed a structured approach and incorporated the fundamental principles of the original design, while optimizing for size, weight, power and cost. Our portable Hirst-type volumetric sampler (FlyHirst) was attached to an ultralight aircraft, together with complementing instrumentation, and was tested for collection of atmospheric concentrations of pollen, fungal spores and hyphae. By linking the temporal resolution of the samples with the spatial position of the aircraft, using flight time, we calculated the spatial resolution of our measurements in 3D. In six summer flights over Denmark, our study revealed that the diversity of the recorded spores corresponded to the seasonal expectance. Urtica pollen was recorded up to 1300 m above ground (a.g.l.), and fungal spores up to 2100 m a.g.l. We suggest that, based on this proof-of-concept, FlyHirst can be applied on other mobile platforms or as a personal sampler. Full article
(This article belongs to the Section Air Quality)
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23 pages, 13731 KB  
Article
Time-Resolved On-Board Measurements of TRWP Using Distributed Particle Sensor Systems
by Guido Lehne, Sven Brandt, Frank Schiefer, Benjamin Oelze, Nadine Aschenbrenner, Malte Hothan, Georg-Peter Ostermeyer and Carsten Schilde
Atmosphere 2025, 16(9), 1059; https://doi.org/10.3390/atmos16091059 - 9 Sep 2025
Viewed by 217
Abstract
The focus of this article is on the measurement of tire and road wear particles (TRWPs) during vehicle operation. The long-term objective is to determine the sources of particulate matter. Consequently, the development of sustainable tires can be supported in the future by [...] Read more.
The focus of this article is on the measurement of tire and road wear particles (TRWPs) during vehicle operation. The long-term objective is to determine the sources of particulate matter. Consequently, the development of sustainable tires can be supported in the future by identifying factors influencing the concentration of particulate matter in vehicle-based tire tests. In an initial campaign, a test vehicle was equipped with a total of seven low-cost sensors (LCSs) for measurement campaigns on an isolated outdoor test track. The purpose of this was to evaluate the particle measurements in combination with GNSS data and driving data such as acceleration and speed. The potential observed in the initial investigation led to further investigations with an advanced, interconnectable modular particle and environmental sensor system (iMPES), which was developed in-house. The iMPES records measurement data for PM10 via the PMS7003 and PM100 via the SDS198 at 1 Hz over a period of up to 6 h, using a mobile power supply. The findings of the study indicate a robust characterization of the particle concentrations over the temporal and local course of the campaign drives. The results demonstrate the potential of the method to be part of a methodology to differentiate the particle sources and to derive influencing factors on the particulate matter concentration. The paper proposes a methodology for the mapping and analysis of lap-based data on a normalized route. Consequently, an inquiry into the local and driving-dependent dynamics is conducted, alongside a comparison with driving data. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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17 pages, 3662 KB  
Article
Numerical Study of Moisture Transfer and Methane Emission in Earthen Final Covers: Effects of Ambient Conditions
by Tao Wu, Song Feng, Cheng Chen, Guannian Chen and Zhangjing Zhang
Atmosphere 2025, 16(9), 1058; https://doi.org/10.3390/atmos16091058 - 8 Sep 2025
Viewed by 168
Abstract
Earthen final covers (EFCs) are widely used to mitigate environmental impacts from landfills, particularly in controlling methane emissions and groundwater contamination. In this study, a one-dimensional numerical model was built to simulate the interactions of liquid water, water vapor, landfill gas, and heat, [...] Read more.
