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Challenges and Research Trends of Carbon Capture Utilization and Storage (CCUS)

A special issue of Energies (ISSN 1996-1073). This special issue belongs to the section "B3: Carbon Emission and Utilization".

Deadline for manuscript submissions: closed (17 March 2023) | Viewed by 21425

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Guest Editor
Department of Civil and Environmental Engineering, University of Perugia, Via G. Duranti 93, 06125 Perugia, Italy
Interests: natural gas hydrates; carbon capture and storage; methanation; gas mixture separation
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Special Issue Information

Dear Colleagues,

In addition to the development of strategies and technologies focused on the reduction in green-house gas emissions, the storage of those compounds represents a key factor to reach the main goals fixed in occasion of COP26 in terms of environment preservation and mitigation of the global climate change.

This Special Issue of Energies aims to collect relevant scientific contributions in the field of green-house gas capture and storage, with particular attention to carbon dioxide. Innovative solutions for gas storage, optimization of energy saving, reduction in costs associated to the processes, as well as utilization of proper and innovative “host” materials for gas storage are only some of the scientific topics that we will take into account.

We will also consider works focused on the reuse of these gases, in order to produce a second energetic cycle with the same final quantity of waste gas produced. In this sense, we will consider topics as methanation, power-to-gas and others.

Papers addressing any of these specific topics are welcome.

Dr. Alberto Maria Gambelli
Guest Editor

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Keywords

  • carbon capture and storage
  • chemical processes
  • environmental engineering
  • carbon dioxide reuse
  • innovative storage applications
  • process efficiency

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Published Papers (8 papers)

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Editorial

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4 pages, 177 KiB  
Editorial
CCUS Strategies as Most Viable Option for Global Warming Mitigation
by Alberto Maria Gambelli
Energies 2023, 16(10), 4077; https://doi.org/10.3390/en16104077 - 13 May 2023
Cited by 4 | Viewed by 1217
Abstract
The decarbonization of energy-consuming industrial sectors is nowadays becoming one of the most relevant challenges to counteract global warming and the consequences related to it [...] Full article

