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Toxics
Special Issues
Advanced Processes for Wastewater Treatment
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Advanced Processes for Wastewater Treatment

A special issue of Toxics (ISSN 2305-6304). This special issue belongs to the section "Toxicity Reduction and Environmental Remediation".

Deadline for manuscript submissions: 13 September 2024 | Viewed by 1275

Special Issue Editors

Prof. Dr. Xueqing Shi

E-Mail Website
Guest Editor
School of Environmental and Municipal Engineering, Qingdao University of Technology, Qingdao 400233, China
Interests: persistent organic pollutants; biotoxicity; wastewater treatment; carbon neutral
Dr. Weilong Song

E-Mail Website
Guest Editor
Jiangsu Key Laboratory of Anaerobic Biotechnology, School of Environmental and Civil Engineering, Jiangnan University, Wuxi 214122, China
Interests: membrane separation; water reuse; advanced oxidation processes
Special Issues, Collections and Topics in MDPI journals
Dr. Binghan Xie

E-Mail Website
Guest Editor
School of Marine Science and Technology, Harbin Institute of Technology at Weihai, Weihai 264209, China
Interests: novel wastewater treatment process; resource recovery; environmental chemistry

Special Issue Information

Dear Colleagues,

Under the background of carbon neutral and ecosystem health recovery, a number of advanced processes have emerged in the field of wastewater treatment. Nowadays, the concept of “blue water factory” proposes that on top of treated water reuse, the pollutants from wastewater including chemical energy, biopolymers, nitrogen, phosphorus and cellulose should be recovered and reused through novel and advanced processes. Therefore, it is time for us to move forward from cost reduction or efficiency enhancement to the maximization of value recovery/generation through wastewater treatment. The aim of this Special Issue on “Advanced Processes for Wastewater Treatment” is to publish high-quality papers of original research or review articles addressing, but not limited to, the following topics: (i) novel processes for high-efficiency wastewater treatment with minimal environmental impact; (ii) transformation and toxicity evaluation of POPs, PAHs or other hazardous pollutants from wastewater through the treatment process; and (iii) resource recovery and reuse from wastewater by physical, chemical or biological means. Studies that are designed using a large-scale or long-term framework will be given high priority.

Prof. Dr. Xueqing Shi
Dr. Weilong Song
Dr. Binghan Xie
Guest Editors

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Toxics is an international peer-reviewed open access monthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2600 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • carbon neutral
  • persistent organic pollutants
  • emerging pollutants/new pollutants
  • resource recovery
  • water reuse
  • oxidative technologies
  • sorption technologies
  • bioreactor technologies
  • membrane-based technologies
  • toxicity index

Published Papers (1 paper)

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Research

16 pages, 3177 KiB  
Article
Persulfate–Based Advanced Oxidation Process for Chlorpyrifos Degradation: Mechanism, Kinetics, and Toxicity Assessment
by Youxin Xu, Chenxi Zhang, Haobing Zou, Guangrong Chen, Xiaomin Sun, Shuguang Wang and Huifang Tian
Toxics 2024, 12(3), 207; https://doi.org/10.3390/toxics12030207 - 9 Mar 2024
Viewed by 1027
Abstract
Persulfate-based advanced oxidation process has been proven to be a promising method for the toxic pesticide chlorpyrifos (CPY) degradation in wastewater treatment. However, due to the limitation for the short-lived intermediates detection, a comprehensive understanding for the degradation pathway remains unclear. To address [...] Read more.
Persulfate-based advanced oxidation process has been proven to be a promising method for the toxic pesticide chlorpyrifos (CPY) degradation in wastewater treatment. However, due to the limitation for the short-lived intermediates detection, a comprehensive understanding for the degradation pathway remains unclear. To address this issue, density functional theory was used to analyze the degradation mechanism of CPY at the M06-2X/6-311++G(3df,3pd)//M06-2X/6-31+G(d,p) level, and computational toxicology methods were employed to explore the toxicity of CPY and its degradation products. Results show that hydroxyl radicals (·OH) and sulfate radicals (SO4•−) initiate the degradation reactions by adding to the P=S bond and abstracting the H atom on the ethyl group, rather than undergoing α-elimination of the pyridine ring in the persulfate oxidation process. Moreover, the addition products were attracted and degraded by breaking the P–O bond, while the abstraction products were degraded through dealkylation reactions. The transformation products, including 3,5,6-trichloro-2-pyridynol, O,O-diethyl phosphorothioate, chlorpyrifos oxon, and acetaldehyde, obtained through theoretical calculations have been detected in previous experimental studies. The reaction rate constants of CPY with ·OH and SO4•− were 6.32 × 108 and 9.14 × 108 M−1·s−1 at room temperature, respectively, which was consistent with the experimental values of 4.42 × 109 and 4.5 × 109 M−1 s−1. Toxicity evaluation results indicated that the acute and chronic toxicity to aquatic organisms gradually decreased during the degradation process. However, some products still possess toxic or highly toxic levels, which may pose risks to human health. These research findings contribute to understanding the transformation behavior and risk assessment of CPY in practical wastewater treatment. Full article
(This article belongs to the Special Issue Advanced Processes for Wastewater Treatment)
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