Earthen final covers (EFCs) are widely used to mitigate environmental impacts from landfills, particularly in controlling methane emissions and groundwater contamination. In this study, a one-dimensional numerical model was built to simulate the interactions of liquid water, water vapor, landfill gas, and heat, incorporating the biochemical process of methane oxidation. Parametric studies revealed that both atmospheric and waste temperatures significantly influence the soil temperature and evaporation, thereby affecting methane oxidation. Oxidation efficiency increased from 8.7% to 55.3% as atmospheric temperature rose from 5 °C to 35 °C. High waste temperatures enhanced oxidation by up to 2.9 times under cold conditions. An increase in atmospheric pressure (950–990 mbar) promoted oxygen diffusion into the cover and improved oxidation efficiency from 0.8% to 77.1%. Atmospheric relative humidity also played a critical role by affecting surface evaporation, with higher humidity promoting better water retention but limiting oxygen diffusion. The methane oxidation performance of the cover declined by 12.0% to 68.5% compared to pre-rainfall conditions. Rainfall temporarily inhibited oxidation due to moisture-induced oxygen limitation, with partial recovery after rainfall ceased. This study provided valuable insights into the complex interactions between ambient conditions and EFC performance, contributing to the optimization of landfill cover designs and methane mitigation strategies. Full article
(This article belongs to the Section Biosphere/Hydrosphere/Land–Atmosphere Interactions)
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21 pages, 4617 KB  
Article
Spatiotemporal Analysis of Air Pollutants in Thessaloniki, Greece
by Anthi Chatzopoulou and Ilias Mavroidis
Atmosphere 2025, 16(9), 1057; https://doi.org/10.3390/atmos16091057 - 8 Sep 2025
Viewed by 324
Abstract
This study investigates the variability of major air pollutants, such as nitrogen oxides (NOx, including nitric oxide (NO) and nitrogen dioxide (NO2)), ozone (O3), and particulate matter with a diameter ≤ 10 µm (PM10), in Thessaloniki over [...] Read more.
This study investigates the variability of major air pollutants, such as nitrogen oxides (NOx, including nitric oxide (NO) and nitrogen dioxide (NO2)), ozone (O3), and particulate matter with a diameter ≤ 10 µm (PM10), in Thessaloniki over the period 2001–2022, highlighting their evolution in response to vehicle technology adoption and the COVID-19 pandemic. Four monitoring stations representing urban traffic, urban background, urban industrial, and suburban industrial environments were analyzed. PM10 concentrations generally decreased until 2015 but rose thereafter, mainly due to increased petrol car usage, with the highest levels recorded at the urban traffic station during colder months, influenced by domestic heating and local wind patterns. NO and NO2 concentrations peaked at urban traffic and industrial sites, closely linked to vehicle emissions and industrial activities, respectively, with notable reductions during the 2020 COVID-19 lockdown. O3 levels showed steady trends with diurnal and seasonal variability inversely related to NOx concentrations and positively correlated with temperature. Despite some pollutant reductions, air quality issues persist in Thessaloniki. The findings emphasize the need for robust governmental policies promoting cleaner heating alternatives; two policy scenarios are presented in this respect with the corresponding air pollutant concentrations estimates up to 2035. Full article
(This article belongs to the Special Issue Air Quality in Metropolitan Areas and Megacities (Second Edition))
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22 pages, 3520 KB  
Article
A Deep Learning–Random Forest Hybrid Model for Predicting Historical Temperature Variations Driven by Air Pollution: Methodological Insights from Wuhan
by Yu Liu and Yuanfang Du
Atmosphere 2025, 16(9), 1056; https://doi.org/10.3390/atmos16091056 - 8 Sep 2025
Viewed by 556
Abstract
With the continuous acceleration of industrialization, air pollution has become increasingly severe and has, to some extent, contributed to the progression of global climate change. Against this backdrop, accurate temperature forecasting plays a vital role in various fields, including agricultural production, energy scheduling, [...] Read more.