Research

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15 pages, 1600 KiB  
Article
Mitigation of CO2 Emissions from Commercial Ships: Evaluation of the Technology Readiness Level of Carbon Capture Systems
by Valentina Bortuzzo, Serena Bertagna and Vittorio Bucci
Energies 2023, 16(9), 3646; https://doi.org/10.3390/en16093646 - 24 Apr 2023
Cited by 5 | Viewed by 2946
Abstract
The challenge of achieving net-zero carbon emissions in the shipping sector is a pressing issue that is yet to be fully overcome. While new fuels and technologies hold promise for the future, they are not currently viable solutions on a large scale in [...] Read more.
The challenge of achieving net-zero carbon emissions in the shipping sector is a pressing issue that is yet to be fully overcome. While new fuels and technologies hold promise for the future, they are not currently viable solutions on a large scale in the short-term. One strategy that is being considered as a way to reduce CO2 and CO emissions in the immediate future is carbon capture technology. Additionally, the possibility of a carbon tax being implemented in the future further strengthens the case for the adoption of this technology, which is already quite mature and in use in industries, although it has yet to be developed in the maritime sector. In this paper, the authors start from the definition of carbon capture technology to provide a technical overview of the solutions that are currently available to the maritime sector. Given the absolute innovation of such systems for application on board ships, the authors studied their installation and developed appropriate schemes to illustrate the feasibility of integration of these new technologies on board. Furthermore, the authors highlight the different levels of technological readiness of the proposed systems based on their potential for implementation on board commercial vessels. Full article
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19 pages, 2830 KiB  
Article
Application of the Calcium Looping Process for Thermochemical Storage of Variable Energy
by Kelly Atkinson, Robin Hughes and Arturo Macchi
Energies 2023, 16(7), 3299; https://doi.org/10.3390/en16073299 - 6 Apr 2023
Cited by 3 | Viewed by 2146
Abstract
The calcium looping (CaL) process, which exploits the reversible calcination of calcium carbonate, has been proposed as a solution to the challenges facing deployment of concentrated solar power (CSP). As an extension of the work undertaken to date, this project proposes a novel [...] Read more.
The calcium looping (CaL) process, which exploits the reversible calcination of calcium carbonate, has been proposed as a solution to the challenges facing deployment of concentrated solar power (CSP). As an extension of the work undertaken to date, this project proposes a novel configuration of the CSP-CaL process which may offer advantages over other proposed configurations, including a reduction in process equipment requirements, elimination of pressure differentials between vessels, and a reduction in compression duty during the energy discharge period. The results obtained through process simulation indicate that the proposed process can achieve round-trip efficiencies in the range of 32–46% and energy storage densities in the range of 0.3–1.0 GJ/m3. These parameters are strongly dependent on the residual conversion of the CaO sorbent as well as the efficiency of the power cycles used to remove heat on the carbonator side of the process. Full article
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13 pages, 439 KiB  
Article
Media Coverage of Carbon Capture and Storage: An Analysis of Established and Emerging Themes in Dutch National Newspapers
by Emma ter Mors, Esther van Leeuwen, Christine Boomsma and Renate Meier
Energies 2023, 16(4), 2056; https://doi.org/10.3390/en16042056 - 20 Feb 2023
Cited by 2 | Viewed by 2439
Abstract
Policymakers in several European countries are considering the implementation of carbon capture and storage (CCS) technology as part of a strategy to prevent further climate change. Successful CCS implementation requires societal support but planned CCS projects have encountered significant opposition. In this study, [...] Read more.
Policymakers in several European countries are considering the implementation of carbon capture and storage (CCS) technology as part of a strategy to prevent further climate change. Successful CCS implementation requires societal support but planned CCS projects have encountered significant opposition. In this study, we examine the CCS coverage in Dutch national newspapers from 2017 to 2019, a period during which the Dutch CCS landscape underwent several substantial changes, and compare the results to those of earlier media analyses conducted between 1991 and 2011. Most of the 324 articles identified discussed CCS in a neutral (36.4%) or balanced (24.4%) manner, and more critical articles than supportive ones were found (23.1% vs. 16.0%). Consistent with the earlier media analyses, the potential of CCS to reduce carbon dioxide emissions was a major theme in the positive portrayal of CCS, while the argument that CCS implementation is needed for the prompt reduction in emissions gained prominence. High CCS deployment costs and the perception that CCS is an unproven technology have remained major themes in the negative portrayal of CCS. The availability of and preference for alternative solutions was a more prominent theme in the conversation compared to earlier years, whereas the subject of CCS safety was discussed less than before. The study illustrates how media coverage can shed light on the evolving relationships between society and CCS, and on the established and emerging themes in arguments used for and against the technology. Full article
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15 pages, 6805 KiB  
Article
Utilization of a Commercial 3D Printer for the Construction of a Bio-Hybrid Device Based on Bioink and Adult Human Mesenchymal Cells
by Giulio Morelli, Teresa Pescara, Alessia Greco, Pia Montanucci, Giuseppe Basta, Federico Rossi, Riccardo Calafiore and Alberto Maria Gambelli
Energies 2023, 16(1), 374; https://doi.org/10.3390/en16010374 - 29 Dec 2022
Cited by 2 | Viewed by 1776
Abstract
The biofabrication of three-dimensional scaffolds using 3D printers and cell-containing bioinks is very promising. A wide range of materials and bioink compositions are being created and tested for cell viability and printability in order to satisfy the requirements of a bioink. This methodology [...] Read more.
The biofabrication of three-dimensional scaffolds using 3D printers and cell-containing bioinks is very promising. A wide range of materials and bioink compositions are being created and tested for cell viability and printability in order to satisfy the requirements of a bioink. This methodology has not still achieved technological maturity, and the actual costs mean that they are often inaccessible for researchers, consequently lowering the development and extending the required times. This research aims to apply this methodology on a laboratory scale by re-adapting a commercial 3D printer, consequently lowering the costs and energy impacts, and, at the same time, ensuring a level of accuracy extremely close to the currently adopted devices and, more in general, suitable for the scopes of the research. To accomplish this, we assembled a biomimetic scaffold made of human Umbilical Cord Matrix Stem Cells (hUCMS), cellulose, and alginate. Various molds were used to produce 3D scaffolds of different sizes. After bioprinting, cell viability was analyzed using ethidium bromide and fluorescein diacetate, and a histological stain was used to evaluate cell and bioink morphology. All of the examined bioinks had a uniform final 3D structure and were stable, easily printable, and procedure-adapted. Up until 21 days of culture, the bioinks remained unaltered and were simple to manipulate. After 7 and 21 days of cell culture, the hUCMS in the cellulose/alginate-based bioinks exhibited cell viabilities of 95% and 85%, respectively. The cells did not present with a fibroblast-like shape but appeared to be round-shaped and homogeneously distributed in the 3D structure. Biomimetic bioink, which is based on cellulose and alginate, is an appropriate hydrogel for 3D bioprinting. This preliminary work illustrated the potential use of these two biomaterials for the 3D bioprinting of mesenchymal stem cells. Full article
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16 pages, 4438 KiB  
Article
Experimental Study on the Effect of SDS and Micron Copper Particles Mixture on Carbon Dioxide Hydrates Formation
by Yan Li, Alberto Maria Gambelli and Federico Rossi
Energies 2022, 15(18), 6540; https://doi.org/10.3390/en15186540 - 7 Sep 2022
Cited by 17 | Viewed by 2210
Abstract
CO2 hydrate formation and dissociation are the fundamental processes for investigating hydrate-based carbon storage. To better understand CO2 hydrate phase behaviors in the presence of surfactant and solid additives, this study reports the effects of Sodium Dodecyl Sulfate (SDS) and micron [...] Read more.
CO2 hydrate formation and dissociation are the fundamental processes for investigating hydrate-based carbon storage. To better understand CO2 hydrate phase behaviors in the presence of surfactant and solid additives, this study reports the effects of Sodium Dodecyl Sulfate (SDS) and micron Cu particles on the formation of CO2 hydrates in the presence of porous quartz sands in a lab-scale reactor. This research is part of a wider study focused on defining the properties of solid additives, produced via gas-atomization, on the formation and dissociation of gas hydrates. The morphology of CO2 hydrate formed in SDS solution shows dispersed crystal particles due to the increase of surface tension. SDS works as the kinetic promoter on CO2 hydrates formation whereas the addition of Cu particles inhibits CO2 gas consumption. The mixture additives show a faint kinetic inhibit effect, in which the Brownian motion restrictions may be responsible for the inhibition of CO2 hydrate production. The solid additives also showed a weak thermodynamic effect on CO2 hydrate phase equilibrium. Full article
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15 pages, 2296 KiB  
Article
A Novel Measurement-Based Method for Assessing Global Warming Mitigation via High-Albedo Solutions
by Federico Rossi, Mirko Filipponi, Beatrice Castellani, Stefania Bonafoni and Chaouki Ghenai
Energies 2022, 15(15), 5695; https://doi.org/10.3390/en15155695 - 5 Aug 2022
Cited by 5 | Viewed by 2018
Abstract
Global warming mitigation via terrestrial albedo increase has been widely investigated in literature; the proposed methodologies relate CO2 compensation to albedo increase generally via the concept of Radiative Forcing (RF). However, literature methods calculate RF by averaged input data, without [...] Read more.
Global warming mitigation via terrestrial albedo increase has been widely investigated in literature; the proposed methodologies relate CO2 compensation to albedo increase generally via the concept of Radiative Forcing (RF). However, literature methods calculate RF by averaged input data, without considering RF variation due to many local and temporal phenomena. For instance, an average value of compensated effect of albedo change (Δα = 0.01) is 3 kg CO2eq/m2, which has been introduced no matter the position and climatic condition of the site. In our study, we propose a novel procedure to measure RF continuous time history by means of ground measurements, astronomical equations, and satellite calibration. The procedure is called RF-meter. In this way, a more accurate assessment of compensated CO2 may be achieved. A test facility is also designed and proposed to double check the procedure, and preliminary results are reported in order to show and test the calibration procedure. It is expected that albedo-increased surfaces as well as cool roofs and/or other technical solutions will be eligible to obtain Emission Credits (EC). The proposed procedure will aid in the assignment of EC to High-Albedo Solutions (HAS), as it could represent an objective and accurate method to relate the albedo increase to a corresponding CO2 offset. Full article
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Review

