The increasing availability of low-cost air quality sensors has led to novel sensing approaches. Distributed networks of low-cost sensors, together with data fusion and analytics, have enabled unprecedented, spatiotemporal resolution when observing the urban atmosphere. Several projects have demonstrated the potential of different approaches for high-resolution measurement networks ranging from static, low-cost sensor networks over vehicular and airborne sensing to crowdsourced measurements as well as ranging from a research-based operation to citizen science. Yet, sustaining the operation of such low-cost air quality sensor networks remains challenging because of the lack of regulatory support and the lack of an organizational framework linking these measurements to the official air quality network. This paper discusses the logical inclusion of lower-cost air quality sensors into the existing air quality network via a dynamic field calibration process, the resulting sustainable business models, and how this expansion can be self-funded. Full article

Aerosol vertical profiling is crucial to understand the formation mechanism and evolution processes of haze, which have not yet been comprehensively clarified. In this study, we investigated a severe, persistent haze event in Wuhan (30.5° N, 114.4° E), China during 5–18 January 2013 by the use of a polarization lidar, a Cimel sun photometer, meteorological datasets, and the hybrid single-particle Lagrangian integrated trajectory (HYSPLIT) model, focusing on the time–height evolution of aerosols in both the atmospheric boundary layer (ABL) and elevated layers. During the haze period, the integrated particle depolarization ratio was 0.05 ± 0.02, and the fine mode fraction reached 0.91 ± 0.03, indicating haze particles were rather spherical and predominately submicron, that is, of anthropogenic nature. Compared with the clear period, columnar aerosol optical depth at 500 nm tripled to 1.32 ± 0.31, and the strongest enhancement in aerosol concentration occurred from near the ground to an altitude of 1.2 km during the haze period. The daytime evolution of aerosol vertical distribution in the ABL exhibited a distinct pattern under haze weather. Abundant particles accumulated below 0.5 km in the morning hours due to stable meteorological conditions, including a strong surface-based inversion (4.4–8.1 °C), late development (from 1000–1100 LT) of the convective boundary layer, and weak wind (<4 m∙s⁻¹) in the lowermost troposphere. In the afternoon, improved ventilation delivered an overall reduction in boundary layer aerosols but was insufficient to eliminate haze. Particularly, the morning residual layer had an optical depth of 0.29–0.56. It influenced air quality indirectly by weakening convective activities in the morning and directly through the fumigation process around noon, suggesting it may be an important element in aerosol–ABL interactions during consecutive days with haze. Our lidar also captured the presence of the elevated aerosol layers (EALs) embodying regional/long-range transport. Most of the EALs were observed to subside to <1.2 km and exacerbate the pollution level. Backward trajectory analysis and lidar data revealed the EALs originated from the transport of anthropogenic pollutants from the Sichuan Basin, China, and of dust from the deserts in the northwest. They were estimated to contribute ~19% of columnar aerosol-loading, pointing to a non-negligible role of transport during the intense pollution episode. The results could benefit the complete understanding of aerosol–ABL interactions under haze weather and air quality forecasting and control in Wuhan. Full article

Beijing frequently experiences dust storms during spring, which result in deteriorated visibility and cause negative health impacts. In this paper, the dust particles were collected during a dust storm episode on 4–5 May 2017 in Beijing, and the samples before and after the dust storm were also collected. The morphology and elemental and mineralogical compositions of the dust samples were investigated using a transmission electron microscope equipped with an energy-dispersive X-ray spectrometer (TEM-EDX) and X-ray diffraction (XRD). The TEM-EDX results showed that the particles in the dust samples were mainly Si-rich, Ca-rich, S-rich, Fe-rich, Al-rich, Ti-rich, K-rich, Na-rich and Mg-rich particles. The XRD results demonstrated that the minerals in PM₁₀ samples were mainly clay, calcite, quartz, dolomite, plagioclase, potassium feldspar and hematite, in descending order of their contents. The clay minerals, having the highest content, were mainly kaolinite, chlorite and illite. The mixing state and aging degree of mineral particles before, during and after the dust storm episode behaved very differently. The mineral particles collected before and after the dust storm tended to have an internal mixing state, dominated by the S-rich particles internally mixed with alkaline mineral particles, revealing a more serious ageing degree. The mineral particles collected during the dust storm did not show clear internal mixing, revealing a less serious ageing degree. The amount of the Si-rich, Al-rich, Ca-rich and Ti-rich particles was highest during the dust storm, indicating that these particles mainly originated from long-distance transportation. The S-rich, Fe-rich, K-rich, Na-rich and Mg-rich particles were mainly enriched in the samples before and after the dust storm episode, indicating that they mainly originated from local sources. A comparison of the values of S/(Si + Al) in the individual particles with the particle sizes revealed that the finer mineral particles were associated with higher S contents before and after the dust storm, while the coarse particles were associated with lower S contents during the dust storm. Full article

We investigated the impacts of cold fronts on area-wide peak O₃ and regional background
O₃ mixing ratios on a daily scale over the Houston-Galveston-Brazoria (HGB) area of southeastern
Texas during the O₃ seasons (April–October) of 2003–2016. Back trajectories showed that an 18h time
lag existed between arrival of cold fronts in the HGB area and onset of a predominately northerly
flow. Cold fronts showed increasing effects on both peak and background O₃ over the HGB area.
Compared to no front days, average peak O₃ mixing ratios during the cold front 1st days, cold
front 2+ days, and post frontal days increased 0.7, 5.9, and 9.0 ppbv, respectively while average
background O₃ increased 2.9, 6.8, and 8.6 ppbv, respectively. The change in wind direction from
southerly to northerly was the most important factor causing increasing O₃ levels. Wind direction
shifts caused variation of other meteorological factors (i.e., wind speed, precipitation, temperature,
cloud cover, and relative humidity) and tended to overshadow their effects on O₃ over the HGB area.
On a long-term and large-scale view, cold fronts over the HGB area could be regarded as interruptions
in the cleansing effects of predominantly marine southerly flow from the Gulf of Mexico. Full article