With the continuous acceleration of industrialization, air pollution has become increasingly severe and has, to some extent, contributed to the progression of global climate change. Against this backdrop, accurate temperature forecasting plays a vital role in various fields, including agricultural production, energy scheduling, environmental governance, and public health protection. To improve the accuracy and stability of temperature prediction, this study proposes a hybrid modeling approach that integrates convolutional neural networks (CNNs), Long Short-Term Memory (LSTM) networks, and random forests (RFs). This model fully leverages the strengths of CNNs in extracting local spatial features, the advantages of LSTM in modeling long-term dependencies in time series, and the capabilities of RF in nonlinear modeling and feature selection through ensemble learning. Based on daily temperature, meteorological, and air pollutant observation data from Wuhan during the period 2015–2023, this study conducted multi-scale modeling and seasonal performance evaluations. Pearson correlation analysis and random forest-based feature importance ranking were used to identify two key pollutants (PM2.5 and O3) and two critical meteorological variables (air pressure and visibility) that are strongly associated with temperature variation. A CNN-LSTM model was then constructed using the meteorological variables as input to generate preliminary predictions. These predictions were subsequently combined with the concentrations of the selected pollutants to form a new feature set, which was input into the RF model for secondary regression, thereby enhancing the overall model performance. The main findings are as follows: (1) The six major pollutants exhibit clear seasonal distribution patterns, with generally higher concentrations in winter and lower in summer, while O3 shows the opposite trend. Moreover, the influence of pollutants on temperature demonstrates significant seasonal heterogeneity. (2) The CNN-LSTM-RF hybrid model shows excellent performance in temperature prediction tasks. The predicted values align closely with observed data in the test set, with a low prediction error (RMSE = 0.88, MAE = 0.66) and a high coefficient of determination (R2 = 0.99), confirming the model’s accuracy and robustness. (3) In multi-scale forecasting, the model performs well on both daily (short-term) and monthly (mid- to long-term) scales. While daily-scale predictions exhibit higher precision, monthly-scale forecasts effectively capture long-term trends. A paired-sample t-test on annual mean temperature predictions across the two time scales revealed a statistically significant difference at the 95% confidence level (t = −3.5299, p = 0.0242), indicating that time granularity has a notable impact on prediction outcomes and should be carefully selected and optimized based on practical application needs. (4) One-way ANOVA and the non-parametric Kruskal–Wallis test were employed to assess the statistical significance of seasonal differences in daily absolute prediction errors. Results showed significant variation across seasons (ANOVA: F = 2.94, p = 0.032; Kruskal–Wallis: H = 8.82, p = 0.031; both p < 0.05), suggesting that seasonal changes considerably affect the model’s predictive performance. Specifically, the model exhibited the highest RMSE and MAE in spring, indicating poorer fit, whereas performance was best in autumn, with the highest R2 value, suggesting a stronger fitting capability. Full article
(This article belongs to the Section Atmospheric Techniques, Instruments, and Modeling)
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24 pages, 10838 KB  
Article
Assessing the Performance of the WRF Model in Simulating Squall Line Processes over the South African Highveld
by Innocent L. Mbokodo, Roelof P. Burger, Ann Fridlind, Thando Ndarana, Robert Maisha, Hector Chikoore and Mary-Jane M. Bopape
Atmosphere 2025, 16(9), 1055; https://doi.org/10.3390/atmos16091055 - 6 Sep 2025
Viewed by 461
Abstract
Squall lines are some of the most common types of mesoscale cloud systems in tropical and subtropical regions. Thunderstorms associated with these systems are among the major causes of weather-related disasters and socio-economic losses in many regions across the world. This study investigates [...] Read more.
Squall lines are some of the most common types of mesoscale cloud systems in tropical and subtropical regions. Thunderstorms associated with these systems are among the major causes of weather-related disasters and socio-economic losses in many regions across the world. This study investigates the capability of the Weather Research and Forecasting (WRF) model in simulating squall line features over the South African Highveld region. Two squall line cases were selected based on the availability of South African Weather Service (SAWS) weather radar data: 21 October 2017 (early austral summer) and 31 January–1 February 2018 (late austral summer). The European Centre for Medium-Range Weather Forecasts ERA5 datasets were used as observational proxies to analyze squall line features and compare them with WRF simulations. Mid-tropospheric perturbations were observed along westerly waves in both cases. These perturbations were coupled with surface troughs over central interior together with the high-pressure systems to the south and southeast of the country creating strong pressure gradients over the plateau, which also transports relative humidity onshore and extending to the Highveld region. The 2018 case also had a zonal structured ridging High, which was responsible for driving moisture from the southwest Indian Ocean towards the eastern parts of South Africa. Both ERA5 and WRF captured onshore near surface (800 hPa) winds and high-moisture contents over the eastern parts of the Highveld. A well-defined dryline was observed and well simulated for the 2017 event, while both ERA5 and WRF did not show any dryline for the 2018 case that was triggered by orography. While WRF successfully reproduced the synoptic-scale processes of these extreme weather events, the simulated rainfall over the area of interest exhibited a broader spatial distribution, with large-scale precipitation overestimated and convective rainfall underestimated. Our study shows that models are able to capture these systems but with some shortcomings, highlighting the need for further improvement in forecasts. Full article
(This article belongs to the Section Meteorology)
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18 pages, 3578 KB  
Article
Impacts of Climate Change on Streamflow to Ban Chat Reservoir
by Tran Khac Thac, Nguyen Tien Thanh, Nguyen Hoang Son and Vu Thi Minh Hue
Atmosphere 2025, 16(9), 1054; https://doi.org/10.3390/atmos16091054 - 5 Sep 2025
Viewed by 397
Abstract
Climate change is increasingly altering rainfall regimes and hydrological processes, posing major challenges to reservoir operation, flood control, and hydropower production. Understanding its impacts on the Ban Chat reservoir in Northwest Vietnam is therefore crucial for ensuring reliable water resource management under future [...] Read more.