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29 pages, 2289 KiB  
Review
A Review of Carbon Capture and Valorization Technologies
by Jiban Podder, Biswa R. Patra, Falguni Pattnaik, Sonil Nanda and Ajay K. Dalai
Energies 2023, 16(6), 2589; https://doi.org/10.3390/en16062589 - 9 Mar 2023
Cited by 24 | Viewed by 5446
Abstract
Global fossil fuel consumption has induced emissions of anthropogenic carbon dioxide (CO2), which has emanated global warming. Significant levels of CO2 are released continually into the atmosphere from the extraction of fossil fuels to their processing and combustion for heat [...] Read more.
Global fossil fuel consumption has induced emissions of anthropogenic carbon dioxide (CO2), which has emanated global warming. Significant levels of CO2 are released continually into the atmosphere from the extraction of fossil fuels to their processing and combustion for heat and power generation including the fugitive emissions from industries and unmanaged waste management practices such as open burning of solid wastes. With an increase in the global population and the subsequent rise in energy demands and waste generation, the rate of CO2 release is at a much faster rate than its recycling through photosynthesis or fixation, which increases its net accumulation in the atmosphere. A large amount of CO2 is emitted into the atmosphere from various sources such as the combustion of fossil fuels in power plants, vehicles and manufacturing industries. Thus, carbon capture plays a key role in the race to achieve net zero emissions, paving a path for a decarbonized economy. To reduce the carbon footprints from industrial practices and vehicular emissions and attempt to mitigate the effects of global warming, several CO2 capturing and valorization technologies have become increasingly important. Hence, this article gives a statistical and geographical overview of CO2 and other greenhouse gas emissions based on source and sector. The review also describes different mechanisms involved in the capture and utilization of CO2 such as pre-combustion, post-combustion, oxy-fuels technologies, direct air capture, chemical looping combustion and gasification, ionic liquids, biological CO2 fixation and geological CO2 capture. The article also discusses the utilization of captured CO2 for value-added products such as clean energy, chemicals and materials (carbonates and polycarbonates and supercritical fluids). This article also highlights certain global industries involved in progressing some promising CO2 capture and utilization techniques. Full article
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