Climate change is increasingly altering rainfall regimes and hydrological processes, posing major challenges to reservoir operation, flood control, and hydropower production. Understanding its impacts on the Ban Chat reservoir in Northwest Vietnam is therefore crucial for ensuring reliable water resource management under future uncertainties. This study aims to assess potential changes in streamflow to the Ban Chat reservoir under different climate change scenarios. The study employed nine Global Climate Models (GCMs) from the Coupled Model Intercomparison Project Phase 6 (CMIP6) under three Shared Socioeconomic Pathways (SSP1-2.6, SSP2-4.5, and SSP5-8.5). Future climate projections were bias-corrected using the Quantile Delta Mapping (QDM) method and used as input for the Hydrological Engineering Center–Hydrological Modeling System (HEC-HMS) to simulate future inflows. Streamflow changes were evaluated for near- (2021–2040), mid- (2041–2060), and late-century (2061–2080) periods relative to the baseline (1995–2014). Results show that under SSP1-2.6, mean annual discharge and flood-season flows steadily increase (up to +6.9% by 2061–2080), while storage deficits persist (−27.7% to −13.1%). Under SSP2-4.5, changes remain small, with flood peaks limited to +4.5% mid-century, but severe dry-season deficits continue (−29.5% to −24.4%). In contrast, SSP5-8.5 projects strong late-century increases in mean flows (+7.5%) and flood peaks (+8.2%), though early-century flood flows decline (−2.1%). These findings provide essential scientific evidence for adaptive reservoir operation, hydropower planning, and flood risk management, underscoring the significance of incorporating climate scenarios into sustainable water resource strategies in mountainous regions. Full article
(This article belongs to the Special Issue Hydrometeorological Extremes: Mechanisms, Impacts and Future Risks)
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24 pages, 4363 KB  
Article
Mechanistic Links Between Freeze–Thaw Cycles and Topsoil Erosion on the Qinghai–Tibet Plateau
by Zhenghu Ge, Kang Gao, Hongchao Dun, Ning Huang, Rezaali Pakzad and Yang Meng
Atmosphere 2025, 16(9), 1053; https://doi.org/10.3390/atmos16091053 - 5 Sep 2025
Viewed by 425
Abstract
The Qinghai-Tibet Plateau (QTP) is uniquely characterized by widespread permafrost and desertification due to its distinctive natural environment and geographic setting. The current lack of understanding regarding the mechanisms by which the number of freeze-thaw cycles (N) exacerbates soil erosion poses [...] Read more.
The Qinghai-Tibet Plateau (QTP) is uniquely characterized by widespread permafrost and desertification due to its distinctive natural environment and geographic setting. The current lack of understanding regarding the mechanisms by which the number of freeze-thaw cycles (N) exacerbates soil erosion poses a significant challenge to accurately assessing regional erosion dynamics. Here, we simulate realistic freeze-thaw conditions using an optimized cryogenic simulator and systematically quantify changes in soil physical properties, surface microstructure, and frost heave deformation. Research shows that as the number of freeze-thaw cycles rises, the surface soil moisture content decreases by 54.3%. Total porosity and bulk density display opposite trends. These changes in soil properties are mainly driven by frost heave forces disrupting soil cohesion. In particular, repeated water-ice phase transitions lead to continuous accumulation of axial frost heave stress, which rearranges soil particles. This significantly raises surface porosity with a growth rate as high as 60.3% and greatly reduces the soil’s resistance to external erosion. At the same time, the aggregate size distribution shifts toward finer particles, accompanied by a continued decrease in the mean weight diameter (MWD), which declines by approximately 8%. Notably, this degradation persists even when external loading partially suppresses frost heave. Therefore, the progressive physical degradation induced by frost heave-manifested through as moisture loss, porosity changes, aggregate breakdown, and compromised stability even under load-establishes the core mechanistic pathway through which freeze-thaw cycles intensify erosion in QTP soils. Full article
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